Defect Engineering of Monoisotopic Hexagonal Boron Nitride Crystals via Neutron Transmutation Doping

Li, Jiahan; Glaser, Evan R.; Elias, Christine; Ye, Gaihua; Evans, Dylan; Xue, Lianjie; Liu, Song; Cassabois, Guillaume; Gil, Bernard; Valvin, Pierre; Pelini, Thomas; Yeats, Andrew L.; He, Rui; Liu, Bin; Edgar, James H.

doi:10.1021/acs.chemmater.1c02849

Defect Engineering of Monoisotopic Hexagonal Boron Nitride Crystals via Neutron Transmutation Doping

Journal Article · 18 November 2021 · Chemistry of Materials

DOI:https://doi.org/10.1021/acs.chemmater.1c02849· OSTI ID:1981823

^[1]; Glaser, Evan R. ^[2]; Elias, Christine ^[3]; Ye, Gaihua ^[4]; Evans, Dylan ^[1]; Xue, Lianjie ^[1]; Liu, Song ^[1]; ^[3]; Gil, Bernard ^[3]; Valvin, Pierre ^[3]; Pelini, Thomas ^[3]; Yeats, Andrew L. ^[2]; ^[4]; ^[1]; Edgar, James H. ^[1]

Tim Taylor Department of Chemical Engineering, Kansas State University, Manhattan, Kansas 66506, United States
Naval Research Laboratory, Washington, District of Columbia 20375-5347, United States
Laboratoire Charles Coulomb (L2C), Université de Montpellier, CNRS, Montpellier 34095, France
Department of Electrical and Computer Engineering, Texas Tech University, Lubbock, Texas 79409, United States

Not provided.

Research Organization:: Idaho National Laboratory (INL), Idaho Falls, ID (United States). Nuclear Science User Facility (NSUF)

Sponsoring Organization:: USDOE

DOE Contract Number:: AC07-05ID14517

OSTI ID:: 1981823

Journal Information:: Chemistry of Materials, Vol. 33, Issue 23; ISSN 0897-4756

Publisher:: American Chemical Society (ACS)

Country of Publication:: United States

Language:: English

References (30)

