Elucidating the Size and Shape of Individual Clinker Phases via Raman Imaging: Impact on Cement Hydration

Polavaram, Krishna C.; Garg, Nishant

doi:10.1021/acs.jpcc.3c03453

Elucidating the Size and Shape of Individual Clinker Phases via Raman Imaging: Impact on Cement Hydration

Journal Article · 17 August 2023 · Journal of Physical Chemistry. C

DOI:https://doi.org/10.1021/acs.jpcc.3c03453· OSTI ID:2418344

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Department of Civil and Environmental Engineering, University of Illinois at Urbana-Champaign, Newmark 2129, 205 N. Mathews, Urbana, Illinois 61801, United States; OSTI
Department of Civil and Environmental Engineering, University of Illinois at Urbana-Champaign, Newmark 2129, 205 N. Mathews, Urbana, Illinois 61801, United States

Not provided.

Research Organization:: Univ. of Illinois at Urbana-Champaign, IL (United States)

Sponsoring Organization:: USDOE Office of Nuclear Energy (NE)

DOE Contract Number:: NE0008886

OSTI ID:: 2418344

Journal Information:: Journal of Physical Chemistry. C, Journal Name: Journal of Physical Chemistry. C Journal Issue: 34 Vol. 127; ISSN 1932-7447

Publisher:: American Chemical Society

Country of Publication:: United States

Language:: English

References (70)

