In situ imaging of amorphous intermediates during brucite carbonation in supercritical CO[subscript

Zhang, Xin; Lea, Alan S.; Chaka, Anne M.; Loring, John S.; Mergelsberg, Sebastian T.; Nakouzi, Elias; Qafoku, Odeta; De Yoreo, James J.; Schaef, Herbert T.; Rosso, Kevin M.

doi:10.1038/s41563-021-01154-5

Title: In situ imaging of amorphous intermediates during brucite carbonation in supercritical CO[subscript

Journal Article · 01 January 2022 · Nat. Mater.

DOI:https://doi.org/10.1038/s41563-021-01154-5· OSTI ID:1855436

Zhang, Xin; Lea, Alan S.; Chaka, Anne M.; Loring, John S.; Mergelsberg, Sebastian T.; Nakouzi, Elias; Qafoku, Odeta; De Yoreo, James J.; Schaef, Herbert T.; Rosso, Kevin M.

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Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source (APS)

Sponsoring Organization:: DOE - Office Of Science; DOE - BASIC ENERGY SCIENCES

OSTI ID:: 1855436

Journal Information:: Nat. Mater., Vol. 21

Country of Publication:: United States

Language:: ENGLISH

References (51)

Crystallization by particle attachment in synthetic, biogenic, and geologic environments De Yoreo, J. J.; Gilbert, P. U. P. A.; Sommerdijk, N. A. J. M. Science, Vol. 349, Issue 6247 https://doi.org/10.1126/science.aaa6760	journal	July 2015
Studien über die Bildung und Umwandlung fester Körper Ostwald, W. Zeitschrift für Physikalische Chemie, Vol. 22U, Issue 1 https://doi.org/10.1515/zpch-1897-2233	journal	January 1897
Principles of Crystal Nucleation and Growth De Yoreo, J. J. Reviews in Mineralogy and Geochemistry, Vol. 54, Issue 1 https://doi.org/10.2113/0540057	journal	January 2003
The thermodynamics of calcite nucleation at organic interfaces: Classical vs. non-classical pathways Hu, Q.; Nielsen, M. H.; Freeman, C. L. Faraday Discussions, Vol. 159 https://doi.org/10.1039/c2fd20124k	journal	January 2012
In situ TEM imaging of CaCO3 nucleation reveals coexistence of direct and indirect pathways Nielsen, M. H.; Aloni, S.; De Yoreo, J. J. Science, Vol. 345, Issue 6201 https://doi.org/10.1126/science.1254051	journal	September 2014
Solid-State Phase Transformation and Self-Assembly of Amorphous Nanoparticles into Higher-Order Mineral Structures Von Euw, Stanislas; Azaïs, Thierry; Manichev, Viacheslav Journal of the American Chemical Society, Vol. 142, Issue 29 https://doi.org/10.1021/jacs.0c05591	journal	June 2020
Shape-preserving amorphous-to-crystalline transformation of CaCO ₃ revealed by in situ TEM Liu, Zhaoming; Zhang, Zhisen; Wang, Zheming Proceedings of the National Academy of Sciences, Vol. 117, Issue 7 https://doi.org/10.1073/pnas.1914813117	journal	February 2020
A Review of Classical and Nonclassical Nucleation Theories Karthika, S.; Radhakrishnan, T. K.; Kalaichelvi, P. Crystal Growth & Design, Vol. 16, Issue 11 https://doi.org/10.1021/acs.cgd.6b00794	journal	October 2016
Time-Resolved in Situ Raman Spectroscopy of the Nucleation and Growth of Siderite, Magnesite, and Calcite and Their Precursors Montes-Hernandez, German; Renard, François Crystal Growth & Design, Vol. 16, Issue 12 https://doi.org/10.1021/acs.cgd.6b01406	journal	November 2016
Transformation process of amorphous magnesium carbonate in aqueous solution Tanaka, Jun–ya; Kawano, Jun; Nagai, Takaya Journal of Mineralogical and Petrological Sciences, Vol. 114, Issue 2 https://doi.org/10.2465/jmps.181119b	journal	January 2019
