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Mono-Ether and Alcohol Bioblendstocks to Reduce the Fuel Penalty of Mixing Controlled Compression Ignition (MCCI) Engine Aftertreatment

Technical Report ·
DOI:https://doi.org/10.2172/2376545· OSTI ID:2376545
An integrated approach utilizing catalysis experiments, process systems engineering, fuel property modeling, and engine testing was utilized in this project to optimize the production process and composition of a #2 diesel bioblendstock produced from ethanol consisting primarily of long-chain mono-ethers. The primary objective of the project was to determine the composition and to design the production process for a bioblendstock for #2 diesel fuel with > 50% reduction in greenhouse gas emissions relative to conventional diesel fuel. The desired bioblendstock needed to be blendable with #2 diesel fuel at > 5 vol. % while still meeting ASTM D975 diesel fuel specification properties and achieving improvements in fuel properties: increased cetane number, decreased sooting, and reduced pour point and cloud point temperatures. At the same time, it needed to reduce the fuel energy penalty associated with MCCI engine aftertreatment resulting in improved system efficiency. The findings of the current project demonstrate that primary objective of the work has been met, i.e., to determine the composition and to design the production process for a bioblendstock for #2 diesel fuel with > 50% reduction in greenhouse gas emissions relative to conventional diesel fuel. Additionally, the results indicate that the property objectives (increased cetane number, reduced pour and cloud points, and reduced sooting propensity) for the designed bioblendstock composition have also been met. Engine testing performed has also confirmed that the increased reactivity of the bioblendstock can be used to improve catalyst heating operation and to reduce the fuel penalty associated with this operation mode. The fuel property results demonstrate that >5 vol.% blending is easily achieved while meeting the ASTM D975 #2 diesel fuel property specifications tested in this work, as this was achieved for a blend with 43 vol. % of the bioblendstock. The results provide a foundation for future work to scaleup the catalytic production process designed in this work, with many of the challenges and areas for improvement being identified in this work to enable economic production with low GHG lifecycle emissions.
Research Organization:
Univ. of Wisconsin, Madison, WI (United States)
Sponsoring Organization:
USDOE Office of Energy Efficiency and Renewable Energy (EERE), Office of Sustainable Transportation. Bioenergy Technologies Office (BETO)
DOE Contract Number:
EE0008480
OSTI ID:
2376545
Report Number(s):
DOE-UW-Madison--08480
Country of Publication:
United States
Language:
English

References (13)

Catalytic Upgrading of Ethanol to C8+ Distillate Range Ethers via Guerbet Coupling and Etherification
  • Huber, George; Canales, Emmanuel; Penaloza, Paolo
  • The American Chemical Society fall meeting; USA-Europe Symposium on Energy. Chicago, Illinois. August 21 - 25. https://doi.org/10.2172/2294078
conference August 2022
Exploration of Fuel Property Impacts on the Combustion of Late Post Injections Using Binary Blends and High-Reactivity Ether Bioblendstocks conference April 2023
Production of bio-diesel blend stocks via acid-catalyzed dehydration of ethanol oligomerization products
  • Canales, Emmanuel; Restrepo-Florez, Juan Manuel; Chavarrio-Canas, Javier
  • The 28th North American Catalysis Society Meeting. Providence, Rhode Island. June 18 - 23. https://doi.org/10.2172/2294042
conference June 2023
Impact of Fuel Properties on the Combustion of Late Post Injections used for Aftertreatment Thermal Management
  • Subramanian, Srinath; Rothamer, David
  • 39th International Symposium on Combustion, 07/24-07/29 2022. Vancouver, BC, Canada https://doi.org/10.2172/2248083
conference July 2022
Advanced fuels from ethanol – a superstructure optimization approach journal January 2021
Production of drop-in biodiesel blendstocks via competitive acid-catalyzed dehydration reactions using ethanol oligomerization products journal January 2024
Kinetic model-based group contribution method for derived cetane number prediction of oxygenated fuel components and blends journal September 2023
Reaction chemistry of ethanol oligomerization to distillate-range molecules using low loading Cu/MgxAlOy catalysts journal December 2022
Exploration of Fuel Property Impacts on the Combustion of Late Post Injections Using Binary Blends and High-Reactivity Ether Bioblendstocks conference April 2023
Catalytic upgrading of ethanol to C8+ distillate range ethers via Guerbet coupling and etherification
  • Huber, George; Canales, Emmanuel; Penaloza, Paolo
  • The American Chemical Society fall meeting. San Francisco, California. August 13 - 17. https://doi.org/10.2172/2294079
conference August 2023
Catalytic Upgrading of Ethanol into Diesel-Fuel Range C10+ Ethers conference September 2023
Ethanol to diesel: a sustainable alternative for the heavy-duty transportation sector journal January 2023
A systems level analysis of ethanol upgrading strategies to middle distillates journal January 2022

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