3D analytical mathematical models of random star-shape particles via a combination of X-ray computed microtomography and spherical harmonic analysis Garboczi, E. J.; Bullard, J. W. Advanced Powder Technology, Vol. 28, Issue 2 https://doi.org/10.1016/j.apt.2016.10.014	journal	February 2017
A model investigation of the influence of particle shape on portland cement hydration Bullard, Jeffrey W.; Garboczi, Edward J. Cement and Concrete Research, Vol. 36, Issue 6 https://doi.org/10.1016/j.cemconres.2006.01.003	journal	June 2006
Eco-efficient cements: Potential economically viable solutions for a low-CO2 cement-based materials industry Scrivener, Karen L.; John, Vanderley M.; Gartner, Ellis M. Cement and Concrete Research, Vol. 114 https://doi.org/10.1016/j.cemconres.2018.03.015	journal	December 2018
Advances in understanding cement hydration mechanisms Scrivener, Karen; Ouzia, Alexandre; Juilland, Patrick Cement and Concrete Research, Vol. 124 https://doi.org/10.1016/j.cemconres.2019.105823	journal	October 2019
Raman microscopy of alkali-silica reaction (ASR) products formed in concrete Leemann, Andreas Cement and Concrete Research, Vol. 102 https://doi.org/10.1016/j.cemconres.2017.08.014	journal	December 2017
Phase Analysis of Portland Cement by Combined Quantitative X-Ray Powder Diffraction and Scanning Electron Microscopy Stutzman, Paul E.; Feng, Pan; Bullard, Jeffrey W. Journal of Research of the National Institute of Standards and Technology, Vol. 121 https://doi.org/10.6028/jres.121.004	journal	January 2016
Where is the iron? Clinker microanalysis with XRD Rietveld, optical microscopy/point counting, Bogue and SEM-EDS techniques Crumbie, Alison; Walenta, Günther; Füllmann, Thomas Cement and Concrete Research, Vol. 36, Issue 8 https://doi.org/10.1016/j.cemconres.2006.05.031	journal	August 2006
Modeling the linear elastic properties of Portland cement paste Haecker, C. -J.; Garboczi, E. J.; Bullard, J. W. Cement and Concrete Research, Vol. 35, Issue 10 https://doi.org/10.1016/j.cemconres.2005.05.001	journal	October 2005
In situ full view of the Portland cement hydration by confocal Raman microscopy Torres‐Carrasco, Manuel; Campo, Adolfo; Rubia, Miguel A. Journal of Raman Spectroscopy, Vol. 50, Issue 5 https://doi.org/10.1002/jrs.5574	journal	February 2019
Investigation of blended cement hydration by isothermal calorimetry and thermal analysis Pane, Ivindra; Hansen, Will Cement and Concrete Research, Vol. 35, Issue 6 https://doi.org/10.1016/j.cemconres.2004.10.027	journal	June 2005
Direct three-dimensional observation of the microstructure and chemistry of C3S hydration Hu, Qinang; Aboustait, Mohammed; Kim, Taehwan Cement and Concrete Research, Vol. 88 https://doi.org/10.1016/j.cemconres.2016.07.006	journal	October 2016
Shape and size of microfine aggregates: X-ray microcomputed tomography vs. laser diffraction Erdoğan, S. T.; Garboczi, E. J.; Fowler, D. W. Powder Technology, Vol. 177, Issue 2 https://doi.org/10.1016/j.powtec.2007.02.016	journal	August 2007
Particle size distribution analysis of sand‐sized particles by laser diffraction: an experimental investigation of instrument sensitivity and the effects of particle shape Blott, Simon J.; Pye, Kenneth Sedimentology, Vol. 53, Issue 3 https://doi.org/10.1111/j.1365-3091.2006.00786.x	journal	May 2006
Determination of particle size, surface area, and shape of supplementary cementitious materials by different techniques Arvaniti, Eleni C.; Juenger, Maria C. G.; Bernal, Susan A. Materials and Structures, Vol. 48, Issue 11 https://doi.org/10.1617/s11527-014-0431-3	journal	October 2014
Effects of cement particle size distribution on performance properties of Portland cement-based materials Bentz, Dale P.; Garboczi, Edward J.; Haecker, Claus J. Cement and Concrete Research, Vol. 29, Issue 10 https://doi.org/10.1016/s0008-8846(99)00163-5	journal	October 1999
High-Resolution Particle Size Analysis of Naturally Occurring Very Fine-Grained Sediment Through Laser Diffractometry Sperazza, M.; Moore, J. N.; Hendrix, M. S. Journal of Sedimentary Research, Vol. 74, Issue 5 https://doi.org/10.1306/031104740736	journal	September 2004
