Evaporation and Molecular Beam Scattering from a Flat Liquid Jet

Lee, Chin; Pohl, Marvin N.; Ramphal, Isaac A.; Yang, Walt; Winter, Bernd; Abel, Bernd; Neumark, Daniel M.

doi:10.1021/acs.jpca.2c01174

Title: Evaporation and Molecular Beam Scattering from a Flat Liquid Jet

Journal Article · Tue May 17 00:00:00 EDT 2022 · Journal of Physical Chemistry. A, Molecules, Spectroscopy, Kinetics, Environment, and General Theory

DOI:https://doi.org/10.1021/acs.jpca.2c01174· OSTI ID:1871192

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Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Fritz-Haber-Inst. der Max-Planck-Gesellschaft, Berlin (Germany)
Leibniz Inst. of Surface Engineering (IOM) (Germany); Univ. of Leipzig (Germany)

An experimental setup for molecular beam scattering from flat liquid sheets has been developed, with the goal of studying reactions at gas–liquid interfaces for volatile liquids. Specifically, a crossed molecular beam instrument that can measure angular and translational energy distributions of scattered products has been adapted for liquid jet scattering. A microfluidic chip is used to create a stable flat liquid sheet inside vacuum from which scattering occurs, and both evaporation and scattering from this sheet are characterized using a rotatable mass spectrometer that can measure product time-of-flight distributions. Furthermore, this article describes the instrument and reports on the first measurements of evaporation of dodecane and Ne from a Ne-doped dodecane flat jet, as well as scattering of Ne from a flat jet of pure dodecane.

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Research Organization:: Univ. of California, Berkeley, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division; Alexander von Humboldt Foundation; German Research Foundation (DFG); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-05CH11231; AC02-76SF00515

OSTI ID:: 1871192

Alternate ID(s):: OSTI ID: 1871033; OSTI ID: 1896694

Journal Information:: Journal of Physical Chemistry. A, Molecules, Spectroscopy, Kinetics, Environment, and General Theory, Vol. 126, Issue 21; ISSN 1089-5639

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Title: Evaporation and Molecular Beam Scattering from a Flat Liquid Jet

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