General Synthetic Strategy to Ordered Mesoporous Carbon Catalysts with Single-Atom Metal Sites for E

Luo, Zhicheng; Yin, Zhouyang; Yu, Jiaqi; Yan, Yu; Hu, Bing; Nie, Renfeng; Kolln, Anna F.; Wu, Xun; Behera, Ranjan K; Chen, Minda; Zhou, Lin; Liu, Fudong; Wang, Bin; Huang, Wenyu; Zhang, Sen; Qi, Long

doi:10.1002/smll.202107799

Title: General Synthetic Strategy to Ordered Mesoporous Carbon Catalysts with Single-Atom Metal Sites for E

Journal Article · 01 April 2022 · Small

DOI:https://doi.org/10.1002/smll.202107799· OSTI ID:1866460

Luo, Zhicheng; Yin, Zhouyang; Yu, Jiaqi; Yan, Yu; Hu, Bing; Nie, Renfeng; Kolln, Anna F.; Wu, Xun; Behera, Ranjan K; Chen, Minda; Zhou, Lin; Liu, Fudong; Wang, Bin; Huang, Wenyu; Zhang, Sen; Qi, Long

Cite

Export

Save

Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source (APS)

Sponsoring Organization:: DOE - Office Of Science; National Science Foundation (NSF)

OSTI ID:: 1866460

Journal Information:: Small, Vol. 18, Issue (16)

Country of Publication:: United States

Language:: ENGLISH

References (47)

