Identifying Boron Active Sites for the Oxidative Dehydrogenation of Propane

Yan, Huan; Alayoglu, Selim; Wu, Weiqiang; Zhang, Yongbo; Weitz, Eric; Stair, Peter C.; Notestein, Justin M.

doi:10.1021/acscatal.1c02168

Identifying Boron Active Sites for the Oxidative Dehydrogenation of Propane

Journal Article · 13 July 2021 · ACS Catalysis

DOI:https://doi.org/10.1021/acscatal.1c02168· OSTI ID:1849446

Yan, Huan ^[1]; Alayoglu, Selim ^[2]; Wu, Weiqiang ^[2]; Zhang, Yongbo ^[3]; ^[4]; ^[4]; ^[5]

Department of Chemistry, Northwestern University, Evanston, Illinois 60208, United States; OSTI
Center for Catalysis and Surface Science, Northwestern University, Evanston, Illinois 60208, United States
Integrated Molecular Structure Education and Research Center, Northwestern University, Evanston, Illinois 60208, United States
Department of Chemistry, Northwestern University, Evanston, Illinois 60208, United States
Department of Chemical and Biological Engineering, Northwestern University, Evanston, Illinois 60208, United States

Not provided.

Research Organization:: Northwestern Univ., Evanston, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

DOE Contract Number:: FG02-03ER15457

OSTI ID:: 1849446

Journal Information:: ACS Catalysis, Journal Name: ACS Catalysis Journal Issue: 15 Vol. 11; ISSN 2155-5435

Publisher:: American Chemical Society (ACS)

Country of Publication:: United States

Language:: English

References (33)

