Importance of Many Particle Correlations to the Collective Debye–Waller Factor in a Single-Particle Activated Dynamic Theory of the Glass Transition

Ghosh, Ashesh

doi:10.1021/acs.jpcb.3c02089

Importance of Many Particle Correlations to the Collective Debye–Waller Factor in a Single-Particle Activated Dynamic Theory of the Glass Transition

Journal Article · 25 May 2023 · Journal of Physical Chemistry. B

DOI:https://doi.org/10.1021/acs.jpcb.3c02089· OSTI ID:2419236

^[1]

Department of Chemical Engineering, Stanford University, Stanford, California 94305, USA; OSTI

Not provided.

Research Organization:: Univ. of Illinois at Urbana-Champaign, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

DOE Contract Number:: FG02-07ER46471

OSTI ID:: 2419236

Journal Information:: Journal of Physical Chemistry. B, Journal Name: Journal of Physical Chemistry. B Journal Issue: 22 Vol. 127; ISSN 1520-6106

Publisher:: American Chemical Society

Country of Publication:: United States

Language:: English

References (38)

Relaxation in glassforming liquids and amorphous solids Angell, C. A.; Ngai, K. L.; McKenna, G. B. Journal of Applied Physics, Vol. 88, Issue 6 https://doi.org/10.1063/1.1286035	journal	September 2000
Transport coefficients in glassy colloidal fluids Saltzman, Erica J.; Schweizer, Kenneth S. The Journal of Chemical Physics, Vol. 119, Issue 2 https://doi.org/10.1063/1.1578633	journal	July 2003
Microscopic Theory of Softness in Supercooled Liquids Nandi, Manoj Kumar; Bhattacharyya, Sarika Maitra Physical Review Letters, Vol. 126, Issue 20 https://doi.org/10.1103/PhysRevLett.126.208001	journal	May 2021
Role of the Pair Correlation Function in the Dynamical Transition Predicted by Mode Coupling Theory Nandi, Manoj Kumar; Banerjee, Atreyee; Dasgupta, Chandan Physical Review Letters, Vol. 119, Issue 26 https://doi.org/10.1103/PhysRevLett.119.265502	journal	December 2017
Microscopic theory of onset of decaging and bond-breaking activated dynamics in ultradense fluids with strong short-range attractions Ghosh, Ashesh; Schweizer, Kenneth S. Physical Review E, Vol. 101, Issue 6 https://doi.org/10.1103/PhysRevE.101.060601	journal	June 2020
Atomic Dynamics in Simple Liquid: de Gennes Narrowing Revisited Wu, Bin; Iwashita, Takuya; Egami, Takeshi Physical Review Letters, Vol. 120, Issue 13 https://doi.org/10.1103/PhysRevLett.120.135502	journal	March 2018
Relaxation processes in supercooled liquids Gotze, W.; Sjogren, L. Reports on Progress in Physics, Vol. 55, Issue 3 https://doi.org/10.1088/0034-4885/55/3/001	journal	March 1992
Theoretical perspective on the glass transition and amorphous materials Berthier, Ludovic; Biroli, Giulio Reviews of Modern Physics, Vol. 83, Issue 2 https://doi.org/10.1103/RevModPhys.83.587	journal	June 2011
Mode-coupling theory Reichman, David R.; Charbonneau, Patrick Journal of Statistical Mechanics: Theory and Experiment, Vol. 2005, Issue 05 https://doi.org/10.1088/1742-5468/2005/05/P05013	journal	May 2005
Thermodynamics–Structure–Dynamics Correlations and Nonuniversal Effects in the Elastically Collective Activated Hopping Theory of Glass-Forming Liquids Mei, Baicheng; Zhou, Yuxing; Schweizer, Kenneth S. The Journal of Physical Chemistry B, Vol. 124, Issue 28 https://doi.org/10.1021/acs.jpcb.0c03613	journal	July 2020
The role of attractive forces in viscous liquids Berthier, Ludovic; Tarjus, Gilles The Journal of Chemical Physics, Vol. 134, Issue 21 https://doi.org/10.1063/1.3592709	journal	June 2011