Estimation of three-dimensional particle size and shape characteristics using a modified 2D–3D conversion method employing spherical harmonic-based principal component analysis Ueda, Takao Powder Technology, Vol. 404 https://doi.org/10.1016/j.powtec.2022.117461	journal	May 2022
3D particle size distributions from 2D observations: stereology for natural applications Sahagian, Dork L.; Proussevitch, Alexander A. Journal of Volcanology and Geothermal Research, Vol. 84, Issue 3-4 https://doi.org/10.1016/s0377-0273(98)00043-2	journal	September 1998
A methodology to extract the component size distributions in interground composite (limestone) cements Arora, Aashay; Vance, Kirk; Sant, Gaurav Construction and Building Materials, Vol. 121 https://doi.org/10.1016/j.conbuildmat.2016.06.006	journal	September 2016
Real‐time monitoring of carbonation of hardened cement pastes using Raman microscopy Zhang, Kai; Yio, Marcus; Wong, Hong Journal of Microscopy, Vol. 286, Issue 2 https://doi.org/10.1111/jmi.13084	journal	February 2022
Environmental impacts and decarbonization strategies in the cement and concrete industries Habert, G.; Miller, S. A.; John, V. M. Nature Reviews Earth & Environment, Vol. 1, Issue 11 https://doi.org/10.1038/s43017-020-0093-3	journal	September 2020
Effects of Sample Preparation on Particle Size Distributions of Different Types of Silica in Suspensions Retamal Marín, Rodrigo; Babick, Frank; Lindner, Gottlieb-Georg Nanomaterials, Vol. 8, Issue 7 https://doi.org/10.3390/nano8070454	journal	June 2018
Three-dimensional characterisation of particle size and shape for ballast Sun, Y.; Indraratna, B.; Nimbalkar, S. Géotechnique Letters, Vol. 4, Issue 3 https://doi.org/10.1680/geolett.14.00036	journal	July 2014
A New Type of Secondary Radiation Raman, C. V.; Krishnan, K. S. Nature, Vol. 121, Issue 3048 https://doi.org/10.1038/121501c0	journal	March 1928
Sustainable cement production—present and future Schneider, M.; Romer, M.; Tschudin, M. Cement and Concrete Research, Vol. 41, Issue 7 https://doi.org/10.1016/j.cemconres.2011.03.019	journal	July 2011
Effects of SCMs particles on the compressive strength of micro-structurally designed cement paste: Inherent characteristic effect, particle size refinement effect, and hydration effect Liu, Shaolong; Zhang, Tongsheng; Guo, Yiqun Powder Technology, Vol. 330 https://doi.org/10.1016/j.powtec.2018.01.087	journal	May 2018
Picture Thresholding Using an Iterative Selection Method Ridler, T. W.; Calvard, S. IEEE Transactions on Systems, Man, and Cybernetics, Vol. 8, Issue 8, p. 630-632 https://doi.org/10.1109/tsmc.1978.4310039	journal	January 1978
Advances in shape measurement in the digital world Jia, Xiaodong; Garboczi, Edward J. Particuology, Vol. 26 https://doi.org/10.1016/j.partic.2015.12.005	journal	June 2016
3D experimental investigation of the microstructure of cement pastes using synchrotron X-ray microtomography (μCT) Gallucci, E.; Scrivener, K.; Groso, A. Cement and Concrete Research, Vol. 37, Issue 3 https://doi.org/10.1016/j.cemconres.2006.10.012	journal	March 2007
Cement chemistry (2nd edition) Taylor, H. F. W. https://doi.org/10.1680/cc.25929	book	January 1997
SEM–SCA: combined SEM – Raman spectrometer for analysis of OPC clinker Black, L.; Brooker, A. Advances in Applied Ceramics, Vol. 106, Issue 6 https://doi.org/10.1179/174367607x228052	journal	December 2007
Deciphering mineralogical changes and carbonation development during hydration and ageing of a consolidated ternary blended cement paste Claret, Francis; Grangeon, Sylvain; Loschetter, Annick IUCrJ, Vol. 5, Issue 2 https://doi.org/10.1107/s205225251701836x	journal	January 2018
Particle Size Analysis in Pharmaceutics: Principles, Methods and Applications Shekunov, Boris Y.; Chattopadhyay, Pratibhash; Tong, Henry H. Y. Pharmaceutical Research, Vol. 24, Issue 2 https://doi.org/10.1007/s11095-006-9146-7	journal	December 2006
Time-Space-Resolved Chemical Deconvolution of Cementitious Colloidal Systems Using Raman Spectroscopy Loh, Hyun-Chae; Kim, Hee-Jeong; Ulm, Franz-Josef Langmuir, Vol. 37, Issue 23 https://doi.org/10.1021/acs.langmuir.1c00609	journal	June 2021
Ferruginous phases in 19th century lime and cement mortars: A Raman microspectroscopic study Dariz, Petra; Schmid, Thomas Materials Characterization, Vol. 129 https://doi.org/10.1016/j.matchar.2017.04.009	journal	July 2017
