Alternate source term models for Yucca Mountain performance assessment based on natural analog data and secondary mineral solubility
Performance assessment calculations for the proposed high level radioactive waste repository at Yucca Mountain, Nevada, were conducted using the Nuclear Regulatory Commission Total-System Performance Assessment (TPA 3.2) code to test conceptual models and parameter values for the source term based on data from the Pena Blanca, Mexico, natural analog site and based on a model for coprecipitation and solubility of secondary schoepite. In previous studies the value for the maximum constant oxidative alteration rate of uraninite at the Nopal I uranium body at Pena Blanca was estimated. Scaling this rate to the mass of uranium for the proposed Yucca Mountain repository yields an oxidative alteration rate of 22 kg/y, which was assumed to be an upper limit on the release rate from the proposed repository. A second model was developed assuming releases of radionuclides are based on the solubility of secondary schoepite as a function of temperature and solution chemistry. Releases of uranium are given by the product of uranium concentrations at equilibrium with schoepite and the flow of water through the waste packages. For both models, radionuclides other than uranium and those in the cladding and gap fraction were modeled to be released at a rate proportional to the uranium release rate, with additional elemental solubility limits applied. Performance assessment results using the Pena Blanca oxidation rate and schoepite solubility models for Yucca Mountain were compared to the TPA 3.2 base case model, in which release was based on laboratory studies of spent fuel dissolution, cladding and gap release, and solubility limits. Doses calculated using the release rate based on natural analog data and the schoepite solubility models were smaller than doses generated using the base case model. These results provide a degree of confidence in safety predictions using the base case model and an indication of how conservatism in the base case model may be reduced in future analyses.
- Research Organization:
- Southwest Research Inst., San Antonio, TX (US)
- Sponsoring Organization:
- USNRC
- OSTI ID:
- 20015802
- Resource Relation:
- Conference: 1998 Materials Research Society Fall Meeting, Boston, MA (US), 11/30/1998--12/04/1998; Other Information: Single article reprints are available from University Microfilms Inc., 300 North Zeeb Road, Ann Arbor, Michigan 48106; PBD: 1999; Related Information: In: Scientific basis for nuclear waste management XXII. Materials Research Society symposium proceedings: Volume 556, by Wronkiewicz, D.J.; Lee, J.H. [eds.], 1355 pages.
- Country of Publication:
- United States
- Language:
- English
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