Theory of Transient Localization, Activated Dynamics, and a Macromolecular Glass Transition in Ring Polymer Liquids

Mei, Baicheng; Dell, Zachary E.; Schweizer, Kenneth S.

doi:10.1021/acsmacrolett.1c00530

Theory of Transient Localization, Activated Dynamics, and a Macromolecular Glass Transition in Ring Polymer Liquids

Journal Article · 24 September 2021 · ACS Macro Letters

DOI:https://doi.org/10.1021/acsmacrolett.1c00530· OSTI ID:1978361

; Dell, Zachary E.; Schweizer, Kenneth S.

Not provided.

Research Organization:: Univ. of Illinois at Urbana-Champaign, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

DOE Contract Number:: FG02-07ER46471

OSTI ID:: 1978361

Journal Information:: ACS Macro Letters, Vol. 10, Issue 10; ISSN 2161-1653

Publisher:: American Chemical Society (ACS)

Country of Publication:: United States

Language:: English

References (41)

Unexpected power-law stress relaxation of entangled ring polymers Kapnistos, M.; Lang, M.; Vlassopoulos, D. Nature Materials, Vol. 7, Issue 12 https://doi.org/10.1038/nmat2292	journal	October 2008
Structure and Dynamics of Ring Polymers: Entanglement Effects Because of Solution Density and Ring Topology Rosa, Angelo; Orlandini, Enzo; Tubiana, Luca Macromolecules, Vol. 44, Issue 21 https://doi.org/10.1021/ma201827f	journal	November 2011
Compact structure and non-Gaussian dynamics of ring polymer melts Brás, Ana R.; Gooßen, Sebastian; Krutyeva, Margarita Soft Matter, Vol. 10, Issue 20 https://doi.org/10.1039/C3SM52717D	journal	January 2014
Minimal Surfaces on Unconcatenated Polymer Rings in Melt Smrek, Jan; Grosberg, Alexander Y. ACS Macro Letters, Vol. 5, Issue 6 https://doi.org/10.1021/acsmacrolett.6b00289	journal	May 2016
Intermolecular structural correlations in model globular and unconcatenated ring polymer liquids Dell, Zachary E.; Schweizer, Kenneth S. Soft Matter, Vol. 14, Issue 45 https://doi.org/10.1039/C8SM01722K	journal	January 2018
Molecular dynamics simulation study of nonconcatenated ring polymers in a melt. II. Dynamics Halverson, Jonathan D.; Lee, Won Bo; Grest, Gary S. The Journal of Chemical Physics, Vol. 134, Issue 20 https://doi.org/10.1063/1.3587138	journal	May 2011
Molecular dynamics simulation study of nonconcatenated ring polymers in a melt. I. Statics Halverson, Jonathan D.; Lee, Won Bo; Grest, Gary S. The Journal of Chemical Physics, Vol. 134, Issue 20 https://doi.org/10.1063/1.3587137	journal	May 2011
Annealed lattice animal model and Flory theory for the melt of non-concatenated rings: towards the physics of crumpling Grosberg, Alexander Y. Soft Matter, Vol. 10, Issue 4 https://doi.org/10.1039/C3SM52805G	journal	January 2014
From a melt of rings to chromosome territories: the role of topological constraints in genome folding Halverson, Jonathan D.; Smrek, Jan; Kremer, Kurt Reports on Progress in Physics, Vol. 77, Issue 2 https://doi.org/10.1088/0034-4885/77/2/022601	journal	January 2014
Dynamics of Ring Polymers in the Presence of Fixed Obstacles Rubinstein, Michael Physical Review Letters, Vol. 57, Issue 24 https://doi.org/10.1103/PhysRevLett.57.3023	journal	December 1986
Dynamics of a Ring Polymer in a Gel Obukhov, Sergei P.; Rubinstein, Michael; Duke, Thomas Physical Review Letters, Vol. 73, Issue 9 https://doi.org/10.1103/PhysRevLett.73.1263	journal	August 1994
