Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Identical Water Dynamics in Acrylamide Hydrogels, Polymers, and Monomers in Solution: Ultrafast IR Spectroscopy and Molecular Dynamics Simulations

Journal Article · · Journal of the American Chemical Society
DOI:https://doi.org/10.1021/jacs.1c07151· OSTI ID:1850226

Not provided.

Research Organization:
Stanford Univ., CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC)
DOE Contract Number:
FG03-84ER13251
OSTI ID:
1850226
Journal Information:
Journal of the American Chemical Society, Vol. 143, Issue 36; ISSN 0002-7863
Publisher:
American Chemical Society (ACS)
Country of Publication:
United States
Language:
English

References (74)

Hydrogel: Preparation, characterization, and applications: A review March 2015
Polyacrylamide Gel Electrophoresis April 1971
Electrophoresis in Highly Cross-linked Polyacrylamide Gels December 1972
Polyacrylamide degradation and its implications in environmental systems September 2018
Soft contact lens polymers: an evolution December 2001
Hydraulically amplified self-healing electrostatic actuators with muscle-like performance January 2018
Designing hydrogels for controlled drug delivery October 2016
Self-Healing Hydrogels August 2016
Molecular Dynamics Study of Polymer−Water Interaction in Hydrogels. 1. Hydrogen-Bond Structure January 1996
Molecular Dynamics Study of Polymer−Water Interaction in Hydrogels. 2. Hydrogen-Bond Dynamics January 1996
Computer Simulation Studies on the Polymer-Induced Modification of Water Properties in Polyacrylamide Hydrogels May 1998
Dielectric Relaxation and Solvation Dynamics of Water in Complex Chemical and Biological Systems June 2000
Characterization of free, restricted, and entrapped water environments in poly( N -isopropyl acrylamide) hydrogels via 1 H HRMAS PFG NMR spectroscopy September 2014
Water Dynamics in Polyacrylamide Hydrogels July 2018
Dynamics of water probed with vibrational echo correlation spectroscopy January 2004
Water Dynamics:  Vibrational Echo Correlation Spectroscopy and Comparison to Molecular Dynamics Simulations February 2004
Watching Hydrogen Bonds Break:  A Transient Absorption Study of Water December 2004
On the orientational relaxation of HDO in liquid water September 2005
Hydrogen bond dynamics in aqueous NaBr solutions October 2007
Structural Dynamics of Aqueous Salt Solutions April 2008
Water Dynamics in Divalent and Monovalent Concentrated Salt Solutions November 2012
Effect of urea on the structural dynamics of water December 2006
Observation of Immobilized Water Molecules around Hydrophobic Groups October 2007
Water Dynamics in Water/DMSO Binary Mixtures April 2012
Water Dynamics in the Hydration Shells of Biomolecules March 2017
Water Dynamics in Nanoporous Silica: Ultrafast Vibrational Spectroscopy and Molecular Dynamics Simulations January 2019
Water dynamics in large and small reverse micelles: From two ensembles to collective behavior July 2009
Geometry and Nanolength Scales versus Interface Interactions: Water Dynamics in AOT Lamellar Structures and Reverse Micelles June 2009
Bulk-like and Interfacial Water Dynamics in Nafion Fuel Cell Membranes Investigated with Ultrafast Nonlinear IR Spectroscopy October 2019
Combined electronic structure/molecular dynamics approach for ultrafast infrared spectroscopy of dilute HOD in liquid H2O and D2O May 2004
Vibrational spectroscopy of HOD in liquid D2O. III. Spectral diffusion, and hydrogen-bonding and rotational dynamics January 2003
A Molecular Jump Mechanism of Water Reorientation February 2006
Why Water Reorientation Slows without Iceberg Formation around Hydrophobic Solutes February 2009
Vibrational Spectroscopy as a Probe of Structure and Dynamics in Liquid Water March 2010
Water Hydrogen-Bond Dynamics around Amino Acids: The Key Role of Hydrophilic Hydrogen-Bond Acceptor Groups February 2010
Structure and Dynamics of Urea/Water Mixtures Investigated by Vibrational Spectroscopy and Molecular Dynamics Simulation July 2013
On the role of hydrogen-bond exchanges in the spectral diffusion of water February 2021
Resonant intermolecular transfer of vibrational energy in liquid water December 1999
