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Title: Antimony orthophosphate glasses with large nonlinear refractive indices, low two-photon absorption coefficients, and ultrafast response

Journal Article · · Journal of Applied Physics
DOI:https://doi.org/10.1063/1.1828216· OSTI ID:20664955
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  1. Departamento de Fisica, Universidade Federal de Pernambuco, 50670-901 Recife, PE (Brazil)

Antimony glasses based on the composition Sb{sub 2}O{sub 3}-SbPO{sub 4} were prepared and characterized. The samples present high refractive index, good transmission from 380 to 2000 nm, and high thermal stability. The nonlinear refractive index, n{sub 2}, of the samples was studied using the optical Kerr shutter technique at 800 nm. The third-order correlation signals between pump and probe pulses indicate ultrafast response (<100 fs) for all compositions. Enhancement of n{sub 2} was observed by adding lead oxide to the Sb{sub 2}O{sub 3}-SbPO{sub 4} composition. Large values of n{sub 2}{approx_equal}10{sup -14} cm{sup 2}/W and negligible two-photon absorption coefficients (smaller than 0.01 cm/GW) were determined for all samples. The glass compositions studied present appropriate figure-of-merit for all-optical switching applications.

OSTI ID:
20664955
Journal Information:
Journal of Applied Physics, Vol. 97, Issue 1; Other Information: DOI: 10.1063/1.1828216; (c) 2005 American Institute of Physics; Country of input: International Atomic Energy Agency (IAEA); ISSN 0021-8979
Country of Publication:
United States
Language:
English