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Title: On the analysis of photo-electron spectra

Abstract

We analyze Photo-Electron Spectra (PES) for a variety of excitation mechanisms from a simple mono-frequency laser pulse to involved combination of pulses as used, e.g., in attosecond experiments. In the case of simple pulses, the peaks in PES reflect the occupied single-particle levels in combination with the given laser frequency. This usual, simple rule may badly fail in the case of excitation pulses with mixed frequencies and if resonant modes of the system are significantly excited. We thus develop an extension of the usual rule to cover all possible excitation scenarios, including mixed frequencies in the attosecond regime. We find that the spectral distributions of dipole, monopole and quadrupole power for the given excitation taken together and properly shifted by the single-particle energies provide a pertinent picture of the PES in all situations. This leads to the derivation of a generalized relation allowing to understand photo-electron yields even in complex experimental setups.

Authors:
 [1];  [2];  [1];  [2];  [3];  [1];  [2]
  1. Université de Toulouse, UPS, Laboratoire de Physique Théorique (IRSAMC), F-31062 Toulouse Cedex (France)
  2. (IRSAMC), Université de Toulouse, F-31062 Toulouse Cedex (France)
  3. Institut für Theoretische Physik, Universität Erlangen, D-91058 Erlangen (Germany)
Publication Date:
OSTI Identifier:
22451210
Resource Type:
Journal Article
Resource Relation:
Journal Name: Annals of Physics; Journal Volume: 360; Other Information: Copyright (c) 2015 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.; Country of input: International Atomic Energy Agency (IAEA)
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; ABSORPTION SPECTRA; ELECTRON SPECTRA; EXCITATION; LASERS; PHOTOELECTRON SPECTROSCOPY

Citation Formats

Gao, C.-Z., E-mail: gao@irsamc.ups-tlse.fr, CNRS, LPT, Dinh, P.M., CNRS, LPT, Reinhard, P.-G., Suraud, E., and CNRS, LPT. On the analysis of photo-electron spectra. United States: N. p., 2015. Web. doi:10.1016/J.AOP.2015.05.007.
Gao, C.-Z., E-mail: gao@irsamc.ups-tlse.fr, CNRS, LPT, Dinh, P.M., CNRS, LPT, Reinhard, P.-G., Suraud, E., & CNRS, LPT. On the analysis of photo-electron spectra. United States. doi:10.1016/J.AOP.2015.05.007.
Gao, C.-Z., E-mail: gao@irsamc.ups-tlse.fr, CNRS, LPT, Dinh, P.M., CNRS, LPT, Reinhard, P.-G., Suraud, E., and CNRS, LPT. 2015. "On the analysis of photo-electron spectra". United States. doi:10.1016/J.AOP.2015.05.007.
@article{osti_22451210,
title = {On the analysis of photo-electron spectra},
author = {Gao, C.-Z., E-mail: gao@irsamc.ups-tlse.fr and CNRS, LPT and Dinh, P.M. and CNRS, LPT and Reinhard, P.-G. and Suraud, E. and CNRS, LPT},
abstractNote = {We analyze Photo-Electron Spectra (PES) for a variety of excitation mechanisms from a simple mono-frequency laser pulse to involved combination of pulses as used, e.g., in attosecond experiments. In the case of simple pulses, the peaks in PES reflect the occupied single-particle levels in combination with the given laser frequency. This usual, simple rule may badly fail in the case of excitation pulses with mixed frequencies and if resonant modes of the system are significantly excited. We thus develop an extension of the usual rule to cover all possible excitation scenarios, including mixed frequencies in the attosecond regime. We find that the spectral distributions of dipole, monopole and quadrupole power for the given excitation taken together and properly shifted by the single-particle energies provide a pertinent picture of the PES in all situations. This leads to the derivation of a generalized relation allowing to understand photo-electron yields even in complex experimental setups.},
doi = {10.1016/J.AOP.2015.05.007},
journal = {Annals of Physics},
number = ,
volume = 360,
place = {United States},
year = 2015,
month = 9
}
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