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Title: Collapse and reappearance of magnetic orderings in spin frustrated TbMnO{sub 3} induced by Fe substitution

Abstract

We studied the temperature dependent magnetic phase evolution in spin frustrated TbMnO{sub 3} affected by Fe doping via powder neutron diffraction. With the introduction of Fe (10% and 20%), the long range incommensurate magnetic orderings collapse. When the Fe content is increased to 30%, a long-range antiferromagnetic ordering develops, while a spin reorientation transition is found near 35 K from a canted G-type antiferromagnetic ordering to a collinear G-type antiferromagnetic ordering. This work demonstrates the complex magnetic interactions existing in transition metal oxides, which helps to understand the frustrated spin states in other similar systems and design magnetic materials as well.

Authors:
 [1];  [2];  [3];  [4];  [3];  [1];  [5];  [6]; ; ; ;  [1]
  1. Institute for Superconducting and Electronic Materials, Australian Institute of Innovative Materials, University of Wollongong, Innovation Campus, Squires Way, North Wollongong, New South Wales 2500 (Australia)
  2. (China)
  3. (United States)
  4. Center for High Pressure Science and Technology Advanced Research, 1690 Cailun Rd. Pudong, Shanghai 201203 (China)
  5. (ANSTO), Bragg Institute, Lucas Heights, New South Wales 2234 (Australia)
  6. The Australian Nuclear Science and Technology Organization (ANSTO), Bragg Institute, Lucas Heights, New South Wales 2234 (Australia)
Publication Date:
OSTI Identifier:
22594294
Resource Type:
Journal Article
Resource Relation:
Journal Name: Applied Physics Letters; Journal Volume: 109; Journal Issue: 10; Other Information: (c) 2016 Author(s); Country of input: International Atomic Energy Agency (IAEA)
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; ANTIFERROMAGNETISM; DESIGN; IRON; MAGNETIC MATERIALS; MAGNETIZATION; MANGANATES; NEUTRON DIFFRACTION; OXIDES; POWDERS; SPIN; TEMPERATURE DEPENDENCE; YTTERBIUM COMPOUNDS

Citation Formats

Hong, Fang, Center for High Pressure Science and Technology Advanced Research, 1690 Cailun Rd. Pudong, Shanghai 201203, The Advanced Light Source, Lawrence Berkeley National Laboratory, 1 Cyclotron Rd, MS 80R0114, Berkeley, California 94720, Yue, Binbin, E-mail: yuebb@hpstar.ac.cn, E-mail: cheng@uow.edu.au, The Advanced Light Source, Lawrence Berkeley National Laboratory, 1 Cyclotron Rd, MS 80R0114, Berkeley, California 94720, Wang, Jianli, The Australian Nuclear Science and Technology Organization, Studer, Andrew, Fang, Chunsheng, Wang, Xiaolin, Dou, Shixue, and Cheng, Zhenxiang, E-mail: yuebb@hpstar.ac.cn, E-mail: cheng@uow.edu.au. Collapse and reappearance of magnetic orderings in spin frustrated TbMnO{sub 3} induced by Fe substitution. United States: N. p., 2016. Web. doi:10.1063/1.4962465.
Hong, Fang, Center for High Pressure Science and Technology Advanced Research, 1690 Cailun Rd. Pudong, Shanghai 201203, The Advanced Light Source, Lawrence Berkeley National Laboratory, 1 Cyclotron Rd, MS 80R0114, Berkeley, California 94720, Yue, Binbin, E-mail: yuebb@hpstar.ac.cn, E-mail: cheng@uow.edu.au, The Advanced Light Source, Lawrence Berkeley National Laboratory, 1 Cyclotron Rd, MS 80R0114, Berkeley, California 94720, Wang, Jianli, The Australian Nuclear Science and Technology Organization, Studer, Andrew, Fang, Chunsheng, Wang, Xiaolin, Dou, Shixue, & Cheng, Zhenxiang, E-mail: yuebb@hpstar.ac.cn, E-mail: cheng@uow.edu.au. Collapse and reappearance of magnetic orderings in spin frustrated TbMnO{sub 3} induced by Fe substitution. United States. doi:10.1063/1.4962465.
Hong, Fang, Center for High Pressure Science and Technology Advanced Research, 1690 Cailun Rd. Pudong, Shanghai 201203, The Advanced Light Source, Lawrence Berkeley National Laboratory, 1 Cyclotron Rd, MS 80R0114, Berkeley, California 94720, Yue, Binbin, E-mail: yuebb@hpstar.ac.cn, E-mail: cheng@uow.edu.au, The Advanced Light Source, Lawrence Berkeley National Laboratory, 1 Cyclotron Rd, MS 80R0114, Berkeley, California 94720, Wang, Jianli, The Australian Nuclear Science and Technology Organization, Studer, Andrew, Fang, Chunsheng, Wang, Xiaolin, Dou, Shixue, and Cheng, Zhenxiang, E-mail: yuebb@hpstar.ac.cn, E-mail: cheng@uow.edu.au. Mon . "Collapse and reappearance of magnetic orderings in spin frustrated TbMnO{sub 3} induced by Fe substitution". United States. doi:10.1063/1.4962465.
@article{osti_22594294,
title = {Collapse and reappearance of magnetic orderings in spin frustrated TbMnO{sub 3} induced by Fe substitution},
author = {Hong, Fang and Center for High Pressure Science and Technology Advanced Research, 1690 Cailun Rd. Pudong, Shanghai 201203 and The Advanced Light Source, Lawrence Berkeley National Laboratory, 1 Cyclotron Rd, MS 80R0114, Berkeley, California 94720 and Yue, Binbin, E-mail: yuebb@hpstar.ac.cn, E-mail: cheng@uow.edu.au and The Advanced Light Source, Lawrence Berkeley National Laboratory, 1 Cyclotron Rd, MS 80R0114, Berkeley, California 94720 and Wang, Jianli and The Australian Nuclear Science and Technology Organization and Studer, Andrew and Fang, Chunsheng and Wang, Xiaolin and Dou, Shixue and Cheng, Zhenxiang, E-mail: yuebb@hpstar.ac.cn, E-mail: cheng@uow.edu.au},
abstractNote = {We studied the temperature dependent magnetic phase evolution in spin frustrated TbMnO{sub 3} affected by Fe doping via powder neutron diffraction. With the introduction of Fe (10% and 20%), the long range incommensurate magnetic orderings collapse. When the Fe content is increased to 30%, a long-range antiferromagnetic ordering develops, while a spin reorientation transition is found near 35 K from a canted G-type antiferromagnetic ordering to a collinear G-type antiferromagnetic ordering. This work demonstrates the complex magnetic interactions existing in transition metal oxides, which helps to understand the frustrated spin states in other similar systems and design magnetic materials as well.},
doi = {10.1063/1.4962465},
journal = {Applied Physics Letters},
number = 10,
volume = 109,
place = {United States},
year = {Mon Sep 05 00:00:00 EDT 2016},
month = {Mon Sep 05 00:00:00 EDT 2016}
}