Free Trions with Near-Unity Quantum Yield in Monolayer MoSe 2

Kim, Bumho; Luo, Yue; Rhodes, Daniel; Bai, Yusong; Wang, Jue; Liu, Song; Jordan, Abraham; Huang, Baili; Li, Zhaochen; Taniguchi, Takashi; Watanabe, Kenji; Owen, Jonathan; Strauf, Stefan; Barmak, Katayun; Zhu, Xiaoyang; Hone, James

doi:10.1021/acsnano.1c04331

Free Trions with Near-Unity Quantum Yield in Monolayer MoSe ₂

Journal Article · 22 December 2021 · ACS Nano

DOI:https://doi.org/10.1021/acsnano.1c04331· OSTI ID:1978373

^[1]; ^[2]; ^[1]; Bai, Yusong ^[3]; ^[3]; Liu, Song ^[1]; ^[3]; Huang, Baili ^[4]; Li, Zhaochen ^[4]; ^[5]; ^[6]; ^[3]; Strauf, Stefan ^[7]; Barmak, Katayun ^[4]; ^[3]; Hone, James ^[1]

Department of Mechanical Engineering, Columbia University, New York, New York 10027, United States
Department of Physics, Stevens Institute of Technology, Hoboken, New Jersey 07030, United States; Center for Nanoscale Systems, Harvard University, Cambridge, Massachusetts 02138, United States; Department of Physics, Harvard University, Cambridge, Massachusetts 02138, United States
Department of Chemistry, Columbia University, New York, New York 10027, United States
Department of Applied Physics and Applied Mathematics, Columbia University, New York, New York 10027, United States
International Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
Department of Physics, Stevens Institute of Technology, Hoboken, New Jersey 07030, United States

Not provided.

Research Organization:: Cornell Univ., Ithaca, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

DOE Contract Number:: SC0019481

OSTI ID:: 1978373

Journal Information:: ACS Nano, Vol. 16, Issue 1; ISSN 1936-0851

Publisher:: American Chemical Society (ACS)

Country of Publication:: United States

Language:: English

References (50)