Catalysis Research of Relevance to Carbon Management: Progress, Challenges, and Opportunities Arakawa, Hironori; Aresta, Michele; Armor, John N. Chemical Reviews, Vol. 101, Issue 4 https://doi.org/10.1021/cr000018s	journal	April 2001
Transformation of Carbon Dioxide Sakakura, Toshiyasu; Choi, Jun-Chul; Yasuda, Hiroyuki Chemical Reviews, Vol. 107, Issue 6 https://doi.org/10.1021/cr068357u	journal	June 2007
The teraton challenge. A review of fixation and transformation of carbon dioxide Mikkelsen, Mette; Jørgensen, Mikkel; Krebs, Frederik C. Energy Environ. Sci., Vol. 3, Issue 1 https://doi.org/10.1039/B912904A	journal	January 2010
Electrocatalytic Refinery for Sustainable Production of Fuels and Chemicals Tang, Cheng; Zheng, Yao; Jaroniec, Mietek Angewandte Chemie International Edition, Vol. 60, Issue 36 https://doi.org/10.1002/anie.202101522	journal	March 2021
Electrocatalysis for CO ₂ conversion: from fundamentals to value-added products Wang, Genxiang; Chen, Junxiang; Ding, Yichun Chemical Society Reviews, Vol. 50, Issue 8 https://doi.org/10.1039/D0CS00071J	journal	January 2021
Heterogeneous Single‐Atom Catalysts for Electrochemical CO ₂ Reduction Reaction Li, Minhan; Wang, Haifeng; Luo, Wei Advanced Materials, Vol. 32, Issue 34 https://doi.org/10.1002/adma.202001848	journal	July 2020
Advanced Electrocatalysts with Single-Metal-Atom Active Sites Wang, Yuxuan; Su, Hongyang; He, Yanghua Chemical Reviews, Vol. 120, Issue 21 https://doi.org/10.1021/acs.chemrev.0c00594	journal	November 2020
Nickel-Nitrogen-Modified Graphene: An Efficient Electrocatalyst for the Reduction of Carbon Dioxide to Carbon Monoxide Su, Panpan; Iwase, Kazuyuki; Nakanishi, Shuji Small, Vol. 12, Issue 44 https://doi.org/10.1002/smll.201602158	journal	September 2016
Unsaturated edge-anchored Ni single atoms on porous microwave exfoliated graphene oxide for electrochemical CO2 Cheng, Yi; Zhao, Shiyong; Li, Haobo Applied Catalysis B: Environmental, Vol. 243 https://doi.org/10.1016/j.apcatb.2018.10.046	journal	April 2019
Large-Scale and Highly Selective CO2 Electrocatalytic Reduction on Nickel Single-Atom Catalyst Zheng, Tingting; Jiang, Kun; Ta, Na Joule, Vol. 3, Issue 1 https://doi.org/10.1016/j.joule.2018.10.015	journal	January 2019
Carbon dioxide electroreduction on single-atom nickel decorated carbon membranes with industry compatible current densities Yang, Hengpan; Lin, Qing; Zhang, Chao Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-020-14402-0	journal	January 2020
Catalysts for Production of Lower Olefins from Synthesis Gas: A Review Torres Galvis, Hirsa M.; de Jong, Krijn P. ACS Catalysis, Vol. 3, Issue 9 https://doi.org/10.1021/cs4003436	journal	August 2013
Cu nanowire-catalyzed electrochemical reduction of CO or CO ₂ Zhang, Hongyi; Zhang, Yinjia; Li, Yuyang Nanoscale, Vol. 11, Issue 25 https://doi.org/10.1039/C9NR03170G	journal	January 2019
Two Pathways for the Formation of Ethylene in CO Reduction on Single-Crystal Copper Electrodes Schouten, Klaas Jan P.; Qin, Zisheng; Pérez Gallent, Elena Journal of the American Chemical Society, Vol. 134, Issue 24 https://doi.org/10.1021/ja302668n	journal	June 2012
Atomically dispersed Fe ³⁺ sites catalyze efficient CO ₂ electroreduction to CO Gu, Jun; Hsu, Chia-Shuo; Bai, Lichen Science, Vol. 364, Issue 6445 https://doi.org/10.1126/science.aaw7515	journal	June 2019
Constructing FeN4/graphitic nitrogen atomic interface for high-efficiency electrochemical CO2 reduction over a broad potential window Liu, Chuhao; Wu, Yue; Sun, Kaian Chem, Vol. 7, Issue 5 https://doi.org/10.1016/j.chempr.2021.02.001	journal	May 2021
Fe ₁ N ₄ –O ₁ site with axial Fe–O coordination for highly selective CO ₂ reduction over a wide potential range Chen, Zhiqiang; Huang, Aijian; Yu, Ke Energy & Environmental Science, Vol. 14, Issue 6 https://doi.org/10.1039/D1EE00569C	journal	January 2021
Zinc-Coordinated Nitrogen-Codoped Graphene as an Efficient Catalyst for Selective Electrochemical Reduction of CO ₂ to CO Chen, Zhipeng; Mou, Kaiwen; Yao, Shunyu ChemSusChem, Vol. 11, Issue 17 https://doi.org/10.1002/cssc.201800925	journal	July 2018
