Hierarchical mesoporous/microporous carbon with graphitized frameworks for high-performance lithium-ion batteries
Abstract
A hierarchical meso-/micro-porous graphitized carbon with uniform mesopores and ordered micropores, graphitized frameworks, and extra-high surface area of ∼2200 m{sup 2}/g, was successfully synthesized through a simple one-step chemical vapor deposition process. The commercial mesoporous zeolite Y was utilized as a meso-/ micro-porous template, and the small-molecule methane was employed as a carbon precursor. The as-prepared hierarchical meso-/micro-porous carbons have homogeneously distributed mesopores as a host for electrolyte, which facilitate Li{sup +} ions transport to the large-area micropores, resulting a high reversible lithium ion storage of 1000 mA h/g and a high columbic efficiency of 65% at the first cycle.
- Authors:
-
- Department of Chemistry, Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials, Fudan University, Shanghai 200433 (China)
- Department of Chemical Engineering, Monash University, Clayton, VIC 3800 (Australia)
- Chemistry Department and The Center of Excellence for Advanced Materials Research, King Abdulaziz University, P.O. Box 80203, Jeddah 21589 (Saudi Arabia)
- Publication Date:
- OSTI Identifier:
- 22303407
- Resource Type:
- Journal Article
- Journal Name:
- APL Materials
- Additional Journal Information:
- Journal Volume: 2; Journal Issue: 11; Other Information: (c) 2014 Author(s); Country of input: International Atomic Energy Agency (IAEA); Journal ID: ISSN 2166-532X
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 77 NANOSCIENCE AND NANOTECHNOLOGY; CARBON; CHEMICAL VAPOR DEPOSITION; EFFICIENCY; ELECTRIC BATTERIES; ELECTROLYTES; LITHIUM IONS; NANOSTRUCTURES; POROUS MATERIALS; ZEOLITES
Citation Formats
Lv, Yingying, Fang, Yin, Qian, Xufang, Tu, Bo, Wu, Zhangxiong, Asiri, Abdullah M., Zhao, Dongyuan, and Department of Chemical Engineering, Monash University, Clayton, VIC 3800. Hierarchical mesoporous/microporous carbon with graphitized frameworks for high-performance lithium-ion batteries. United States: N. p., 2014.
Web. doi:10.1063/1.4897201.
Lv, Yingying, Fang, Yin, Qian, Xufang, Tu, Bo, Wu, Zhangxiong, Asiri, Abdullah M., Zhao, Dongyuan, & Department of Chemical Engineering, Monash University, Clayton, VIC 3800. Hierarchical mesoporous/microporous carbon with graphitized frameworks for high-performance lithium-ion batteries. United States. https://doi.org/10.1063/1.4897201
Lv, Yingying, Fang, Yin, Qian, Xufang, Tu, Bo, Wu, Zhangxiong, Asiri, Abdullah M., Zhao, Dongyuan, and Department of Chemical Engineering, Monash University, Clayton, VIC 3800. 2014.
"Hierarchical mesoporous/microporous carbon with graphitized frameworks for high-performance lithium-ion batteries". United States. https://doi.org/10.1063/1.4897201.
@article{osti_22303407,
title = {Hierarchical mesoporous/microporous carbon with graphitized frameworks for high-performance lithium-ion batteries},
author = {Lv, Yingying and Fang, Yin and Qian, Xufang and Tu, Bo and Wu, Zhangxiong and Asiri, Abdullah M. and Zhao, Dongyuan and Department of Chemical Engineering, Monash University, Clayton, VIC 3800},
abstractNote = {A hierarchical meso-/micro-porous graphitized carbon with uniform mesopores and ordered micropores, graphitized frameworks, and extra-high surface area of ∼2200 m{sup 2}/g, was successfully synthesized through a simple one-step chemical vapor deposition process. The commercial mesoporous zeolite Y was utilized as a meso-/ micro-porous template, and the small-molecule methane was employed as a carbon precursor. The as-prepared hierarchical meso-/micro-porous carbons have homogeneously distributed mesopores as a host for electrolyte, which facilitate Li{sup +} ions transport to the large-area micropores, resulting a high reversible lithium ion storage of 1000 mA h/g and a high columbic efficiency of 65% at the first cycle.},
doi = {10.1063/1.4897201},
url = {https://www.osti.gov/biblio/22303407},
journal = {APL Materials},
issn = {2166-532X},
number = 11,
volume = 2,
place = {United States},
year = {Sat Nov 01 00:00:00 EDT 2014},
month = {Sat Nov 01 00:00:00 EDT 2014}
}
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