Self-Similar Conformations and Dynamics in Entangled Melts and Solutions of Nonconcatenated Ring Polymers Ge, Ting; Panyukov, Sergey; Rubinstein, Michael Macromolecules, Vol. 49, Issue 2 https://doi.org/10.1021/acs.macromol.5b02319	journal	January 2016
A topologically driven glass in ring polymers Michieletto, Davide; Turner, Matthew S. Proceedings of the National Academy of Sciences, Vol. 113, Issue 19 https://doi.org/10.1073/pnas.1520665113	journal	April 2016
Glassiness and Heterogeneous Dynamics in Dense Solutions of Ring Polymers Michieletto, Davide; Nahali, Negar; Rosa, Angelo Physical Review Letters, Vol. 119, Issue 19 https://doi.org/10.1103/PhysRevLett.119.197801	journal	November 2017
Structure and dynamics of large ring polymers Kruteva, Margarita; Allgaier, Jürgen; Monkenbusch, Michael Journal of Rheology, Vol. 65, Issue 4 https://doi.org/10.1122/8.0000206	journal	July 2021
The topological glass in ring polymers Lo, Wei-Chang; Turner, Matthew S. EPL (Europhysics Letters), Vol. 102, Issue 5 https://doi.org/10.1209/0295-5075/102/58005	journal	June 2013
Transport coefficients in glassy colloidal fluids Saltzman, Erica J.; Schweizer, Kenneth S. The Journal of Chemical Physics, Vol. 119, Issue 2 https://doi.org/10.1063/1.1578633	journal	July 2003
Thermodynamics–Structure–Dynamics Correlations and Nonuniversal Effects in the Elastically Collective Activated Hopping Theory of Glass-Forming Liquids Mei, Baicheng; Zhou, Yuxing; Schweizer, Kenneth S. The Journal of Physical Chemistry B, Vol. 124, Issue 28 https://doi.org/10.1021/acs.jpcb.0c03613	journal	July 2020
Threading Dynamics of Ring Polymers in a Gel Michieletto, Davide; Marenduzzo, Davide; Orlandini, Enzo ACS Macro Letters, Vol. 3, Issue 3 https://doi.org/10.1021/mz500060c	journal	February 2014
Analysis of Slow Modes in Ring Polymers: Threading of Rings Controls Long-Time Relaxation Tsalikis, Dimitrios G.; Mavrantzas, Vlasis G.; Vlassopoulos, Dimitris ACS Macro Letters, Vol. 5, Issue 6 https://doi.org/10.1021/acsmacrolett.6b00259	journal	May 2016
Active topological glass Smrek, Jan; Chubak, Iurii; Likos, Christos N. Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-019-13696-z	journal	January 2020
Microscopic Theory of Long-Time Center-of-Mass Self-Diffusion and Anomalous Transport in Ring Polymer Liquids Mei, Baicheng; Dell, Zachary E.; Schweizer, Kenneth S. Macromolecules, Vol. 53, Issue 23 https://doi.org/10.1021/acs.macromol.0c01737	journal	November 2020
Understanding the dynamics of rings in the melt in terms of the annealed tree model Smrek, Jan; Grosberg, Alexander Y. Journal of Physics: Condensed Matter, Vol. 27, Issue 6 https://doi.org/10.1088/0953-8984/27/6/064117	journal	January 2015
Topological free volume and quasi-glassy dynamics in the melt of ring polymers Sakaue, Takahiro Soft Matter, Vol. 14, Issue 36 https://doi.org/10.1039/C8SM00968F	journal	January 2018
Cooperative strings and glassy interfaces Salez, Thomas; Salez, Justin; Dalnoki-Veress, Kari Proceedings of the National Academy of Sciences, Vol. 112, Issue 27 https://doi.org/10.1073/pnas.1503133112	journal	June 2015
Progress towards a phenomenological picture and theoretical understanding of glassy dynamics and vitrification near interfaces and under nanoconfinement Schweizer, Kenneth S.; Simmons, David S. The Journal of Chemical Physics, Vol. 151, Issue 24 https://doi.org/10.1063/1.5129405	journal	December 2019
Segment-scale, force-level theory of mesoscopic dynamic localization and entropic elasticity in entangled chain polymer liquids Dell, Zachary E.; Schweizer, Kenneth S. The Journal of Chemical Physics, Vol. 146, Issue 13 https://doi.org/10.1063/1.4978774	journal	April 2017
