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Title: Shortening x-ray pulses for pump-probe experiments at synchrotrons

Journal Article · · Journal of Applied Physics
DOI:https://doi.org/10.1063/1.3601057· OSTI ID:21538469
; ; ;  [1]; ;  [2];  [3]; ;  [4];  [1]
  1. Helmholtz-Zentrum Berlin fuer Materialien und Energie GmbH, Wilhelm-Conrad-Roentgen Campus, BESSY II, Albert-Einstein-Str. 15, 12489 Berlin (Germany)
  2. Institut fuer Physik und Astronomie, Universitaet Potsdam, Karl-Liebknecht-Str. 24-25, 14476 Potsdam (Germany)
  3. Max-Planck-Institut fuer Mikrostrukturphysik, Weinberg 2, 06120 Halle (Germany)
  4. European Synchrotron Radiation Facility (ESRF), 6 rue Jules Horowitz, BP220, 38043 Grenoble (France)

We implemented an experimental scheme for ultrafast x-ray diffraction at storage rings based on a laser-driven Bragg-switch that shortens the x-ray pulses emitted from an undulator. The increased time-resolution is demonstrated by observing changes of intensity, position and width of the diffraction peaks of a La{sub 0.7}Sr{sub 0.3}MnO{sub 3}/SrTiO{sub 3} superlattice sample after optical excitation, i.e., by quantitatively measuring the propagation of an expansion wave through the sample. These experimental transients with timescales of 35 to 60 ps evidence a reduction of the x-ray pulse duration by a factor of two.

OSTI ID:
21538469
Journal Information:
Journal of Applied Physics, Vol. 109, Issue 12; Other Information: DOI: 10.1063/1.3601057; (c) 2011 American Institute of Physics; ISSN 0021-8979
Country of Publication:
United States
Language:
English