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Title: Nitrogen-16 Generation and Transport and Associated Shielding Requirements in a Supercritical-Water-Cooled Reactor

Journal Article · · Nuclear Technology
OSTI ID:20837878
 [1];  [1];  [2]
  1. University of Wisconsin at Madison (United States)
  2. Idaho National Engineering and Environmental Laboratory (United States)

As a water-cooled nuclear system with a direct thermal cycle, the supercritical-water-cooled reactor (SCWR) shares with the boiling water reactor (BWR) the issue of coolant activation and transport of the coolant activation products to the turbine and balance of plant (BOP). Consistent with the BWR experience, the dominant nuclide contributing to the SCWR coolant radioactivity at full power is {sup 16}N, which is produced by an (n,p) reaction on {sup 16}O. In this paper the production and decay of {sup 16}N in the SCWR coolant circuit along with the shielding requirements imposed on the BOP are analyzed and compared with those in a BWR with a similar thermal power rating. A simple control-mass approach is adopted in which the {sup 16}N inventory in a unit mass of coolant is tracked as the coolant flows in the SCWR and BWR primary systems, which are divided into several compartments (e.g., core, lower plenum, downcomer, etc.) of known volume, mass flow rate, and neutron flux. The values of the neutron flux and (n,p) cross section in the SCWR and BWR cores are calculated by means of full-length radially reflected Monte Carlo eigenvalue models of the SCWR and BWR fuel assemblies. The results are as follows: The {sup 16}N activities in the steam lines of the BWR with normal water chemistry, in the BWR with hydrogen water chemistry, and in the SCWR are about 40, 180, and 380 {mu}Ci/g, respectively. The calculated BWR values compare well with the trends and ranges found in the literature. The SCWR {sup 16}N concentration is significantly higher than that in the BWR for the following four reasons:1. The coolant transit time in the SCWR core is about twice that in the BWR core.2. The neutron flux is higher in the SCWR because of the higher power density.3. The slow coolant pass in the water rods produces a significant {sup 16}N activity at the SCWR core inlet.4. In the SCWR all the {sup 16}N generated in the core is sent to the steam lines because there is no recirculation within the vessel.A simple gamma attenuation model shows that the higher {sup 16}N activity in the SCWR results in shielding requirements only up to 10% higher than for the BWR with hydrogen water chemistry. However, because of the higher SCWR electric power, the specific shielding costs per unit of electric power associated with {sup 16}N are expected to be similar to or better than that for BWRs.

OSTI ID:
20837878
Journal Information:
Nuclear Technology, Vol. 147, Issue 2; Other Information: Copyright (c) 2006 American Nuclear Society (ANS), United States, All rights reserved. http://epubs.ans.org/; Country of input: International Atomic Energy Agency (IAEA); ISSN 0029-5450
Country of Publication:
United States
Language:
English