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Title: Large theoretical thermoelectric power factor of suspended single-layer MoS{sub 2}

Abstract

We have calculated the semi-classical thermoelectric power factor of suspended single-layer (SL)- MoS{sub 2} utilizing electron relaxation times derived from ab initio calculations. Measurements of the thermoelectric power factor of SL-MoS{sub 2} on substrates reveal poor power factors. In contrast, we find the thermoelectric power factor of suspended SL-MoS{sub 2} to peak at ∼2.8 × 10{sup 4} μW/m K{sup 2} at 300 K, at an electron concentration of 10{sup 12} cm{sup −2}. This figure is higher than that in bulk Bi{sub 2}Te{sub 3}, for example. Given its relatively high thermal conductivity, suspended SL-MoS{sub 2} may hold promise for in-plane thin-film Peltier coolers, provided reasonable mobilities can be realized.

Authors:
 [1];  [2];  [3];  [1]
  1. Mechanical Science and Engineering Department, University of Illinois at Urbana-Champaign, Urbana, Illinois 61801-2906 (United States)
  2. (United States)
  3. Mechanical Engineering Department, Auburn University, Auburn, Alabama 36849-5341 (United States)
Publication Date:
OSTI Identifier:
22391980
Resource Type:
Journal Article
Resource Relation:
Journal Name: Applied Physics Letters; Journal Volume: 105; Journal Issue: 19; Other Information: (c) 2014 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; BISMUTH TELLURIDES; ELECTRONS; MOLYBDENUM SULFIDES; SUBSTRATES; TEMPERATURE RANGE 0273-0400 K; THERMAL CONDUCTIVITY; THERMOELECTRICITY; THIN FILMS

Citation Formats

Babaei, Hasan, E-mail: babaei@illinois.edu, E-mail: babaei@auburn.edu, Mechanical Engineering Department, Auburn University, Auburn, Alabama 36849-5341, Khodadadi, J. M., and Sinha, Sanjiv. Large theoretical thermoelectric power factor of suspended single-layer MoS{sub 2}. United States: N. p., 2014. Web. doi:10.1063/1.4901342.
Babaei, Hasan, E-mail: babaei@illinois.edu, E-mail: babaei@auburn.edu, Mechanical Engineering Department, Auburn University, Auburn, Alabama 36849-5341, Khodadadi, J. M., & Sinha, Sanjiv. Large theoretical thermoelectric power factor of suspended single-layer MoS{sub 2}. United States. doi:10.1063/1.4901342.
Babaei, Hasan, E-mail: babaei@illinois.edu, E-mail: babaei@auburn.edu, Mechanical Engineering Department, Auburn University, Auburn, Alabama 36849-5341, Khodadadi, J. M., and Sinha, Sanjiv. Mon . "Large theoretical thermoelectric power factor of suspended single-layer MoS{sub 2}". United States. doi:10.1063/1.4901342.
@article{osti_22391980,
title = {Large theoretical thermoelectric power factor of suspended single-layer MoS{sub 2}},
author = {Babaei, Hasan, E-mail: babaei@illinois.edu, E-mail: babaei@auburn.edu and Mechanical Engineering Department, Auburn University, Auburn, Alabama 36849-5341 and Khodadadi, J. M. and Sinha, Sanjiv},
abstractNote = {We have calculated the semi-classical thermoelectric power factor of suspended single-layer (SL)- MoS{sub 2} utilizing electron relaxation times derived from ab initio calculations. Measurements of the thermoelectric power factor of SL-MoS{sub 2} on substrates reveal poor power factors. In contrast, we find the thermoelectric power factor of suspended SL-MoS{sub 2} to peak at ∼2.8 × 10{sup 4} μW/m K{sup 2} at 300 K, at an electron concentration of 10{sup 12} cm{sup −2}. This figure is higher than that in bulk Bi{sub 2}Te{sub 3}, for example. Given its relatively high thermal conductivity, suspended SL-MoS{sub 2} may hold promise for in-plane thin-film Peltier coolers, provided reasonable mobilities can be realized.},
doi = {10.1063/1.4901342},
journal = {Applied Physics Letters},
number = 19,
volume = 105,
place = {United States},
year = {Mon Nov 10 00:00:00 EST 2014},
month = {Mon Nov 10 00:00:00 EST 2014}
}