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Title: Plasmon resonance enhanced large third-order optical nonlinearity and ultrafast optical response in Au nanobipyramids

Abstract

The third-order optical nonlinearity and response time of Au nanobipyramids have been investigated by using optical Kerr effect technique. Large third-order nonlinear optical susceptibility (χ{sup (3)}) and ultrafast optical response time have been obtained at the longitudinal surface plasmon resonance (LSPR) wavelength. As the excitation laser wavelength varies from non-resonance wavelength of 780 nm to the LSPR wavelength of 825 nm, χ{sup (3)} increases from 7.4 × 10{sup −14} to 3.9 × 10{sup −13} esu, the fast component of the response time decreases from 141 ± 23 to 83 ± 8 fs and the ratio of the fast component remains around 48%, while the slow response time decreases from 3200 ± 200 to 2310 ± 158 fs. The large enhancement of χ{sup (3)} is due to the large local field enhancement caused by the surface plasmon resonance, and the shortening of the response times are induced by the increased probability of the electron-electron and electron-phonon scatterings in the nanosystem. This significant ultrafast optical property in Au nanobipyramids has great application in future ultrafast information processors.

Authors:
; ; ; ; ;  [1];  [2]
  1. Wuhan National High Magnetic Field Center and School of Physics, Huazhong University of Science and Technology, Wuhan 430074 (China)
  2. Wenhua College, Wuhan 430074 (China)
Publication Date:
OSTI Identifier:
22317991
Resource Type:
Journal Article
Resource Relation:
Journal Name: Applied Physics Letters; Journal Volume: 105; Journal Issue: 6; Other Information: (c) 2014 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA)
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; ELECTRON-ELECTRON INTERACTIONS; ELECTRON-PHONON COUPLING; GOLD; KERR EFFECT; LASERS; NANOSTRUCTURES; NONLINEAR PROBLEMS; PHONONS; PLASMONS; RESONANCE; SCATTERING

Citation Formats

Yu, Ying, Fan, Shan-Shan, Dai, Hong-Wei, Ma, Zong-Wei, Han, Jun-Bo, E-mail: junbo.han@mail.hust.edu.cn, Li, Liang, and Wang, Xia. Plasmon resonance enhanced large third-order optical nonlinearity and ultrafast optical response in Au nanobipyramids. United States: N. p., 2014. Web. doi:10.1063/1.4892887.
Yu, Ying, Fan, Shan-Shan, Dai, Hong-Wei, Ma, Zong-Wei, Han, Jun-Bo, E-mail: junbo.han@mail.hust.edu.cn, Li, Liang, & Wang, Xia. Plasmon resonance enhanced large third-order optical nonlinearity and ultrafast optical response in Au nanobipyramids. United States. doi:10.1063/1.4892887.
Yu, Ying, Fan, Shan-Shan, Dai, Hong-Wei, Ma, Zong-Wei, Han, Jun-Bo, E-mail: junbo.han@mail.hust.edu.cn, Li, Liang, and Wang, Xia. Mon . "Plasmon resonance enhanced large third-order optical nonlinearity and ultrafast optical response in Au nanobipyramids". United States. doi:10.1063/1.4892887.
@article{osti_22317991,
title = {Plasmon resonance enhanced large third-order optical nonlinearity and ultrafast optical response in Au nanobipyramids},
author = {Yu, Ying and Fan, Shan-Shan and Dai, Hong-Wei and Ma, Zong-Wei and Han, Jun-Bo, E-mail: junbo.han@mail.hust.edu.cn and Li, Liang and Wang, Xia},
abstractNote = {The third-order optical nonlinearity and response time of Au nanobipyramids have been investigated by using optical Kerr effect technique. Large third-order nonlinear optical susceptibility (χ{sup (3)}) and ultrafast optical response time have been obtained at the longitudinal surface plasmon resonance (LSPR) wavelength. As the excitation laser wavelength varies from non-resonance wavelength of 780 nm to the LSPR wavelength of 825 nm, χ{sup (3)} increases from 7.4 × 10{sup −14} to 3.9 × 10{sup −13} esu, the fast component of the response time decreases from 141 ± 23 to 83 ± 8 fs and the ratio of the fast component remains around 48%, while the slow response time decreases from 3200 ± 200 to 2310 ± 158 fs. The large enhancement of χ{sup (3)} is due to the large local field enhancement caused by the surface plasmon resonance, and the shortening of the response times are induced by the increased probability of the electron-electron and electron-phonon scatterings in the nanosystem. This significant ultrafast optical property in Au nanobipyramids has great application in future ultrafast information processors.},
doi = {10.1063/1.4892887},
journal = {Applied Physics Letters},
number = 6,
volume = 105,
place = {United States},
year = {Mon Aug 11 00:00:00 EDT 2014},
month = {Mon Aug 11 00:00:00 EDT 2014}
}