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Title: Magnetometry of single ferromagnetic nanoparticles using magneto-optical indicator films with spatial amplification

Abstract

We present a magneto-optical technique to spatially amplify and image fringe fields from single ferromagnetic nanorods. The fringe fields nucleate magnetic domains in a low-coercivity, perpendicularly magnetized indicator film, which are expanded by an applied out-of-plane field from the nanoscale to the microscale for measurement with polar Kerr microscopy. The nucleation location and therefore magnetic orientation of the sample nanorod are detected as spatially dependent field biases in locally measured hysteresis loops of the indicator film. We first discuss our method to fabricate the high-sensitivity indicator film with low energy argon ion irradiation. We then present a map of the amplified signal produced from a single nanorod as measured by the indicator film and compare it with a simultaneously obtained, unamplified fringe field map. The comparison demonstrates the advantage of the amplification mechanism and the capability of the technique to be performed with single-spot magneto-optical Kerr effect magnetometers. Our signal-to-noise ratio determines a minimum measureable particle diameter of tens of nanometers for typical transition metals. We finally use our method to obtain hysteresis loops from multiple nanorods in parallel. Our technique is unperturbed by applied in-plane fields for magnetic manipulation of nanoparticles, is robust against many common noise sources, andmore » is applicable in a variety of test environments. We conclude with a discussion of the future optimization and application of our indicator film technique.« less

Authors:
 [1];  [2];  [3]; ;  [1]
  1. Center for Nanoscale Science and Technology, National Institute of Standards and Technology, Gaithersburg, Maryland 20899 (United States)
  2. (United States)
  3. Materials Science and Engineering Division, Material Measurement Laboratory, National Institute of Standards and Technology, Gaithersburg, Maryland 20899 (United States)
Publication Date:
OSTI Identifier:
22395757
Resource Type:
Journal Article
Resource Relation:
Journal Name: Applied Physics Letters; Journal Volume: 106; Journal Issue: 11; Other Information: (c) 2015 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; AMPLIFICATION; ARGON IONS; COERCIVE FORCE; COMPARATIVE EVALUATIONS; FERROMAGNETIC MATERIALS; FERROMAGNETISM; FILMS; HYSTERESIS; IRRADIATION; KERR EFFECT; MAGNETO-OPTICAL EFFECTS; MICROSCOPY; NANOPARTICLES; NANOSTRUCTURES; NUCLEATION; SIGNAL-TO-NOISE RATIO; TRANSITION ELEMENTS

Citation Formats

Balk, Andrew L., E-mail: andrew.balk@nist.gov, Maryland NanoCenter, University of Maryland, College Park, Maryland 20742, Hangarter, Carlos, Stavis, Samuel M., and Unguris, John. Magnetometry of single ferromagnetic nanoparticles using magneto-optical indicator films with spatial amplification. United States: N. p., 2015. Web. doi:10.1063/1.4916205.
Balk, Andrew L., E-mail: andrew.balk@nist.gov, Maryland NanoCenter, University of Maryland, College Park, Maryland 20742, Hangarter, Carlos, Stavis, Samuel M., & Unguris, John. Magnetometry of single ferromagnetic nanoparticles using magneto-optical indicator films with spatial amplification. United States. doi:10.1063/1.4916205.
Balk, Andrew L., E-mail: andrew.balk@nist.gov, Maryland NanoCenter, University of Maryland, College Park, Maryland 20742, Hangarter, Carlos, Stavis, Samuel M., and Unguris, John. Mon . "Magnetometry of single ferromagnetic nanoparticles using magneto-optical indicator films with spatial amplification". United States. doi:10.1063/1.4916205.
@article{osti_22395757,
title = {Magnetometry of single ferromagnetic nanoparticles using magneto-optical indicator films with spatial amplification},
author = {Balk, Andrew L., E-mail: andrew.balk@nist.gov and Maryland NanoCenter, University of Maryland, College Park, Maryland 20742 and Hangarter, Carlos and Stavis, Samuel M. and Unguris, John},
abstractNote = {We present a magneto-optical technique to spatially amplify and image fringe fields from single ferromagnetic nanorods. The fringe fields nucleate magnetic domains in a low-coercivity, perpendicularly magnetized indicator film, which are expanded by an applied out-of-plane field from the nanoscale to the microscale for measurement with polar Kerr microscopy. The nucleation location and therefore magnetic orientation of the sample nanorod are detected as spatially dependent field biases in locally measured hysteresis loops of the indicator film. We first discuss our method to fabricate the high-sensitivity indicator film with low energy argon ion irradiation. We then present a map of the amplified signal produced from a single nanorod as measured by the indicator film and compare it with a simultaneously obtained, unamplified fringe field map. The comparison demonstrates the advantage of the amplification mechanism and the capability of the technique to be performed with single-spot magneto-optical Kerr effect magnetometers. Our signal-to-noise ratio determines a minimum measureable particle diameter of tens of nanometers for typical transition metals. We finally use our method to obtain hysteresis loops from multiple nanorods in parallel. Our technique is unperturbed by applied in-plane fields for magnetic manipulation of nanoparticles, is robust against many common noise sources, and is applicable in a variety of test environments. We conclude with a discussion of the future optimization and application of our indicator film technique.},
doi = {10.1063/1.4916205},
journal = {Applied Physics Letters},
number = 11,
volume = 106,
place = {United States},
year = {Mon Mar 16 00:00:00 EDT 2015},
month = {Mon Mar 16 00:00:00 EDT 2015}
}