Design of Single-Atom Co–N ₅ Catalytic Site: A Robust Electrocatalyst for CO ₂ Reduction with Nearly 100% CO Selectivity and Remarkable Stability Pan, Yuan; Lin, Rui; Chen, Yinjuan Journal of the American Chemical Society, Vol. 140, Issue 12 https://doi.org/10.1021/jacs.8b00814	journal	February 2018
Scalable Production of Efficient Single-Atom Copper Decorated Carbon Membranes for CO ₂ Electroreduction to Methanol Yang, Hengpan; Wu, Yu; Li, Guodong Journal of the American Chemical Society, Vol. 141, Issue 32 https://doi.org/10.1021/jacs.9b04907	journal	July 2019
Understanding activity and selectivity of metal-nitrogen-doped carbon catalysts for electrochemical reduction of CO2 Ju, Wen; Bagger, Alexander; Hao, Guang-Ping Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/s41467-017-01035-z	journal	October 2017
Selective CO ₂ Reduction to CO in Water using Earth-Abundant Metal and Nitrogen-Doped Carbon Electrocatalysts Hu, Xin-Ming; Hval, Halvor Høen; Bjerglund, Emil Tveden ACS Catalysis, Vol. 8, Issue 7 https://doi.org/10.1021/acscatal.8b01022	journal	May 2018
Iridium single-atom catalyst on nitrogen-doped carbon for formic acid oxidation synthesized using a general host–guest strategy Li, Zhi; Chen, Yuanjun; Ji, Shufang Nature Chemistry, Vol. 12, Issue 8 https://doi.org/10.1038/s41557-020-0473-9	journal	June 2020
A Universal Principle to Accurately Synthesize Atomically Dispersed Metal–N4 Sites for CO2 Electroreduction Zheng, Wanzhen; Chen, Feng; Zeng, Qi Nano-Micro Letters, Vol. 12, Issue 1 https://doi.org/10.1007/s40820-020-00443-z	journal	May 2020
Identification of champion transition metals centers in metal and nitrogen-codoped carbon catalysts for CO2 reduction Pan, Fuping; Deng, Wei; Justiniano, Carlos Applied Catalysis B: Environmental, Vol. 226 https://doi.org/10.1016/j.apcatb.2018.01.001	journal	June 2018
Surface Immobilization of Transition Metal Ions on Nitrogen-Doped Graphene Realizing High-Efficient and Selective CO ₂ Reduction Bi, Wentuan; Li, Xiaogang; You, Rui Advanced Materials, Vol. 30, Issue 18 https://doi.org/10.1002/adma.201706617	journal	March 2018
Formation of metal complexes with ethylenediamine: a critical survey of equilibrium constants, enthalpy and entropy values Paoletti, P. Pure and Applied Chemistry, Vol. 56, Issue 4 https://doi.org/10.1351/pac198456040491	journal	January 1984
Transition metal-like carbocatalyst Luo, Zhicheng; Nie, Renfeng; Nguyen, Vy T. Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-020-17909-8	journal	August 2020
Recent advances in single atom catalysts for the electrochemical carbon dioxide reduction reaction Zhang, Jincheng; Cai, Weizheng; Hu, Fang Xin Chemical Science, Vol. 12, Issue 20 https://doi.org/10.1039/D1SC01375K	journal	January 2021
Deconvoluting the XPS spectra for nitrogen-doped chars: An analysis from first principles Ayiania, Michael; Smith, Matthew; Hensley, Alyssa J. R. Carbon, Vol. 162 https://doi.org/10.1016/j.carbon.2020.02.065	journal	June 2020
Compromising Science by Ignorant Instrument Calibration—Need to Revisit Half a Century of Published XPS Data Greczynski, Grzegorz; Hultman, Lars Angewandte Chemie International Edition, Vol. 59, Issue 13 https://doi.org/10.1002/anie.201916000	journal	March 2020
Encapsulation of Nonprecious Metal into Ordered Mesoporous N-Doped Carbon for Efficient Quinoline Transfer Hydrogenation with Formic Acid Li, Guoqiang; Yang, Huanhuan; Zhang, Haifu ACS Catalysis, Vol. 8, Issue 9 https://doi.org/10.1021/acscatal.8b01404	journal	July 2018
Crystallographic and EXAFS studies of conformationally designed nonplanar nickel(II) porphyrins Barkigia, Kathleen M.; Renner, Mark W.; Furenlid, Lars R. Journal of the American Chemical Society, Vol. 115, Issue 9 https://doi.org/10.1021/ja00062a029	journal	May 1993
Laboratory EXAFS determined structure of the stable complexes in the ternary Ni( ii )–EDTA–CN ⁻ system Németh, Zoltán; Bajnóczi, Éva G.; Csilla, Bogdán Physical Chemistry Chemical Physics, Vol. 21, Issue 18 https://doi.org/10.1039/C9CP00982E	journal	January 2019
