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Title: Dynamic microscale temperature gradient in a gold nanorod solution measured by diffraction-limited nanothermometry

Abstract

We quantify the dynamic microscale temperature gradient in a gold nanorod solution using quantum-dot-based microscopic fluorescence nanothermometry. By incorporating CdSe quantum dots into the solution as a nanothermometer, precise temperature mapping with diffraction-limited spatial resolution and sub-degree temperature resolution is achieved. The acquired data on heat generation and dissipation show an excellent agreement with theoretical simulations. This work reveals an effective approach for noninvasive temperature regulation with localized nanoheaters in microfluidic environment.

Authors:
; ; ;  [1]
  1. Centre for Micro-Photonics, Faculty of Science, Engineering and Technology, Swinburne University of Technology, Hawthorn, Victoria 3122 (Australia)
Publication Date:
OSTI Identifier:
22482111
Resource Type:
Journal Article
Resource Relation:
Journal Name: Applied Physics Letters; Journal Volume: 107; Journal Issue: 12; Other Information: (c) 2015 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA)
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; CADMIUM SELENIDES; DIFFRACTION; FLUORESCENCE; GOLD; MAPPING; MATHEMATICAL SOLUTIONS; QUANTUM DOTS; SIMULATION; SPATIAL RESOLUTION; TEMPERATURE GRADIENTS

Citation Formats

Li, Chengmingyue, Gan, Xiaosong, Li, Xiangping, and Gu, Min, E-mail: mgu@swin.edu.au. Dynamic microscale temperature gradient in a gold nanorod solution measured by diffraction-limited nanothermometry. United States: N. p., 2015. Web. doi:10.1063/1.4931724.
Li, Chengmingyue, Gan, Xiaosong, Li, Xiangping, & Gu, Min, E-mail: mgu@swin.edu.au. Dynamic microscale temperature gradient in a gold nanorod solution measured by diffraction-limited nanothermometry. United States. doi:10.1063/1.4931724.
Li, Chengmingyue, Gan, Xiaosong, Li, Xiangping, and Gu, Min, E-mail: mgu@swin.edu.au. Mon . "Dynamic microscale temperature gradient in a gold nanorod solution measured by diffraction-limited nanothermometry". United States. doi:10.1063/1.4931724.
@article{osti_22482111,
title = {Dynamic microscale temperature gradient in a gold nanorod solution measured by diffraction-limited nanothermometry},
author = {Li, Chengmingyue and Gan, Xiaosong and Li, Xiangping and Gu, Min, E-mail: mgu@swin.edu.au},
abstractNote = {We quantify the dynamic microscale temperature gradient in a gold nanorod solution using quantum-dot-based microscopic fluorescence nanothermometry. By incorporating CdSe quantum dots into the solution as a nanothermometer, precise temperature mapping with diffraction-limited spatial resolution and sub-degree temperature resolution is achieved. The acquired data on heat generation and dissipation show an excellent agreement with theoretical simulations. This work reveals an effective approach for noninvasive temperature regulation with localized nanoheaters in microfluidic environment.},
doi = {10.1063/1.4931724},
journal = {Applied Physics Letters},
number = 12,
volume = 107,
place = {United States},
year = {Mon Sep 21 00:00:00 EDT 2015},
month = {Mon Sep 21 00:00:00 EDT 2015}
}