Coupled dissolution and precipitation at mineral–fluid interfaces Ruiz-Agudo, E.; Putnis, C. V.; Putnis, A. Chemical Geology, Vol. 383 https://doi.org/10.1016/j.chemgeo.2014.06.007	journal	September 2014
In Situ Infrared Spectroscopic Study of Forsterite Carbonation in Wet Supercritical CO ₂ Loring, John S.; Thompson, Christopher J.; Wang, Zheming Environmental Science & Technology, Vol. 45, Issue 14 https://doi.org/10.1021/es201284e	journal	July 2011
In Situ Infrared Spectroscopic Study of Brucite Carbonation in Dry to Water-Saturated Supercritical Carbon Dioxide Loring, John S.; Thompson, Christopher J.; Zhang, Changyong The Journal of Physical Chemistry A, Vol. 116, Issue 19 https://doi.org/10.1021/jp210020t	journal	May 2012
Brucite [Mg(OH2)] carbonation in wet supercritical CO2: An in situ high pressure X-ray diffraction study Schaef, H. T.; Windisch, C. F.; McGrail, B. P. Geochimica et Cosmochimica Acta, Vol. 75, Issue 23 https://doi.org/10.1016/j.gca.2011.09.029	journal	December 2011
Subarctic physicochemical weathering of serpentinized peridotite Ulven, O. I.; Beinlich, A.; Hövelmann, J. Earth and Planetary Science Letters, Vol. 468 https://doi.org/10.1016/j.epsl.2017.03.030	journal	June 2017
Role of Magnesium-Stabilized Amorphous Calcium Carbonate in Mitigating the Extent of Carbonation in Alkali-Activated Slag Morandeau, Antoine E.; White, Claire E. Chemistry of Materials, Vol. 27, Issue 19 https://doi.org/10.1021/acs.chemmater.5b02382	journal	September 2015
On the pore forming mechanism of Upsalite, a micro- and mesoporous magnesium carbonate Frykstrand, Sara; Forsgren, Johan; Mihranyan, Albert Microporous and Mesoporous Materials, Vol. 190 https://doi.org/10.1016/j.micromeso.2013.12.011	journal	May 2014
A crystal-clear view Cölfen, Helmut Nature Materials, Vol. 9, Issue 12 https://doi.org/10.1038/nmat2911	journal	November 2010
Phase transitions in biogenic amorphous calcium carbonate Gong, Y. U. T.; Killian, C. E.; Olson, I. C. Proceedings of the National Academy of Sciences, Vol. 109, Issue 16 https://doi.org/10.1073/pnas.1118085109	journal	April 2012
Experimental investigations of the reaction path in the MgO–CO2–H2O system in solutions with various ionic strengths, and their applications to nuclear waste isolation Xiong, Yongliang; Lord, Anna Snider Applied Geochemistry, Vol. 23, Issue 6 https://doi.org/10.1016/j.apgeochem.2007.12.035	journal	June 2008
Formation of magnesium silicate hydrate cement in nature de Ruiter, Lisa; Austrheim, Håkon Journal of the Geological Society, Vol. 175, Issue 2 https://doi.org/10.1144/jgs2017-089	journal	November 2017
Direct Nanoscale Observations of CO ₂ Sequestration during Brucite [Mg(OH) ₂ ] Dissolution Hövelmann, J.; Putnis, C. V.; Ruiz-Agudo, E. Environmental Science & Technology, Vol. 46, Issue 9 https://doi.org/10.1021/es300403n	journal	April 2012
A high-pressure atomic force microscope for imaging in supercritical carbon dioxide Lea, A. S.; Higgins, S. R.; Knauss, K. G. Review of Scientific Instruments, Vol. 82, Issue 4 https://doi.org/10.1063/1.3580603	journal	April 2011
CO₂-H₂O mixtures in the geological sequestration of CO₂. I. Assessment and calculation of mutual solubilities from 12 to 100°C and up to 600 bar Spycher, Nicolas; Pruess, Karsten; Ennis-King, Jonathan Geochimica et Cosmochimica Acta, Vol. 67, Issue 16, p. 3015-3031 https://doi.org/10.1016/S0016-7037(03)00273-4	journal	August 2003