Integral Equation Theories of the Structure, Thermodynamics, and Phase Transitions of Polymer Fluids Schweizer, Kenneth S.; Curro, John G. Advances in Chemical Physics, Vol. 98 https://doi.org/10.1002/9780470141571.ch1	book	January 2007
Viscosity of colloidal suspensions Verberg, R.; de Schepper, I. M.; Cohen, E. G. D. Physical Review E, Vol. 55, Issue 3 https://doi.org/10.1103/PhysRevE.55.3143	journal	March 1997
Dynamics of polymeric fractals Muthukumar, M. The Journal of Chemical Physics, Vol. 83, Issue 6 https://doi.org/10.1063/1.449222	journal	September 1985
Entropic barriers, activated hopping, and the glass transition in colloidal suspensions Schweizer, Kenneth S.; Saltzman, Erica J. The Journal of Chemical Physics, Vol. 119, Issue 2 https://doi.org/10.1063/1.1578632	journal	July 2003
Derivation of a microscopic theory of barriers and activated hopping transport in glassy liquids and suspensions Schweizer, Kenneth S. The Journal of Chemical Physics, Vol. 123, Issue 24 https://doi.org/10.1063/1.2137701	journal	December 2005
Re-examination of terminal relaxation behavior of high-molecular-weight ring polystyrene melts Doi, Yuya; Matsumoto, Atsushi; Inoue, Tadashi Rheologica Acta, Vol. 56, Issue 6 https://doi.org/10.1007/s00397-017-1014-3	journal	April 2017
Non-Gaussian effects, space-time decoupling, and mobility bifurcation in glassy hard-sphere fluids and suspensions Saltzman, Erica J.; Schweizer, Kenneth S. Physical Review E, Vol. 74, Issue 6 https://doi.org/10.1103/PhysRevE.74.061501	journal	December 2006
Strain softening, yielding, and shear thinning in glassy colloidal suspensions Kobelev, Vladimir; Schweizer, Kenneth S. Physical Review E, Vol. 71, Issue 2 https://doi.org/10.1103/PhysRevE.71.021401	journal	February 2005
The role of collective elasticity on activated structural relaxation, yielding, and steady state flow in hard sphere fluids and colloidal suspensions under strong deformation Ghosh, Ashesh; Schweizer, Kenneth S. The Journal of Chemical Physics, Vol. 153, Issue 19 https://doi.org/10.1063/5.0026258	journal	November 2020
Activated hopping and dynamical fluctuation effects in hard sphere suspensions and fluids Saltzman, Erica J.; Schweizer, Kenneth S. The Journal of Chemical Physics, Vol. 125, Issue 4 https://doi.org/10.1063/1.2217739	journal	July 2006
Large-amplitude jumps and non-Gaussian dynamics in highly concentrated hard sphere fluids Saltzman, Erica J.; Schweizer, Kenneth S. Physical Review E, Vol. 77, Issue 5 https://doi.org/10.1103/PhysRevE.77.051504	journal	May 2008
Concentrated Solutions of Single-Chain Nanoparticles: A Simple Model for Intrinsically Disordered Proteins under Crowding Conditions Moreno, Angel J.; Lo Verso, Federica; Arbe, Arantxa The Journal of Physical Chemistry Letters, Vol. 7, Issue 5 https://doi.org/10.1021/acs.jpclett.6b00144	journal	February 2016
Effect of Molecular Crowding on Conformation and Interactions of Single-Chain Nanoparticles Oberdisse, Julian; González-Burgos, Marina; Mendia, Ander Macromolecules, Vol. 52, Issue 11 https://doi.org/10.1021/acs.macromol.9b00506	journal	May 2019
Anomalous diffusion in polymer monolayers Semenov, A. N.; Meyer, H. Soft Matter, Vol. 9, Issue 16 https://doi.org/10.1039/c3sm27839e	journal	January 2013

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