Water dynamics in small reverse micelles in two solvents: Two-dimensional infrared vibrational echoes with two-dimensional background subtraction February 2011
Frequency-frequency correlation functions and apodization in two-dimensional infrared vibrational echo spectroscopy: A new approach September 2007
Taking apart the two-dimensional infrared vibrational echo spectra: More information and elimination of distortions May 2008
Line shape analysis of two-dimensional infrared spectra June 2015
LigParGen web server: an automatic OPLS-AA parameter generator for organic ligands April 2017
Potential energy functions for atomic-level simulations of water and organic and biomolecular systems May 2005
1.14*CM1A-LBCC: Localized Bond-Charge Corrected CM1A Charges for Condensed-Phase Simulations January 2017
The missing term in effective pair potentials November 1987
PACKMOL: A package for building initial configurations for molecular dynamics simulations October 2009
Fast Parallel Algorithms for Short-Range Molecular Dynamics March 1995
Nuclear Quantum Effects in Water Reorientation and Hydrogen-Bond Dynamics May 2017
A unified formulation of the constant temperature molecular dynamics methods July 1984
Canonical dynamics: Equilibrium phase-space distributions March 1985
Constant pressure molecular dynamics algorithms September 1994
General formulation of pressure and stress tensor for arbitrary many-body interaction potentials under periodic boundary conditions October 2009
Numerical integration of the cartesian equations of motion of a system with constraints: molecular dynamics of n-alkanes March 1977
Comments on P3M, FMM, and the Ewald method for large periodic Coulombic systems June 1996
Particle mesh Ewald: An N ⋅log( N ) method for Ewald sums in large systems June 1993
Infrared and Raman Line Shapes of Dilute HOD in Liquid H 2 O and D 2 O from 10 to 90 °C July 2005
Tracking Water's Response to Structural Changes in Nafion Membranes July 2006
Steam and heat setting of nylon 6 fiber. IX. Changes in infrared spectra with deuteration of heat-set nylon 6 January 1965
Water inertial reorientation: Hydrogen bond strength and the angular potential April 2008
A theory of fluorescence polarization decay in membranes December 1977
On the wobbling-in-cone analysis of fluorescence anisotropy decay February 1982
Effect of librational motion on fluorescence depolarization and nuclear magnetic resonance relaxation in macromolecules and membranes June 1980
Molecular-Sieve Chromatography of Proteins on Granulated Polyacrylamide Gels January 1966
The spaces in a uniform random suspension of fibres January 1958
Water Layer at Hydrophobic Surface: Electrically Dead but Dynamically Alive? November 2020
How different are the dynamics of nanoconfined water? June 2020
CLS Next Gen: Accurate Frequency–Frequency Correlation Functions from Center Line Slope Analysis of 2D Correlation Spectra Using Artificial Neural Networks June 2020
Concepts and Methods of 2D Infrared Spectroscopy January 2011
Excitation Wavelength Dependence of Solvation Dynamics in a Gel. (PEO) 20 −(PPO) 70 −(PEO) 20 Triblock Copolymer June 2007
Hydration dynamics in aqueous Pluronic P123 solution: Concentration and temperature dependence November 2019
Structure, Activity, and Dynamics of Human Serum Albumin in a Crowded Pluronic F127 Hydrogel April 2019
2D IR spectroscopy reveals the role of water in the binding of channel-blocking drugs to the influenza M2 channel June 2014
Watching Proteins Wiggle: Mapping Structures with Two-Dimensional Infrared Spectroscopy January 2017

Similar Records

Dynamics of Water Molecules and Ions in Concentrated Lithium Chloride Solutions Probed with Ultrafast 2D IR Spectroscopy
Journal Article · 2019 · Journal of Physical Chemistry. B, Condensed Matter, Materials, Surfaces, Interfaces and Biophysical Chemistry · OSTI ID:1614573

Ultrafast to Ultraslow Dynamics of a Langmuir Monolayer at the Air/Water Interface Observed with Reflection Enhanced 2D IR Spectroscopy
Journal Article · 2017 · Journal of the American Chemical Society · OSTI ID:1539641

Related Subjects