Evidence for Carbonate Surface Complexation during Forsterite Carbonation in Wet Supercritical Carbon Dioxide Loring, John S.; Chen, Jeffrey; Bénézeth, Pascale Langmuir, Vol. 31, Issue 27 https://doi.org/10.1021/acs.langmuir.5b01052	journal	July 2015
Synthesis, characterization and optical properties of Mg(OH)2 micro-/nanostructure and its conversion to MgO Kumari, Latha; Li, W. Z.; Vannoy, Charles H. Ceramics International, Vol. 35, Issue 8 https://doi.org/10.1016/j.ceramint.2009.05.035	journal	December 2009
Decoupling Local Disorder and Optical Effects in Infrared Spectra: Differentiating Between Calcites with Different Origins Poduska, Kristin M.; Regev, Lior; Boaretto, Elisabetta Advanced Materials, Vol. 23, Issue 4 https://doi.org/10.1002/adma.201003890	journal	November 2010
Local Atomic Order and Infrared Spectra of Biogenic Calcite Gueta, Rachel; Natan, Amir; Addadi, Lia Angewandte Chemie International Edition, Vol. 46, Issue 1-2 https://doi.org/10.1002/anie.200603327	journal	January 2007
Hydrogen Bonding in Amorphous Alkaline Earth Carbonates Leukel, Sebastian; Mondeshki, Mihail; Tremel, Wolfgang Inorganic Chemistry, Vol. 57, Issue 17 https://doi.org/10.1021/acs.inorgchem.8b02170	journal	August 2018
Adsorption of Pb(II) and Cr(III) from aqueous solution on Celtek clay Sarı, Ahmet; Tuzen, Mustafa; Soylak, Mustafa Journal of Hazardous Materials, Vol. 144, Issue 1-2 https://doi.org/10.1016/j.jhazmat.2006.09.080	journal	June 2007
Multivariate Curve Resolution (MCR) from 2000: Progress in Concepts and Applications de Juan, Anna; Tauler, Romà Critical Reviews in Analytical Chemistry, Vol. 36, Issue 3-4 https://doi.org/10.1080/10408340600970005	journal	December 2006
Calcium Carbonate Polyamorphism and Its Role in Biomineralization: How Many Amorphous Calcium Carbonates Are There? Cartwright, Julyan H. E.; Checa, Antonio G.; Gale, Julian D. Angewandte Chemie International Edition, Vol. 51, Issue 48 https://doi.org/10.1002/anie.201203125	journal	November 2012
Uncovering the True Atomic Structure of Disordered Materials: The Structure of a Hydrated Amorphous Magnesium Carbonate (MgCO ₃ ·3D ₂ O) White, Claire E.; Henson, Neil J.; Daemen, Luke L. Chemistry of Materials, Vol. 26, Issue 8 https://doi.org/10.1021/cm500470g	journal	April 2014
Energetic and structural studies of amorphous Ca1−xMgxCO3·nH2O (0⩽x⩽1) Radha, A. V.; Fernandez-Martinez, Alejandro; Hu, Yandi Geochimica et Cosmochimica Acta, Vol. 90 https://doi.org/10.1016/j.gca.2012.04.056	journal	August 2012
Structural Characteristics of Synthetic Amorphous Calcium Carbonate Michel, F. Marc; MacDonald, Jason; Feng, Jian Chemistry of Materials, Vol. 20, Issue 14 https://doi.org/10.1021/cm800324v	journal	July 2008
Nanoporous Structure and Medium-Range Order in Synthetic Amorphous Calcium Carbonate Goodwin, Andrew L.; Michel, F. Marc; Phillips, Brian L. Chemistry of Materials, Vol. 22, Issue 10 https://doi.org/10.1021/cm100294d	journal	May 2010
Structure and Transformation of Amorphous Calcium Carbonate: A Solid-State ⁴³ Ca NMR and Computational Molecular Dynamics Investigation Singer, Jared Wesley; Yazaydin, A. Özgür; Kirkpatrick, R. James Chemistry of Materials, Vol. 24, Issue 10 https://doi.org/10.1021/cm300389q	journal	May 2012