Nickel(II) complexes with dithiadiiminoamine and dithiabis(thiosemicarbazone) ligands † Pavlishchuk, Vitaly V.; Kolotilov, Sergey V.; Addison, Anthony W. Journal of the Chemical Society, Dalton Transactions, Issue 3 https://doi.org/10.1039/a906294g	journal	January 2000
Valence State of Iron in the Sr ₂ Fe(Mo,W,Ta)O _6.0 Double-Perovskite System: an Fe K -edge and L _2,3 -edge XANES Study Karppinen, M.; Yamauchi, H.; Yasukawa, Y. Chemistry of Materials, Vol. 15, Issue 21 https://doi.org/10.1021/cm030397g	journal	September 2003
Polarized Cu K-edge XANES of square planar CuCl42− ion. Experimental and theoretical evidence for shake-down phenomena Kosugi, Nobuhiro; Yokoyama, Toshihiko; Asakura, Kiyotaka Chemical Physics, Vol. 91, Issue 2 https://doi.org/10.1016/0301-0104(84)80058-0	journal	December 1984
Electrochemical Reduction of CO2 Catalyzed by Metal Nanocatalysts Yin, Zhouyang; Palmore, G. Tayhas R.; Sun, Shouheng Trends in Chemistry, Vol. 1, Issue 8 https://doi.org/10.1016/j.trechm.2019.05.004	journal	November 2019
Solid-Diffusion Synthesis of Single-Atom Catalysts Directly from Bulk Metal for Efficient CO2 Reduction Zhao, Changming; Wang, Yu; Li, Zhijun Joule, Vol. 3, Issue 2 https://doi.org/10.1016/j.joule.2018.11.008	journal	February 2019
Electrochemical Conversion of CO ₂ to Syngas with Controllable CO/H ₂ Ratios over Co and Ni Single-Atom Catalysts He, Qun; Liu, Daobin; Lee, Ji Hoon Angewandte Chemie International Edition, Vol. 59, Issue 8 https://doi.org/10.1002/anie.201912719	journal	January 2020
Highly Selective Two‐Electron Electrocatalytic CO ₂ Reduction on Single‐Atom Cu Catalysts Xu, Chaochen; Zhi, Xing; Vasileff, Anthony Small Structures, Vol. 2, Issue 1 https://doi.org/10.1002/sstr.202000058	journal	October 2020
ATHENA , ARTEMIS , HEPHAESTUS : data analysis for X-ray absorption spectroscopy using IFEFFIT Ravel, B.; Newville, M. Journal of Synchrotron Radiation, Vol. 12, Issue 4 https://doi.org/10.1107/S0909049505012719	journal	June 2005
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set Kresse, G.; Furthmüller, J. Physical Review B, Vol. 54, Issue 16, p. 11169-11186 https://doi.org/10.1103/PhysRevB.54.11169	journal	October 1996
Generalized Gradient Approximation Made Simple Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868 https://doi.org/10.1103/PhysRevLett.77.3865	journal	October 1996
Projector augmented-wave method Blöchl, P. E. Physical Review B, Vol. 50, Issue 24, p. 17953-17979 https://doi.org/10.1103/PhysRevB.50.17953	journal	December 1994
A consistent and accurate ab initio parametrization of density functional dispersion correction (DFT-D) for the 94 elements H-Pu Grimme, Stefan; Antony, Jens; Ehrlich, Stephan The Journal of Chemical Physics, Vol. 132, Issue 15 https://doi.org/10.1063/1.3382344	journal	April 2010
The Entropies of Adsorbed Molecules Campbell, Charles T.; Sellers, Jason R. V. Journal of the American Chemical Society, Vol. 134, Issue 43 https://doi.org/10.1021/ja3080117	journal	October 2012

Similar Records

General Synthetic Strategy to Ordered Mesoporous Carbon Catalysts with Single-Atom Metal Sites for Electrochemical CO₂ Reduction

Journal Article · 2022 · Small · OSTI ID:1866460

Luo, Zhicheng; Yin, Zhouyang; Yu, Jiaqi; +13 more

A universal and versatile route for selective covalent tethering of single-site catalyst and functional grops on the surface of ordered mesoporous carbons

Journal Article · 2014 · Chem. Mater. · OSTI ID:1866460

Joglekar, Madhura; Pylypenko, Svitlana; Otting, Megan M.; +2 more

Universal and Versatile Route for Selective Covalent Tethering of Single-Site Catalysts and Functional Groups on the Surface of Ordered Mesoporous Carbons

Journal Article · 2014 · Chemistry of Materials · OSTI ID:1866460

Joglekar, Madhura; Pylypenko, Svitlana; Otting, Megan M.; +2 more

Title: General Synthetic Strategy to Ordered Mesoporous Carbon Catalysts with Single-Atom Metal Sites for E

Citation Formats

References (47)

Similar Records

Related Subjects