Characterisation of cement hydrate phases by TEM, NMR and Raman spectroscopy Richardson, I. G.; Skibsted, J.; Black, L. Advances in Cement Research, Vol. 22, Issue 4 https://doi.org/10.1680/adcr.2010.22.4.233	journal	October 2010
Direct imaging of micrometer-thick interfaces in salt–salt aqueous biphasic systems Degoulange, Damien; Pandya, Raj; Deschamps, Michael Proceedings of the National Academy of Sciences, Vol. 120, Issue 17 https://doi.org/10.1073/pnas.2220662120	journal	April 2023
Spatiotemporal dynamic monitoring of fatty acid–receptor interaction on single living cells by multiplexed Raman imaging Zhang, Wei; Lin, Fangjun; Liu, Yan Proceedings of the National Academy of Sciences, Vol. 117, Issue 7 https://doi.org/10.1073/pnas.1916238117	journal	February 2020
Structural Features of C?S?H(I) and Its Carbonation in Air?A Raman Spectroscopic Study. Part I: Fresh Phases Garbev, Krassimir; Stemmermann, Peter; Black, Leon Journal of the American Ceramic Society, Vol. 90, Issue 3 https://doi.org/10.1111/j.1551-2916.2006.01428.x	journal	March 2007
High-fidelity and high-resolution phase mapping of granites via confocal Raman imaging Polavaram, Krishna C.; Garg, Nishant Scientific Reports, Vol. 11, Issue 1 https://doi.org/10.1038/s41598-021-87488-1	journal	April 2021
Three-dimensional mathematical analysis of particle shape using X-ray tomography and spherical harmonics: Application to aggregates used in concrete Garboczi, E. J. Cement and Concrete Research, Vol. 32, Issue 10 https://doi.org/10.1016/s0008-8846(02)00836-0	journal	October 2002
Characterization of alkali silica reaction gels using Raman spectroscopy Balachandran, C.; Muñoz, J. F.; Arnold, T. Cement and Concrete Research, Vol. 92 https://doi.org/10.1016/j.cemconres.2016.11.018	journal	February 2017
Cementing CO2 into C-S-H: A step toward concrete carbon neutrality Stefaniuk, Damian; Hajduczek, Marcin; Weaver, James C. PNAS Nexus, Vol. 2, Issue 3 https://doi.org/10.1093/pnasnexus/pgad052	journal	March 2023
Identifying Improved Standardized Tests for Measuring Cement Particle Size and Surface Area Ferraris, Chiara; Garboczi, Edward Transportation Research Record: Journal of the Transportation Research Board, Vol. 2342, Issue 1 https://doi.org/10.3141/2342-02	journal	January 2013
NIH Image to ImageJ: 25 years of image analysis Schneider, Caroline A.; Rasband, Wayne S.; Eliceiri, Kevin W. Nature Methods, Vol. 9, Issue 7 https://doi.org/10.1038/nmeth.2089	journal	June 2012
A comparison of TEM and DLS methods to characterize size distribution of ceramic nanoparticles Souza, T. G. F.; Ciminelli, V. S. T.; Mohallem, N. D. S. Journal of Physics: Conference Series, Vol. 733 https://doi.org/10.1088/1742-6596/733/1/012039	journal	July 2016
3D chemical segmentation of fly ash particles with X-ray computed tomography and electron probe microanalysis Hu, Qinang; Ley, M. Tyler; Davis, Jeffrey Fuel, Vol. 116 https://doi.org/10.1016/j.fuel.2013.07.037	journal	January 2014
X-ray computed tomography for additive manufacturing: a review Thompson, A.; Maskery, I.; Leach, R. K. Measurement Science and Technology, Vol. 27, Issue 7 https://doi.org/10.1088/0957-0233/27/7/072001	journal	June 2016
Quantitative evaluation of cement paste carbonation using Raman spectroscopy Mi, Tangwei; Li, Yongqiang; Liu, Wei npj Materials Degradation, Vol. 5, Issue 1 https://doi.org/10.1038/s41529-021-00181-6	journal	June 2021
Multiplexed imaging of surface enhanced Raman scattering nanotags in living mice using noninvasive Raman spectroscopy Zavaleta, C. L.; Smith, B. R.; Walton, I. Proceedings of the National Academy of Sciences, Vol. 106, Issue 32 https://doi.org/10.1073/pnas.0813327106	journal	July 2009
Enabling phase quantification of anhydrous cements via Raman imaging Polavaram, Krishna C.; Garg, Nishant Cement and Concrete Research, Vol. 150 https://doi.org/10.1016/j.cemconres.2021.106592	journal	December 2021
Towards sustainable concrete Monteiro, Paulo J. M.; Miller, Sabbie A.; Horvath, Arpad Nature Materials, Vol. 16, Issue 7 https://doi.org/10.1038/nmat4930	journal	June 2017
Micrometer-scale 3-D shape characterization of eight cements: Particle shape and cement chemistry, and the effect of particle shape on laser diffraction particle size measurement Erdoğan, S. T.; Nie, X.; Stutzman, P. E. Cement and Concrete Research, Vol. 40, Issue 5 https://doi.org/10.1016/j.cemconres.2009.12.006	journal	May 2010
