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Title: Generalized spectral method for near-field optical microscopy

Journal Article · · Journal of Applied Physics
DOI:https://doi.org/10.1063/1.4941343· OSTI ID:22494978
; ; ;  [1];  [2]
  1. Department of Physics, University of California San Diego, 9500 Gilman Drive, La Jolla, California 92093 (United States)
  2. Department of Physics, Boston University, 590 Commonwealth Avenue, Boston, Massachusetts 02215 (United States)

Electromagnetic interaction between a sub-wavelength particle (the “probe”) and a material surface (the “sample”) is studied theoretically. The interaction is shown to be governed by a series of resonances corresponding to surface polariton modes localized near the probe. The resonance parameters depend on the dielectric function and geometry of the probe as well as on the surface reflectivity of the material. Calculation of such resonances is carried out for several types of axisymmetric probes: spherical, spheroidal, and pear-shaped. For spheroids, an efficient numerical method is developed, capable of handling cases of large or strongly momentum-dependent surface reflectivity. Application of the method to highly resonant materials, such as aluminum oxide (by itself or covered with graphene), reveals a rich structure of multi-peak spectra and nonmonotonic approach curves, i.e., the probe-sample distance dependence. These features also strongly depend on the probe shape and optical constants of the model. For less resonant materials such as silicon oxide, the dependence is weak, so that the spheroidal model is reliable. The calculations are done within the quasistatic approximation with radiative damping included perturbatively.

OSTI ID:
22494978
Journal Information:
Journal of Applied Physics, Vol. 119, Issue 5; Other Information: (c) 2016 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA); ISSN 0021-8979
Country of Publication:
United States
Language:
English

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Dipole modelling for a robust description of subdiffractional polariton waves journal January 2019
Polarization-dependent near-field phonon nanoscopy of oxides: SrTiO 3 ,   LiNbO 3 , and PbZr 0.2 Ti 0.8 O 3 journal July 2019
Photonic crystals for nano-light in moiré graphene superlattices journal December 2018
Ultrabroadband infrared near-field spectroscopy and imaging of local resonators in percolative gold films journal January 2019