Atomically Thin MoS2 A New Direct-Gap Semiconductor Mak, Kin Fai; Lee, Changgu; Hone, James Physical Review Letters, Vol. 105, Issue 13, Article No.136805 https://doi.org/10.1103/PhysRevLett.105.136805	journal	September 2010
Exciton Binding Energy and Nonhydrogenic Rydberg Series in Monolayer WS 2 Chernikov, Alexey; Berkelbach, Timothy C.; Hill, Heather M. Physical Review Letters, Vol. 113, Issue 7 https://doi.org/10.1103/PhysRevLett.113.076802	journal	August 2014
Electrical control of neutral and charged excitons in a monolayer semiconductor Ross, Jason S.; Wu, Sanfeng; Yu, Hongyi Nature Communications, Vol. 4, Issue 1 https://doi.org/10.1038/ncomms2498	journal	February 2013
Tightly bound trions in monolayer MoS2 Mak, Kin Fai; He, Keliang; Lee, Changgu Nature Materials, Vol. 12, Issue 3 https://doi.org/10.1038/nmat3505	journal	December 2012
Efficient generation of neutral and charged biexcitons in encapsulated WSe2 monolayers Ye, Ziliang; Waldecker, Lutz; Ma, Eric Yue Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-05917-8	journal	September 2018
Excited State Biexcitons in Atomically Thin MoSe ₂ Pei, Jiajie; Yang, Jiong; Wang, Xibin ACS Nano, Vol. 11, Issue 7 https://doi.org/10.1021/acsnano.7b03909	journal	July 2017
Neutral and charged inter-valley biexcitons in monolayer MoSe2 Hao, Kai; Specht, Judith F.; Nagler, Philipp Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/ncomms15552	journal	June 2017
Observation of biexcitons in monolayer WSe2 You, Yumeng; Zhang, Xiao-Xiao; Berkelbach, Timothy C. Nature Physics, Vol. 11, Issue 6 https://doi.org/10.1038/nphys3324	journal	May 2015
Revealing the biexciton and trion-exciton complexes in BN encapsulated WSe2 Li, Zhipeng; Wang, Tianmeng; Lu, Zhengguang Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-05863-5	journal	September 2018
Coulomb-bound four- and five-particle intervalley states in an atomically-thin semiconductor Chen, Shao-Yu; Goldstein, Thomas; Taniguchi, Takashi Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-05558-x	journal	September 2018
Charge-tuneable biexciton complexes in monolayer WSe2 Barbone, Matteo; Montblanch, Alejandro R. -P.; Kara, Dhiren M. Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-05632-4	journal	September 2018
Valley excitons in two-dimensional semiconductors Yu, Hongyi; Cui, Xiaodong; Xu, Xiaodong National Science Review, Vol. 2, Issue 1 https://doi.org/10.1093/nsr/nwu078	journal	December 2014
Theory of neutral and charged excitons in monolayer transition metal dichalcogenides Berkelbach, Timothy C.; Hybertsen, Mark S.; Reichman, David R. Physical Review B, Vol. 88, Issue 4 https://doi.org/10.1103/PhysRevB.88.045318	journal	July 2013
Many-body theory of trion absorption features in two-dimensional semiconductors Efimkin, Dmitry K.; MacDonald, Allan H. Physical Review B, Vol. 95, Issue 3 https://doi.org/10.1103/PhysRevB.95.035417	journal	January 2017
Fermi polaron-polaritons in charge-tunable atomically thin semiconductors Sidler, Meinrad; Back, Patrick; Cotlet, Ovidiu Nature Physics, Vol. 13, Issue 3 https://doi.org/10.1038/nphys3949	journal	October 2016
Electron-exciton interactions in the exciton-polaron problem Efimkin, Dmitry K.; Laird, Emma K.; Levinsen, Jesper Physical Review B, Vol. 103, Issue 7 https://doi.org/10.1103/PhysRevB.103.075417	journal	February 2021
Many-body theory of the optical conductivity of excitons and trions in two-dimensional materials Rana, Farhan; Koksal, Okan; Manolatou, Christina Physical Review B, Vol. 102, Issue 8 https://doi.org/10.1103/PhysRevB.102.085304	journal	August 2020
Virtual Trions in the Photoluminescence of Monolayer Transition-Metal Dichalcogenides Van Tuan, Dinh; Jones, Aaron M.; Yang, Min Physical Review Letters, Vol. 122, Issue 21 https://doi.org/10.1103/PhysRevLett.122.217401	journal	May 2019
Electrical suppression of all nonradiative recombination pathways in monolayer semiconductors Lien, Der-Hsien; Uddin, Shiekh Zia; Yeh, Matthew Science, Vol. 364, Issue 6439 https://doi.org/10.1126/science.aaw8053	journal	May 2019
