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Title: The emission wavelength dependent photoluminescence lifetime of the N-doped graphene quantum dots

Abstract

Aromatic nitrogen doped graphene quantum dots were investigated by steady-state and time-resolved photoluminescence (PL) techniques. The PL lifetime was found to be dependent on the emission wavelength and coincident with the PL spectrum, which is different from most semiconductor quantum dots and fluorescent dyes. This result shows the synergy and competition between the quantum confinement effect and edge functional groups, which may have the potential to guide the synthesis and expand the applications of graphene quantum dots.

Authors:
 [1];  [2];  [2]; ; ;  [3]; ; ;  [1];  [1];  [2]
  1. Research Center of Quantum Macro-Phenomenon and Application, Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201210 (China)
  2. (China)
  3. State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai 200050 (China)
Publication Date:
OSTI Identifier:
22486231
Resource Type:
Journal Article
Resource Relation:
Journal Name: Applied Physics Letters; Journal Volume: 107; Journal Issue: 24; Other Information: (c) 2015 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA)
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; CONFINEMENT; DOPED MATERIALS; DYES; FLUORESCENCE; GRAPHENE; LIFETIME; NITROGEN; PHOTOLUMINESCENCE; QUANTUM DOTS; SEMICONDUCTOR MATERIALS; TIME RESOLUTION; WAVELENGTHS

Citation Formats

Deng, Xingxia, School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, University of Chinese Academy of Sciences, Beijing 100049, Sun, Jing, Yang, Siwei, Ding, Guqiao, E-mail: gqding@mail.sim.ac.cn, Shen, Hao, Zhou, Wei, Lu, Jian, Wang, Zhongyang, E-mail: wangzy@sari.ac.cn, and School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210. The emission wavelength dependent photoluminescence lifetime of the N-doped graphene quantum dots. United States: N. p., 2015. Web. doi:10.1063/1.4937923.
Deng, Xingxia, School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, University of Chinese Academy of Sciences, Beijing 100049, Sun, Jing, Yang, Siwei, Ding, Guqiao, E-mail: gqding@mail.sim.ac.cn, Shen, Hao, Zhou, Wei, Lu, Jian, Wang, Zhongyang, E-mail: wangzy@sari.ac.cn, & School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210. The emission wavelength dependent photoluminescence lifetime of the N-doped graphene quantum dots. United States. doi:10.1063/1.4937923.
Deng, Xingxia, School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, University of Chinese Academy of Sciences, Beijing 100049, Sun, Jing, Yang, Siwei, Ding, Guqiao, E-mail: gqding@mail.sim.ac.cn, Shen, Hao, Zhou, Wei, Lu, Jian, Wang, Zhongyang, E-mail: wangzy@sari.ac.cn, and School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210. Mon . "The emission wavelength dependent photoluminescence lifetime of the N-doped graphene quantum dots". United States. doi:10.1063/1.4937923.
@article{osti_22486231,
title = {The emission wavelength dependent photoluminescence lifetime of the N-doped graphene quantum dots},
author = {Deng, Xingxia and School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210 and University of Chinese Academy of Sciences, Beijing 100049 and Sun, Jing and Yang, Siwei and Ding, Guqiao, E-mail: gqding@mail.sim.ac.cn and Shen, Hao and Zhou, Wei and Lu, Jian and Wang, Zhongyang, E-mail: wangzy@sari.ac.cn and School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210},
abstractNote = {Aromatic nitrogen doped graphene quantum dots were investigated by steady-state and time-resolved photoluminescence (PL) techniques. The PL lifetime was found to be dependent on the emission wavelength and coincident with the PL spectrum, which is different from most semiconductor quantum dots and fluorescent dyes. This result shows the synergy and competition between the quantum confinement effect and edge functional groups, which may have the potential to guide the synthesis and expand the applications of graphene quantum dots.},
doi = {10.1063/1.4937923},
journal = {Applied Physics Letters},
number = 24,
volume = 107,
place = {United States},
year = {Mon Dec 14 00:00:00 EST 2015},
month = {Mon Dec 14 00:00:00 EST 2015}
}