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Title: Laser cooling of semiconductor quantum wells: Theoretical framework and strategy for deep optical refrigeration by luminescence upconversion

Abstract

Optical refrigeration has great potential as a viable solution to thermal management for semiconductor devices and microsystems. We have developed a first-principles-based theory that describes the evolution of thermodynamics - i.e., thermokinetics - of a semiconductor quantum well under laser pumping. This thermokinetic theory partitions a well into three subsystems: interacting electron-hole pairs (carriers) within the well, the lattice (thermal phonons), and the ambient (a thermal reservoir). We start from the Boltzmann kinetic equations and derive the equations of motion for carrier density and temperature, and lattice temperature, under the adiabatic approximation. A simplification is possible as a result of ultrafast energy exchange between the carriers and phonons in semiconductors: a single-temperature equation is sufficient for them, whereas the lattice cooling is ultimately driven by the much slower radiative recombination (upconverted luminescence) process. Our theory microscopically incorporates photogeneration and radiative recombination of the interacting electron-hole pairs. We verify that Kubo-Martin-Schwinger relation holds for our treatment, as a necessary condition for consistency in treatment. The current theory supports steady-state solutions and allows studies of cooling strategies and thermodynamics. We show by numerical investigation of an exemplary GaAs quantum well that higher power cools better when the laser is detuned from themore » band edge between a critical negative value and the ambient thermal energy. We argue for the existence of such a counterintuitive lower bound. Most importantly, we show that there exists an actual detuning, 3 meV above the band edge in the simulated free-carrier case and expected to be pinned at the excitonlike absorption peak owing to Coulomb many-body effects, for optimal laser cooling. Significant improvement in cooling efficacy and theoretical possibility of deep refrigeration are verified with such a fixed optimal actual detuning. In essence, this work provides a consistent microscopic framework and an optimization strategy for achieving net deep cooling of semiconductor quantum wells and related microsystems.« less

Authors:
 [1]
  1. NanoScience Solutions, Inc., Cupertino, California 95014 (United States)
Publication Date:
OSTI Identifier:
20957811
Resource Type:
Journal Article
Resource Relation:
Journal Name: Physical Review. B, Condensed Matter and Materials Physics; Journal Volume: 75; Journal Issue: 15; Other Information: DOI: 10.1103/PhysRevB.75.155315; (c) 2007 The American Physical Society; Country of input: International Atomic Energy Agency (IAEA)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; ADIABATIC APPROXIMATION; BOLTZMANN EQUATION; CARRIER DENSITY; ELECTRONS; EQUATIONS OF MOTION; GALLIUM ARSENIDES; HOLES; LASERS; LUMINESCENCE; MANY-BODY PROBLEM; MEV RANGE 01-10; PHONONS; QUANTUM WELLS; REFRIGERATION; SEMICONDUCTOR MATERIALS

Citation Formats

Li Jianzhong. Laser cooling of semiconductor quantum wells: Theoretical framework and strategy for deep optical refrigeration by luminescence upconversion. United States: N. p., 2007. Web. doi:10.1103/PHYSREVB.75.155315.
Li Jianzhong. Laser cooling of semiconductor quantum wells: Theoretical framework and strategy for deep optical refrigeration by luminescence upconversion. United States. doi:10.1103/PHYSREVB.75.155315.
Li Jianzhong. Sun . "Laser cooling of semiconductor quantum wells: Theoretical framework and strategy for deep optical refrigeration by luminescence upconversion". United States. doi:10.1103/PHYSREVB.75.155315.
@article{osti_20957811,
title = {Laser cooling of semiconductor quantum wells: Theoretical framework and strategy for deep optical refrigeration by luminescence upconversion},
author = {Li Jianzhong},
abstractNote = {Optical refrigeration has great potential as a viable solution to thermal management for semiconductor devices and microsystems. We have developed a first-principles-based theory that describes the evolution of thermodynamics - i.e., thermokinetics - of a semiconductor quantum well under laser pumping. This thermokinetic theory partitions a well into three subsystems: interacting electron-hole pairs (carriers) within the well, the lattice (thermal phonons), and the ambient (a thermal reservoir). We start from the Boltzmann kinetic equations and derive the equations of motion for carrier density and temperature, and lattice temperature, under the adiabatic approximation. A simplification is possible as a result of ultrafast energy exchange between the carriers and phonons in semiconductors: a single-temperature equation is sufficient for them, whereas the lattice cooling is ultimately driven by the much slower radiative recombination (upconverted luminescence) process. Our theory microscopically incorporates photogeneration and radiative recombination of the interacting electron-hole pairs. We verify that Kubo-Martin-Schwinger relation holds for our treatment, as a necessary condition for consistency in treatment. The current theory supports steady-state solutions and allows studies of cooling strategies and thermodynamics. We show by numerical investigation of an exemplary GaAs quantum well that higher power cools better when the laser is detuned from the band edge between a critical negative value and the ambient thermal energy. We argue for the existence of such a counterintuitive lower bound. Most importantly, we show that there exists an actual detuning, 3 meV above the band edge in the simulated free-carrier case and expected to be pinned at the excitonlike absorption peak owing to Coulomb many-body effects, for optimal laser cooling. Significant improvement in cooling efficacy and theoretical possibility of deep refrigeration are verified with such a fixed optimal actual detuning. In essence, this work provides a consistent microscopic framework and an optimization strategy for achieving net deep cooling of semiconductor quantum wells and related microsystems.},
doi = {10.1103/PHYSREVB.75.155315},
journal = {Physical Review. B, Condensed Matter and Materials Physics},
number = 15,
volume = 75,
place = {United States},
year = {Sun Apr 15 00:00:00 EDT 2007},
month = {Sun Apr 15 00:00:00 EDT 2007}
}