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Title: A dominant role of oxygen additive on cold atmospheric-pressure He + O{sub 2} plasmas

Abstract

We present in this paper how oxygen additive impacts on the cold atmospheric-pressure helium plasmas by means of a one-dimensional fluid model. For the oxygen concentration [O{sub 2}] > ∼0.1%, the influence of oxygen on the electron characteristics and the power dissipation becomes important, e.g., the electron density, the electron temperature in sheath, the electron-coupling power, and the sheath width decreasing by 1.6 to 16 folds with a two-log increase in [O{sub 2}] from 0.1% to 10%. Also the discharge mode evolves from the γ mode to the α mode. The reactive oxygen species are found to peak in the narrow range of [O{sub 2}] = 0.4%–0.9% in the plasmas, similar to their power-coupling values. This applies to their wall fluxes except for those of O* and O{sub 2}{sup −}. These two species have very short lifetimes, thus only when generated in boundary layers within several micrometers next to the electrode can contribute to the fluxes. The dominant reactive oxygen species and the corresponding main reactions are schematically presented, and their relations are quantified for selected applications.

Authors:
; ; ;  [1];  [1];  [2];  [2]
  1. Centre for Plasma Biomedicine, State Key Laboratory of Electrical Insulation and Power Equipment, Xi'an Jiaotong University, Xi'an 710049 (China)
  2. (United States)
Publication Date:
OSTI Identifier:
22303801
Resource Type:
Journal Article
Resource Relation:
Journal Name: Physics of Plasmas; Journal Volume: 21; Journal Issue: 8; Other Information: (c) 2014 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA)
Country of Publication:
United States
Language:
English
Subject:
70 PLASMA PHYSICS AND FUSION TECHNOLOGY; ADDITIVES; ATMOSPHERIC PRESSURE; BOUNDARY LAYERS; CONCENTRATION RATIO; ELECTRODES; ELECTRON DENSITY; ELECTRON TEMPERATURE; HELIUM; ONE-DIMENSIONAL CALCULATIONS; OXYGEN; PLASMA

Citation Formats

Yang, Aijun, Liu, Dingxin, E-mail: liudingxin@gmail.com, E-mail: xhw@mail.xjtu.edu.cn, Rong, Mingzhe, Wang, Xiaohua, E-mail: liudingxin@gmail.com, E-mail: xhw@mail.xjtu.edu.cn, Kong, Michael G., Frank Reidy Research Center for Bioelectrics, Old Dominion University, Norfolk, Virginia 23508, and Department of Electrical and Computer Engineering, Old Dominion University, Norfolk, Virginia 23529. A dominant role of oxygen additive on cold atmospheric-pressure He + O{sub 2} plasmas. United States: N. p., 2014. Web. doi:10.1063/1.4884787.
Yang, Aijun, Liu, Dingxin, E-mail: liudingxin@gmail.com, E-mail: xhw@mail.xjtu.edu.cn, Rong, Mingzhe, Wang, Xiaohua, E-mail: liudingxin@gmail.com, E-mail: xhw@mail.xjtu.edu.cn, Kong, Michael G., Frank Reidy Research Center for Bioelectrics, Old Dominion University, Norfolk, Virginia 23508, & Department of Electrical and Computer Engineering, Old Dominion University, Norfolk, Virginia 23529. A dominant role of oxygen additive on cold atmospheric-pressure He + O{sub 2} plasmas. United States. doi:10.1063/1.4884787.
Yang, Aijun, Liu, Dingxin, E-mail: liudingxin@gmail.com, E-mail: xhw@mail.xjtu.edu.cn, Rong, Mingzhe, Wang, Xiaohua, E-mail: liudingxin@gmail.com, E-mail: xhw@mail.xjtu.edu.cn, Kong, Michael G., Frank Reidy Research Center for Bioelectrics, Old Dominion University, Norfolk, Virginia 23508, and Department of Electrical and Computer Engineering, Old Dominion University, Norfolk, Virginia 23529. Fri . "A dominant role of oxygen additive on cold atmospheric-pressure He + O{sub 2} plasmas". United States. doi:10.1063/1.4884787.
@article{osti_22303801,
title = {A dominant role of oxygen additive on cold atmospheric-pressure He + O{sub 2} plasmas},
author = {Yang, Aijun and Liu, Dingxin, E-mail: liudingxin@gmail.com, E-mail: xhw@mail.xjtu.edu.cn and Rong, Mingzhe and Wang, Xiaohua, E-mail: liudingxin@gmail.com, E-mail: xhw@mail.xjtu.edu.cn and Kong, Michael G. and Frank Reidy Research Center for Bioelectrics, Old Dominion University, Norfolk, Virginia 23508 and Department of Electrical and Computer Engineering, Old Dominion University, Norfolk, Virginia 23529},
abstractNote = {We present in this paper how oxygen additive impacts on the cold atmospheric-pressure helium plasmas by means of a one-dimensional fluid model. For the oxygen concentration [O{sub 2}] > ∼0.1%, the influence of oxygen on the electron characteristics and the power dissipation becomes important, e.g., the electron density, the electron temperature in sheath, the electron-coupling power, and the sheath width decreasing by 1.6 to 16 folds with a two-log increase in [O{sub 2}] from 0.1% to 10%. Also the discharge mode evolves from the γ mode to the α mode. The reactive oxygen species are found to peak in the narrow range of [O{sub 2}] = 0.4%–0.9% in the plasmas, similar to their power-coupling values. This applies to their wall fluxes except for those of O* and O{sub 2}{sup −}. These two species have very short lifetimes, thus only when generated in boundary layers within several micrometers next to the electrode can contribute to the fluxes. The dominant reactive oxygen species and the corresponding main reactions are schematically presented, and their relations are quantified for selected applications.},
doi = {10.1063/1.4884787},
journal = {Physics of Plasmas},
number = 8,
volume = 21,
place = {United States},
year = {Fri Aug 15 00:00:00 EDT 2014},
month = {Fri Aug 15 00:00:00 EDT 2014}
}