Elastically cooperative activated barrier hopping theory of relaxation in viscous fluids. I. General formulation and application to hard sphere fluids Mirigian, Stephen; Schweizer, Kenneth S. The Journal of Chemical Physics, Vol. 140, Issue 19 https://doi.org/10.1063/1.4874842	journal	May 2014
Microscopic Theory for the Role of Attractive Forces in the Dynamics of Supercooled Liquids Dell, Zachary E.; Schweizer, Kenneth S. Physical Review Letters, Vol. 115, Issue 20 https://doi.org/10.1103/PhysRevLett.115.205702	journal	November 2015
De Gennes Narrowing and Hard-Sphere Approach Sobolev, Oleg The Journal of Physical Chemistry B, Vol. 120, Issue 37 https://doi.org/10.1021/acs.jpcb.6b04685	journal	August 2016
Elastically cooperative activated barrier hopping theory of relaxation in viscous fluids. II. Thermal liquids Mirigian, Stephen; Schweizer, Kenneth S. The Journal of Chemical Physics, Vol. 140, Issue 19 https://doi.org/10.1063/1.4874843	journal	May 2014
Measurement of the self-intermediate scattering function of suspensions of hard spherical particles near the glass transition van Megen, W.; Mortensen, T. C.; Williams, S. R. Physical Review E, Vol. 58, Issue 5 https://doi.org/10.1103/PhysRevE.58.6073	journal	November 1998
Toward a microscopic basis for the de Gennes narrowing Kleban, Peter Journal of Statistical Physics, Vol. 11, Issue 4 https://doi.org/10.1007/BF01009791	journal	October 1974
Entropic barriers, activated hopping, and the glass transition in colloidal suspensions Schweizer, Kenneth S.; Saltzman, Erica J. The Journal of Chemical Physics, Vol. 119, Issue 2 https://doi.org/10.1063/1.1578632	journal	July 2003
Unified Theory of Activated Relaxation in Liquids over 14 Decades in Time Mirigian, Stephen; Schweizer, Kenneth S. The Journal of Physical Chemistry Letters, Vol. 4, Issue 21 https://doi.org/10.1021/jz4018943	journal	October 2013
Critical test of the mode-coupling theory of the glass transition Berthier, Ludovic; Tarjus, Gilles Physical Review E, Vol. 82, Issue 3 https://doi.org/10.1103/PhysRevE.82.031502	journal	September 2010
The role of collective elasticity on activated structural relaxation, yielding, and steady state flow in hard sphere fluids and colloidal suspensions under strong deformation Ghosh, Ashesh; Schweizer, Kenneth S. The Journal of Chemical Physics, Vol. 153, Issue 19 https://doi.org/10.1063/5.0026258	journal	November 2020
Slow dynamics in glycerol: collective de gennes narrowing and independent angstrom motion Saito, Makina; Kobayashi, Yasuhiro; Masuda, Ryo Hyperfine Interactions, Vol. 237, Issue 1 https://doi.org/10.1007/s10751-016-1243-3	journal	February 2016
Experimental test of a predicted dynamics–structure–thermodynamics connection in molecularly complex glass-forming liquids Mei, Baicheng; Zhou, Yuxing; Schweizer, Kenneth S. Proceedings of the National Academy of Sciences, Vol. 118, Issue 18 https://doi.org/10.1073/pnas.2025341118	journal	April 2021
Mode-Coupling Theory of the Glass Transition: A Primer Janssen, Liesbeth M. C. Frontiers in Physics, Vol. 6 https://doi.org/10.3389/fphy.2018.00097	journal	October 2018
Attractive versus truncated repulsive supercooled liquids: The dynamics is encoded in the pair correlation function Landes, François P.; Biroli, Giulio; Dauchot, Olivier Physical Review E, Vol. 101, Issue 1 https://doi.org/10.1103/PhysRevE.101.010602	journal	January 2020
A collective elastic fluctuation mechanism for decoupling and stretched relaxation in glassy colloidal and molecular liquids Xie, Shi-Jie; Schweizer, Kenneth S. The Journal of Chemical Physics, Vol. 152, Issue 3 https://doi.org/10.1063/1.5129550	journal	January 2020