Whisper Gallery Modes in Monolayer Tungsten Disulfide-Hexagonal Boron Nitride Optical Cavity Ren, Tianhua; Song, Peng; Chen, Jianyi ACS Photonics, Vol. 5, Issue 2 https://doi.org/10.1021/acsphotonics.7b01245	journal	November 2017
Exciton dynamics and annihilation in WS ₂ 2D semiconductors Yuan, Long; Huang, Libai Nanoscale, Vol. 7, Issue 16 https://doi.org/10.1039/C5NR00383K	journal	January 2015
Near-unity photoluminescence quantum yield in MoS2 Amani, M.; Lien, D. -H.; Kiriya, D. Science, Vol. 350, Issue 6264 https://doi.org/10.1126/science.aad2114	journal	November 2015
Synthetic WSe ₂ monolayers with high photoluminescence quantum yield Kim, Hyungjin; Ahn, Geun Ho; Cho, Joy Science Advances, Vol. 5, Issue 1 https://doi.org/10.1126/sciadv.aau4728	journal	January 2019
Exciton radiative lifetime in transition metal dichalcogenide monolayers Robert, C.; Lagarde, D.; Cadiz, F. Physical Review B, Vol. 93, Issue 20 https://doi.org/10.1103/PhysRevB.93.205423	journal	May 2016
Valley dynamics probed through charged and neutral exciton emission in monolayer WSe 2 Wang, G.; Bouet, L.; Lagarde, D. Physical Review B, Vol. 90, Issue 7 https://doi.org/10.1103/PhysRevB.90.075413	journal	August 2014
Filtering the photoluminescence spectra of atomically thin semiconductors with graphene Lorchat, Etienne; López, Luis E. Parra; Robert, Cédric Nature Nanotechnology, Vol. 15, Issue 4 https://doi.org/10.1038/s41565-020-0644-2	journal	March 2020
Observation of Charge Transport by Negatively Charged Excitons Sanvitto, D. Science, Vol. 294, Issue 5543 https://doi.org/10.1126/science.1064847	journal	September 2001
Exciton diffusion in WSe ₂ monolayers embedded in a van der Waals heterostructure Cadiz, F.; Robert, C.; Courtade, E. Applied Physics Letters, Vol. 112, Issue 15 https://doi.org/10.1063/1.5026478	journal	April 2018
Transport Dynamics of Neutral Excitons and Trions in Monolayer WS ₂ Kato, Toshiaki; Kaneko, Toshiro ACS Nano, Vol. 10, Issue 10 https://doi.org/10.1021/acsnano.6b05580	journal	September 2016
Approaching the Intrinsic Limit in Transition Metal Diselenides via Point Defect Control Edelberg, Drew; Rhodes, Daniel; Kerelsky, Alexander Nano Letters, Vol. 19, Issue 7 https://doi.org/10.1021/acs.nanolett.9b00985	journal	June 2019
Exploring atomic defects in molybdenum disulphide monolayers Hong, Jinhua; Hu, Zhixin; Probert, Matt Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms7293	journal	February 2015
Post-Synthesis Modifications of Two-Dimensional MoSe ₂ or MoTe ₂ by Incorporation of Excess Metal Atoms into the Crystal Structure Coelho, Paula Mariel; Komsa, Hannu-Pekka; Coy Diaz, Horacio ACS Nano, Vol. 12, Issue 4 https://doi.org/10.1021/acsnano.8b01580	journal	March 2018
Approaching the intrinsic photoluminescence linewidth in transition metal dichalcogenide monolayers Ajayi, Obafunso A.; Ardelean, Jenny V.; Shepard, Gabriella D. 2D Materials, Vol. 4, Issue 3 https://doi.org/10.1088/2053-1583/aa6aa1	journal	July 2017
Boron nitride substrates for high-quality graphene electronics Dean, C. R.; Young, A. F.; Meric, I. Nature Nanotechnology, Vol. 5, Issue 10, p. 722-726 https://doi.org/10.1038/nnano.2010.172	journal	August 2010
Trion-Species-Resolved Quantum Beats in MoSe ₂ Shepard, Gabriella D.; Ardelean, Jenny V.; Ajayi, Obafunso A. ACS Nano, Vol. 11, Issue 11 https://doi.org/10.1021/acsnano.7b06444	journal	September 2017
Probing dark excitons in atomically thin semiconductors via near-field coupling to surface plasmon polaritons Zhou, You; Scuri, Giovanni; Wild, Dominik S. Nature Nanotechnology, Vol. 12, Issue 9 https://doi.org/10.1038/nnano.2017.106	journal	June 2017
Gate control of carrier distribution in k -space in MoS 2 monolayer and bilayer crystals Kümmell, Tilmar; Quitsch, Wolf; Matthis, Sebastian Physical Review B, Vol. 91, Issue 12 https://doi.org/10.1103/PhysRevB.91.125305	journal	March 2015
