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Title: Tailoring local density of optical states to control emission intensity and anisotropy of quantum dots in hybrid photonic-plasmonic templates

Abstract

We report results of controlled tuning of the local density of states (LDOS) in versatile, flexible, and hierarchical self assembled plasmonic templates. Using 5 nm diameter gold (Au) spherical nanoantenna within a polymer template randomly dispersed with quantum dots, we show how the photoluminescence intensity and lifetime anisotropy of these dots can be significantly enhanced through LDOS tuning. Finite difference time domain simulations corroborate the experimental observations and extend the regime of enhancement to a wider range of geometric and spectral parameters bringing out the versatility of these functional plasmonic templates. It is also demonstrated how the templates act as plasmonic resonators for effectively engineer giant enhancement of the scattering efficiency of these nano antenna embedded in the templates. Our work provides an alternative method to achieve spontaneous emission intensity and anisotropy enhancement with true nanoscale plasmon resonators.

Authors:
; ;  [1]
  1. Department of Physics, Indian Institute of Science, Bangalore 560012 (India)
Publication Date:
OSTI Identifier:
22398805
Resource Type:
Journal Article
Resource Relation:
Journal Name: Applied Physics Letters; Journal Volume: 106; Journal Issue: 13; Other Information: (c) 2015 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA)
Country of Publication:
United States
Language:
English
Subject:
77 NANOSCIENCE AND NANOTECHNOLOGY; ANISOTROPY; ANTENNAS; COMPUTERIZED SIMULATION; DENSITY OF STATES; EFFICIENCY; GOLD; LIFETIME; PHOTOLUMINESCENCE; PLASMONS; POLYMERS; QUANTUM DOTS; RANDOMNESS; RESONATORS; SCATTERING; SPHERICAL CONFIGURATION; TUNING

Citation Formats

Indukuri, Chaitanya, Mukherjee, Arnab, and Basu, J. K., E-mail: basu@physics.iisc.ernet.in. Tailoring local density of optical states to control emission intensity and anisotropy of quantum dots in hybrid photonic-plasmonic templates. United States: N. p., 2015. Web. doi:10.1063/1.4916548.
Indukuri, Chaitanya, Mukherjee, Arnab, & Basu, J. K., E-mail: basu@physics.iisc.ernet.in. Tailoring local density of optical states to control emission intensity and anisotropy of quantum dots in hybrid photonic-plasmonic templates. United States. doi:10.1063/1.4916548.
Indukuri, Chaitanya, Mukherjee, Arnab, and Basu, J. K., E-mail: basu@physics.iisc.ernet.in. Mon . "Tailoring local density of optical states to control emission intensity and anisotropy of quantum dots in hybrid photonic-plasmonic templates". United States. doi:10.1063/1.4916548.
@article{osti_22398805,
title = {Tailoring local density of optical states to control emission intensity and anisotropy of quantum dots in hybrid photonic-plasmonic templates},
author = {Indukuri, Chaitanya and Mukherjee, Arnab and Basu, J. K., E-mail: basu@physics.iisc.ernet.in},
abstractNote = {We report results of controlled tuning of the local density of states (LDOS) in versatile, flexible, and hierarchical self assembled plasmonic templates. Using 5 nm diameter gold (Au) spherical nanoantenna within a polymer template randomly dispersed with quantum dots, we show how the photoluminescence intensity and lifetime anisotropy of these dots can be significantly enhanced through LDOS tuning. Finite difference time domain simulations corroborate the experimental observations and extend the regime of enhancement to a wider range of geometric and spectral parameters bringing out the versatility of these functional plasmonic templates. It is also demonstrated how the templates act as plasmonic resonators for effectively engineer giant enhancement of the scattering efficiency of these nano antenna embedded in the templates. Our work provides an alternative method to achieve spontaneous emission intensity and anisotropy enhancement with true nanoscale plasmon resonators.},
doi = {10.1063/1.4916548},
journal = {Applied Physics Letters},
number = 13,
volume = 106,
place = {United States},
year = {Mon Mar 30 00:00:00 EDT 2015},
month = {Mon Mar 30 00:00:00 EDT 2015}
}