Particle size distribution measurement of anisotropic—particles cylinders and platelets—practical examples Bowen, P.; Sheng, J.; Jongen, N. Powder Technology, Vol. 128, Issue 2-3 https://doi.org/10.1016/s0032-5910(02)00182-1	journal	December 2002
Confocal Raman Microscopy Dieing, Thomas; Hollricher, Olaf; Toporski, Jan Springer Series in Optical Sciences https://doi.org/10.1007/978-3-642-12522-5	book	January 2011
Measurement of Particle Size Distribution in Portland Cement Powder: Analysis of ASTM Round Robin Studies Ferraris, Cf; Hackley, Va; Avilés, Ai Cement, Concrete, and Aggregates, Vol. 26, Issue 2 https://doi.org/10.1520/cca11920	journal	December 2004
Why some carbonate fillers cause rapid increases of viscosity in dispersed cement-based materials Nehdi, Moncef Cement and Concrete Research, Vol. 30, Issue 10 https://doi.org/10.1016/s0008-8846(00)00353-7	journal	October 2000
Laser Diffraction Spectrometers/Experience in Particle Size Analysis Bürkholz, Armin; Polke, Reinhard Particle & Particle Systems Characterization, Vol. 1, Issue 1-4 https://doi.org/10.1002/ppsc.19840010126	journal	January 1984
A Raman spectroscopic study of the evolution of sulfates and hydroxides in cement–fly ash pastes Garg, Nishant; Wang, Kejin; Martin, Steve W. Cement and Concrete Research, Vol. 53 https://doi.org/10.1016/j.cemconres.2013.06.009	journal	November 2013
The influence of nano-silica on the hydration of ordinary Portland cement Land, G.; Stephan, D. Journal of Materials Science, Vol. 47, Issue 2 https://doi.org/10.1007/s10853-011-5881-1	journal	September 2011
A comparison study of Portland cement hydration kinetics as measured by chemical shrinkage and isothermal calorimetry Pang, Xueyu; Bentz, Dale P.; Meyer, Christian Cement and Concrete Composites, Vol. 39 https://doi.org/10.1016/j.cemconcomp.2013.03.007	journal	May 2013
Tracking spatiotemporal evolution of cementitious carbonation via Raman imaging Srivastava, Sonali; Garg, Nishant Journal of Raman Spectroscopy, Vol. 54, Issue 4 https://doi.org/10.1002/jrs.6483	journal	December 2022
A comparative study of submicron particle sizing platforms: Accuracy, precision and resolution analysis of polydisperse particle size distributions Anderson, Will; Kozak, Darby; Coleman, Victoria A. Journal of Colloid and Interface Science, Vol. 405 https://doi.org/10.1016/j.jcis.2013.02.030	journal	September 2013
Effect of Particle Optical Properties on Size Distribution of Soils Obtained by Laser Diffraction Ozer, M.; Orhan, M.; Isik, N. S. Environmental and Engineering Geoscience, Vol. 16, Issue 2 https://doi.org/10.2113/gseegeosci.16.2.163	journal	May 2010
Cement substitution with secondary materials can reduce annual global CO2 emissions by up to 1.3 gigatons Shah, Izhar Hussain; Miller, Sabbie A.; Jiang, Daqian Nature Communications, Vol. 13, Issue 1 https://doi.org/10.1038/s41467-022-33289-7	journal	September 2022
Mechanisms of cement hydration Bullard, Jeffrey W.; Jennings, Hamlin M.; Livingston, Richard A. Cement and Concrete Research, Vol. 41, Issue 12 https://doi.org/10.1016/j.cemconres.2010.09.011	journal	December 2011
The method to determine the optimum refractive index parameter in the laser diffraction and scattering method Kinoshita, Takeshi Advanced Powder Technology, Vol. 12, Issue 4 https://doi.org/10.1163/15685520152756697	journal	January 2001
Use of micro‐Raman spectroscopy to study reaction kinetics in blended white cement pastes containing metakaolin Frías, Moisés; Martínez‐Ramírez, Sagrario Journal of Raman Spectroscopy, Vol. 40, Issue 12 https://doi.org/10.1002/jrs.2372	journal	July 2009
Laser Diffraction Spectrometry: Fraunhofer Diffraction Versus Mie Scattering de Boer, Gerben B. J.; de Weerd, Cornelis; Thoenes, Dirk Particle & Particle Systems Characterization, Vol. 4, Issue 1-4 https://doi.org/10.1002/ppsc.19870040104	journal	January 1987
Multidimensional visualization of the dynamic evolution of Li metal via in situ/operando methods Lang, Shuangyan; Colletta, Michael; Krumov, Mihail R. Proceedings of the National Academy of Sciences, Vol. 120, Issue 7 https://doi.org/10.1073/pnas.2220419120	journal	February 2023

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