Magnetic 2D materials and heterostructures Gibertini, M.; Koperski, M.; Morpurgo, A. F. Nature Nanotechnology, Vol. 14, Issue 5 https://doi.org/10.1038/s41565-019-0438-6	journal	May 2019
Photonics with hexagonal boron nitride Caldwell, Joshua D.; Aharonovich, Igor; Cassabois, Guillaume Nature Reviews Materials, Vol. 4, Issue 8 https://doi.org/10.1038/s41578-019-0124-1	journal	July 2019
Excellent electronic transport in heterostructures of graphene and monoisotopic boron-nitride grown at atmospheric pressure Sonntag, J.; Li, J.; Plaud, A. 2D Materials, Vol. 7, Issue 3 https://doi.org/10.1088/2053-1583/ab89e5	journal	June 2020
Modulating the thermal conductivity in hexagonal boron nitride via controlled boron isotope concentration Yuan, Chao; Li, Jiahan; Lindsay, Lucas Communications Physics, Vol. 2, Issue 1 https://doi.org/10.1038/s42005-019-0145-5	journal	May 2019
Ultralow-loss polaritons in isotopically pure boron nitride Giles, Alexander J.; Dai, Siyuan; Vurgaftman, Igor Nature Materials, Vol. 17, Issue 2 https://doi.org/10.1038/nmat5047	journal	December 2017
Initialization and read-out of intrinsic spin defects in a van der Waals crystal at room temperature Gottscholl, Andreas; Kianinia, Mehran; Soltamov, Victor Nature Materials, Vol. 19, Issue 5 https://doi.org/10.1038/s41563-020-0619-6	journal	February 2020
Quantum emitters in two dimensions Aharonovich, Igor; Toth, Milos Science, Vol. 358, Issue 6360 https://doi.org/10.1126/science.aao6951	journal	October 2017
Fabrication and characterization of solid-state thermal neutron detectors based on hexagonal boron nitride epilayers Doan, T. C.; Majety, S.; Grenadier, S. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 748 https://doi.org/10.1016/j.nima.2014.02.031	journal	June 2014
Neutron bombardment of lithium bis(oxalato) borate: LiBOB Cataldo, Franco; Iglesias-Groth, Susana; Prata, Michele Journal of Radioanalytical and Nuclear Chemistry, Vol. 313, Issue 1 https://doi.org/10.1007/s10967-017-5285-z	journal	May 2017
Tunable and high-purity room temperature single-photon emission from atomic defects in hexagonal boron nitride Grosso, Gabriele; Moon, Hyowon; Lienhard, Benjamin Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/s41467-017-00810-2	journal	September 2017
Postradiation Defects in Neutron-Irradiated Pyrolytic Boron Nitride Kabyshev, A. V.; Kezkalo, V. M.; Lopatin, V. V. Physica Status Solidi (a), Vol. 126, Issue 1 https://doi.org/10.1002/pssa.2211260136	journal	July 1991
Paramagnetic defects in boron nitride nanostructures Kolodiazhnyi, T.; Golberg, D. Chemical Physics Letters, Vol. 413, Issue 1-3 https://doi.org/10.1016/j.cplett.2005.07.065	journal	September 2005
Temperature-Dependent Energy-Level Shifts of Spin Defects in Hexagonal Boron Nitride Liu, Wei; Li, Zhi-Peng; Yang, Yuan-Ze ACS Photonics, Vol. 8, Issue 7 https://doi.org/10.1021/acsphotonics.1c00320	journal	July 2021
Color Centers in Hexagonal Boron Nitride Monolayers: A Group Theory and Ab Initio Analysis Abdi, Mehdi; Chou, Jyh-Pin; Gali, Adam ACS Photonics, Vol. 5, Issue 5 https://doi.org/10.1021/acsphotonics.7b01442	journal	April 2018
Edge effects on optically detected magnetic resonance of vacancy defects in hexagonal boron nitride Sajid, A.; Thygesen, Kristian S.; Reimers, Jeffrey R. Communications Physics, Vol. 3, Issue 1 https://doi.org/10.1038/s42005-020-00416-z	journal	August 2020
Ab initio theory of the negatively charged boron vacancy qubit in hexagonal boron nitride Ivády, Viktor; Barcza, Gergely; Thiering, Gergő npj Computational Materials, Vol. 6, Issue 1 https://doi.org/10.1038/s41524-020-0305-x	journal	April 2020
Hexagonal boron nitride neutron detectors with high detection efficiencies Maity, A.; Grenadier, S. J.; Li, J. Journal of Applied Physics, Vol. 123, Issue 4 https://doi.org/10.1063/1.5017979	journal	January 2018
Low frequency Raman spectroscopy of few-atomic-layer thick hBN crystals Stenger, I.; Schué, L.; Boukhicha, M. 2D Materials, Vol. 4, Issue 3 https://doi.org/10.1088/2053-1583/aa77d4	journal	June 2017
Single Crystal Growth of Millimeter-Sized Monoisotopic Hexagonal Boron Nitride Liu, Song; He, Rui; Xue, Lianjie Chemistry of Materials, Vol. 30, Issue 18 https://doi.org/10.1021/acs.chemmater.8b02589	journal	September 2018
Semiconductor Optics Klingshirn, Claus F. Graduate Texts in Physics https://doi.org/10.1007/978-3-642-28362-8	book	January 2012
Hexagonal boron nitride is an indirect bandgap semiconductor Cassabois, G.; Valvin, P.; Gil, B. Nature Photonics, Vol. 10, Issue 4 https://doi.org/10.1038/nphoton.2015.277	journal	January 2016
Deep ultraviolet emission in hexagonal boron nitride grown by high-temperature molecular beam epitaxy Vuong, T. Q. P.; Cassabois, G.; Valvin, P. 2D Materials, Vol. 4, Issue 2 https://doi.org/10.1088/2053-1583/aa604a	journal	March 2017
Hexagonal Boron Nitride Single Crystal Growth from Solution with a Temperature Gradient Li, Jiahan; Yuan, Chao; Elias, Christine Chemistry of Materials, Vol. 32, Issue 12 https://doi.org/10.1021/acs.chemmater.0c00830	journal	May 2020
Hexagonal Boron Nitride Crystal Growth from Iron, a Single Component Flux Li, Jiahan; Wang, Junyong; Zhang, Xiaotian ACS Nano, Vol. 15, Issue 4 https://doi.org/10.1021/acsnano.1c00115	journal	April 2021
Photoluminescence studies of vacancies and vacancy-impurity complexes in annealed GaAs Chiang, S. Y.; Pearson, G. L. Journal of Luminescence, Vol. 10, Issue 5 https://doi.org/10.1016/0022-2313(75)90054-x	journal	June 1975
Magnetic-field-dependent quantum emission in hexagonal boron nitride at room temperature Exarhos, Annemarie L.; Hopper, David A.; Patel, Raj N. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-018-08185-8	journal	January 2019
Single-spin resonance in a van der Waals embedded paramagnetic defect Chejanovsky, Nathan; Mukherjee, Amlan; Geng, Jianpei Nature Materials, Vol. 20, Issue 8 https://doi.org/10.1038/s41563-021-00979-4	journal	May 2021
Identification and thermal stability of point defects in neutron-irradiated hexagonal boron nitride (h-BN) Toledo, J. R.; Krambrock, K. Journal of Physics D: Applied Physics, Vol. 54, Issue 6 https://doi.org/10.1088/1361-6463/abc37c	journal	November 2020
Identifying carbon as the source of visible single-photon emission from hexagonal boron nitride Mendelson, Noah; Chugh, Dipankar; Reimers, Jeffrey R. Nature Materials, Vol. 20, Issue 3 https://doi.org/10.1038/s41563-020-00850-y	journal	November 2020
Creation of Negatively Charged Boron Vacancies in Hexagonal Boron Nitride Crystal by Electron Irradiation and Mechanism of Inhomogeneous Broadening of Boron Vacancy-Related Spin Resonance Lines Murzakhanov, Fadis; Yavkin, Boris; Mamin, Georgiy Nanomaterials, Vol. 11, Issue 6 https://doi.org/10.3390/nano11061373	journal	May 2021

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