Many-body theory of radiative lifetimes of exciton-trion superposition states in doped two-dimensional materials Rana, Farhan; Koksal, Okan; Jung, Minwoo Physical Review B, Vol. 103, Issue 3 https://doi.org/10.1103/PhysRevB.103.035424	journal	January 2021
Polarization and time-resolved photoluminescence spectroscopy of excitons in MoSe ₂ monolayers Wang, G.; Palleau, E.; Amand, T. Applied Physics Letters, Vol. 106, Issue 11 https://doi.org/10.1063/1.4916089	journal	March 2015
Coherent and Incoherent Coupling Dynamics between Neutral and Charged Excitons in Monolayer MoSe ₂ Hao, Kai; Xu, Lixiang; Nagler, Philipp Nano Letters, Vol. 16, Issue 8 https://doi.org/10.1021/acs.nanolett.6b02041	journal	July 2016
Intrinsic coherence time of trions in monolayer MoSe 2 measured via two-dimensional coherent spectroscopy Titze, Michael; Li, Bo; Zhang, Xiang Physical Review Materials, Vol. 2, Issue 5 https://doi.org/10.1103/PhysRevMaterials.2.054001	journal	May 2018
Radiative lifetimes of excitons and trions in monolayers of the metal dichalcogenide MoS 2 Wang, Haining; Zhang, Changjian; Chan, Weimin Physical Review B, Vol. 93, Issue 4 https://doi.org/10.1103/PhysRevB.93.045407	journal	January 2016
Control of the Exciton Radiative Lifetime in van der Waals Heterostructures Fang, H. H.; Han, B.; Robert, C. Physical Review Letters, Vol. 123, Issue 6 https://doi.org/10.1103/PhysRevLett.123.067401	journal	August 2019
Exciton Radiative Lifetimes in Two-Dimensional Transition Metal Dichalcogenides Palummo, Maurizia; Bernardi, Marco; Grossman, Jeffrey C. Nano Letters, Vol. 15, Issue 5 https://doi.org/10.1021/nl503799t	journal	March 2015
Exciton trapping is responsible for the long apparent lifetime in acid-treated MoS 2 Goodman, A. J.; Willard, A. P.; Tisdale, W. A. Physical Review B, Vol. 96, Issue 12 https://doi.org/10.1103/PhysRevB.96.121404	journal	September 2017
Electroluminescence from multi-particle exciton complexes in transition metal dichalcogenide semiconductors Paur, Matthias; Molina-Mendoza, Aday J.; Bratschitsch, Rudolf Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-09781-y	journal	April 2019
Light-emitting diodes by band-structure engineering in van der Waals heterostructures Withers, F.; Del Pozo-Zamudio, O.; Mishchenko, A. Nature Materials, Vol. 14, Issue 3 https://doi.org/10.1038/nmat4205	journal	February 2015
Strong Light-Matter Interactions in Heterostructures of Atomically Thin Films Britnell, L.; Ribeiro, R. M.; Eckmann, A. Science, Vol. 340, Issue 6138 https://doi.org/10.1126/science.1235547	journal	May 2013
Strongly adhesive dry transfer technique for van der Waals heterostructure Son, Suhan; Shin, Young Jae; Zhang, Kaixuan 2D Materials, Vol. 7, Issue 4 https://doi.org/10.1088/2053-1583/abad0b	journal	September 2020
One-Dimensional Electrical Contact to a Two-Dimensional Material Wang, L.; Meric, I.; Huang, P. Y. Science, Vol. 342, Issue 6158 https://doi.org/10.1126/science.1244358	journal	October 2013

Similar Records

K₂CuX₃ (X = Cl, Br): All-Inorganic Lead-Free Blue Emitters with Near-Unity Photoluminescence Quantum Yield

Journal Article · 2020 · Chemistry of Materials · OSTI ID:1649144

Creason, Tielyr D.; McWhorter, Timothy M.; Bell, Zane; +2 more

Tunable Exciton-Optomechanical Coupling in Suspended Monolayer MoSe ₂

Journal Article · 2021 · Nano Letters · OSTI ID:1853332

Xie, Hongchao; Jiang, Shengwei; Rhodes, Daniel A.; +3 more

Coherent heteroepitaxial growth of I-III-VI₂ Ag(In,Ga)S₂ colloidal nanocrystals with near-unity quantum yield for use in luminescent solar concentrators

Journal Article · 2023 · Nature Communications · OSTI ID:1998138

Lee, Hak June; Im, Seongbin; Jung, Dongju; +14 more

Related Subjects

Chemistry
Science & Technology - Other Topics
Materials Science

Free Trions with Near-Unity Quantum Yield in Monolayer MoSe 2

Citation Formats

References (50)

Similar Records

Related Subjects

Free Trions with Near-Unity Quantum Yield in Monolayer MoSe ₂