A Molecular Dynamics Study of the Early Stages of Calcium Carbonate Growth Tribello, Gareth A.; Bruneval, Fabien; Liew, CheeChin The Journal of Physical Chemistry B, Vol. 113, Issue 34 https://doi.org/10.1021/jp902606x	journal	August 2009
Structure and dynamics of the hydrated magnesium ion and of the solvated magnesium carbonates: insights from first principles simulations Tommaso, Devis Di; de Leeuw, Nora H. Phys. Chem. Chem. Phys., Vol. 12, Issue 4 https://doi.org/10.1039/B915329B	journal	January 2010
Hydration Energies and Structures of Alkaline Earth Metal Ions, M ²⁺ (H ₂ O) _n , n = 5−7, M = Mg, Ca, Sr, and Ba Rodriguez-Cruz, Sandra E.; Jockusch, Rebecca A.; Williams, Evan R. Journal of the American Chemical Society, Vol. 121, Issue 38 https://doi.org/10.1021/ja9911871	journal	September 1999
Transformation and crystallization energetics of synthetic and biogenic amorphous calcium carbonate Radha, A. V.; Forbes, T. Z.; Killian, C. E. Proceedings of the National Academy of Sciences, Vol. 107, Issue 38 https://doi.org/10.1073/pnas.1009959107	journal	September 2010
Automated high-pressure titration system with in situ infrared spectroscopic detection Thompson, Christopher J.; Martin, Paul F.; Chen, Jeffrey Review of Scientific Instruments, Vol. 85, Issue 4 https://doi.org/10.1063/1.4870411	journal	April 2014
A new method for in situ structural investigations of nano-sized amorphous and crystalline materials using mixed-flow reactors Hoeher, Alexandria; Mergelsberg, Sebastian; Borkiewicz, Olaf J. Acta Crystallographica Section A Foundations and Advances, Vol. 75, Issue 5 https://doi.org/10.1107/S2053273319008623	journal	August 2019
GSAS-II : the genesis of a modern open-source all purpose crystallography software package Toby, Brian H.; Von Dreele, Robert B. Journal of Applied Crystallography, Vol. 46, Issue 2 https://doi.org/10.1107/S0021889813003531	journal	March 2013
PDFfit2 and PDFgui: computer programs for studying nanostructure in crystals Farrow, C. L.; Juhas, P.; Liu, J. W. Journal of Physics: Condensed Matter, Vol. 19, Issue 33 https://doi.org/10.1088/0953-8984/19/33/335219	journal	July 2007
Generalized Gradient Approximation Made Simple Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868 https://doi.org/10.1103/PhysRevLett.77.3865	journal	October 1996
An all‐electron numerical method for solving the local density functional for polyatomic molecules Delley, B. The Journal of Chemical Physics, Vol. 92, Issue 1 https://doi.org/10.1063/1.458452	journal	January 1990
From molecules to solids with the DMol3 approach Delley, B. The Journal of Chemical Physics, Vol. 113, Issue 18 https://doi.org/10.1063/1.1316015	journal	November 2000
Special points for Brillouin-zone integrations Monkhorst, Hendrik J.; Pack, James D. Physical Review B, Vol. 13, Issue 12, p. 5188-5192 https://doi.org/10.1103/PhysRevB.13.5188	journal	June 1976
Semiempirical GGA-type density functional constructed with a long-range dispersion correction Grimme, Stefan Journal of Computational Chemistry, Vol. 27, Issue 15, p. 1787-1799 https://doi.org/10.1002/jcc.20495	journal	January 2006
Ab Initio Thermodynamic Model for Magnesium Carbonates and Hydrates Chaka, Anne M.; Felmy, Andrew R. The Journal of Physical Chemistry A, Vol. 118, Issue 35 https://doi.org/10.1021/jp500271n	journal	April 2014

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