Linear and nonlinear rheology and structural relaxation in dense glassy and jammed soft repulsive pNIPAM microgel suspensions Ghosh, Ashesh; Chaudhary, Gaurav; Kang, Jin Gu Soft Matter, Vol. 15, Issue 5 https://doi.org/10.1039/C8SM02014K	journal	January 2019
Dynamical Theory of Segmental Relaxation and Emergent Elasticity in Supercooled Polymer Melts Mirigian, Stephen; Schweizer, Kenneth S. Macromolecules, Vol. 48, Issue 6 https://doi.org/10.1021/ma5022083	journal	March 2015
A comparative study of a class of mean field theories of the glass transition Saha, Indranil; Nandi, Manoj Kumar; Dasgupta, Chandan Journal of Statistical Mechanics: Theory and Experiment, Vol. 2019, Issue 8 https://doi.org/10.1088/1742-5468/ab3115	journal	August 2019
Activated hopping and dynamical fluctuation effects in hard sphere suspensions and fluids Saltzman, Erica J.; Schweizer, Kenneth S. The Journal of Chemical Physics, Vol. 125, Issue 4 https://doi.org/10.1063/1.2217739	journal	July 2006
Hopping and the Stokes–Einstein relation breakdown in simple glass formers Charbonneau, Patrick; Jin, Yuliang; Parisi, Giorgio Proceedings of the National Academy of Sciences, Vol. 111, Issue 42 https://doi.org/10.1073/pnas.1417182111	journal	October 2014
Liquid dynamics and inelastic scattering of neutrons De Gennes, P. G. Physica, Vol. 25, Issue 7-12 https://doi.org/10.1016/0031-8914(59)90006-0	journal	January 1959
Connections between some kinetic and equilibrium theories of the glass transition Kirkpatrick, T. R.; Wolynes, P. G. Physical Review A, Vol. 35, Issue 7 https://doi.org/10.1103/PhysRevA.35.3072	journal	April 1987
Microscopic theory of the influence of strong attractive forces on the activated dynamics of dense glass and gel forming fluids Ghosh, Ashesh; Schweizer, Kenneth S. The Journal of Chemical Physics, Vol. 151, Issue 24 https://doi.org/10.1063/1.5129941	journal	December 2019
Perspective: Supercooled liquids and glasses Ediger, M. D.; Harrowell, Peter The Journal of Chemical Physics, Vol. 137, Issue 8 https://doi.org/10.1063/1.4747326	journal	August 2012
Derivation of a microscopic theory of barriers and activated hopping transport in glassy liquids and suspensions Schweizer, Kenneth S. The Journal of Chemical Physics, Vol. 123, Issue 24 https://doi.org/10.1063/1.2137701	journal	December 2005
Testing “microscopic” theories of glass-forming liquids Berthier, L.; Tarjus, G. The European Physical Journal E, Vol. 34, Issue 9 https://doi.org/10.1140/epje/i2011-11096-5	journal	September 2011
Nonperturbative Effect of Attractive Forces in Viscous Liquids Berthier, Ludovic; Tarjus, Gilles Physical Review Letters, Vol. 103, Issue 17 https://doi.org/10.1103/PhysRevLett.103.170601	journal	October 2009

Similar Records

Theory of Transient Localization, Activated Dynamics, and a Macromolecular Glass Transition in Ring Polymer Liquids

Journal Article · 2021 · ACS Macro Letters · OSTI ID:1978361

Thermodynamics–Structure–Dynamics Correlations and Nonuniversal Effects in the Elastically Collective Activated Hopping Theory of Glass-Forming Liquids

Journal Article · 2020 · Journal of Physical Chemistry. B, Condensed Matter, Materials, Surfaces, Interfaces and Biophysical Chemistry · OSTI ID:1637754

Debye-Waller Factors in a Quasicrystal

Journal Article · 1999 · Phys. Rev. B · OSTI ID:796519

Related Subjects

Chemistry

Importance of Many Particle Correlations to the Collective Debye–Waller Factor in a Single-Particle Activated Dynamic Theory of the Glass Transition

Citation Formats

References (38)

Similar Records

Related Subjects