Synthesis and Characterization of Silica-Supported Boron Oxide Catalysts for the Oxidative Dehydrogenation of Propane Love, Alyssa M.; Cendejas, Melissa C.; Thomas, Brijith The Journal of Physical Chemistry C, Vol. 123, Issue 44 https://doi.org/10.1021/acs.jpcc.9b07429	journal	July 2019
Structure and properties of vanadium oxide-zirconia catalysts for propane oxidative dehydrogenation Khodakov, A.; Yang, J.; Su, S. Journal of Catalysis, Vol. 177, Issue 2 https://doi.org/10.1006/jcat.1998.2143	journal	July 1998
Edge-hydroxylated Boron Nitride for Oxidative Dehydrogenation of Propane to Propylene Shi, Lei; Wang, Dongqi; Song, Wei ChemCatChem, Vol. 9, Issue 10 https://doi.org/10.1002/cctc.201700004	journal	April 2017
An ultraviolet Raman spectroscopic study of coke formation in methanol to hydrocarbons conversion over zeolite H-MFI Chua, Yek Tann; Stair, Peter C. Journal of Catalysis, Vol. 213, Issue 1 https://doi.org/10.1016/s0021-9517(02)00026-x	journal	January 2003
Boric acid treated HZSM-5 for improved catalyst activity in non-oxidative methane dehydroaromatization Balyan, Sonit; Haider, M. Ali; Khan, Tuhin S. Catalysis Science & Technology, Vol. 10, Issue 12 https://doi.org/10.1039/D0CY00286K	journal	January 2020
Isolated boron in zeolite for oxidative dehydrogenation of propane Zhou, Hang; Yi, Xianfeng; Hui, Yu Science, Vol. 372, Issue 6537 https://doi.org/10.1126/science.abe7935	journal	April 2021
Network Modification in Potassium Borate Glasses: Structural Studies with NMR and Raman Spectroscopies Youngman, Randall E.; Zwanziger, Josef W. The Journal of Physical Chemistry, Vol. 100, Issue 41 https://doi.org/10.1021/jp961439+	journal	January 1996
Borosilicate nanoparticles prepared by exothermic phase separation Parashar, Virendra K.; Orhan, Jean-Baptiste; Sayah, Abdeljalil Nature Nanotechnology, Vol. 3, Issue 10 https://doi.org/10.1038/nnano.2008.262	journal	September 2008
Selective oxidative dehydrogenation of propane to propene using boron nitride catalysts Grant, J. T.; Carrero, C. A.; Goeltl, F. Science, Vol. 354, Issue 6319 https://doi.org/10.1126/science.aaf7885	journal	December 2016
Highly Efficient Activation, Regeneration, and Active Site Identification of Oxide-Based Olefin Metathesis Catalysts Ding, Kunlun; Gulec, Ahmet; Johnson, Alexis M. ACS Catalysis, Vol. 6, Issue 9 https://doi.org/10.1021/acscatal.6b00098	journal	August 2016
Low cost tips for tip-enhanced Raman spectroscopy fabricated by two-step electrochemical etching of 125 µm diameter gold wires Foti, Antonino; Barreca, Francesco; Fazio, Enza Beilstein Journal of Nanotechnology, Vol. 9 https://doi.org/10.3762/bjnano.9.254	journal	January 2018
Boron and Boron-Containing Catalysts for the Oxidative Dehydrogenation of Propane Grant, Joseph T.; McDermott, William P.; Venegas, Juan M. ChemCatChem, Vol. 9, Issue 19 https://doi.org/10.1002/cctc.201701140	journal	September 2017
Analysis of TiO ₂ Atomic Layer Deposition Surface Chemistry and Evidence of Propene Oligomerization Using Surface-Enhanced Raman Spectroscopy Hackler, Ryan A.; Kang, Gyeongwon; Schatz, George C. Journal of the American Chemical Society, Vol. 141, Issue 1 https://doi.org/10.1021/jacs.8b10689	journal	December 2018
Dalton communication. Solid-state nuclear magnetic resonance studies on the co-ordination geometry of boron in polyoxotungstates Couto, Alexandra R.; Trovão, Cristina N.; Rocha, João J. Chem. Soc., Dalton Trans., Issue 17 https://doi.org/10.1039/dt9940002585	journal	January 1994
Supported Boron Oxide Catalysts for Selective and Low-Temperature Oxidative Dehydrogenation of Propane Lu, Wen-Duo; Wang, Dongqi; Zhao, Zhenchao ACS Catalysis, Vol. 9, Issue 9 https://doi.org/10.1021/acscatal.9b02284	journal	July 2019
Partial Oxidation of Ethane over Boron Oxide Added Catalysts Murakami, Yasushi; Otsuka, Kiyoshi; Wada, Yuji Chemistry Letters, Vol. 18, Issue 4 https://doi.org/10.1246/cl.1989.535	journal	April 1989
Dynamic Phase Diagram of Catalytic Surface of Hexagonal Boron Nitride under Conditions of Oxidative Dehydrogenation of Propane Zhang, Zisheng; Jimenez-Izal, Elisa; Hermans, Ive The Journal of Physical Chemistry Letters, Vol. 10, Issue 1 https://doi.org/10.1021/acs.jpclett.8b03373	journal	December 2018
Binaphthol-Catalyzed Asymmetric Conjugate Arylboration of Enones Turner, Heather M.; Patel, Jignesh; Niljianskul, Nootaree Organic Letters, Vol. 13, Issue 21 https://doi.org/10.1021/ol202391r	journal	October 2011
Probing the Chemistry of Alumina Atomic Layer Deposition Using Operando Surface-Enhanced Raman Spectroscopy Masango, Sicelo S.; Hackler, Ryan A.; Henry, Anne-Isabelle The Journal of Physical Chemistry C, Vol. 120, Issue 7 https://doi.org/10.1021/acs.jpcc.5b11487	journal	February 2016
Sustainability in Catalytic Oxidation: An Alternative Approach or a Structural Evolution? Cavani, Fabrizio; Teles, Joaquim Henrique ChemSusChem, Vol. 2, Issue 6 https://doi.org/10.1002/cssc.200900020	journal	June 2009
Why Boron Nitride is such a Selective Catalyst for the Oxidative Dehydrogenation of Propane Venegas, Juan M.; Zhang, Zisheng; Agbi, Theodore O. Angewandte Chemie International Edition, Vol. 59, Issue 38 https://doi.org/10.1002/anie.202003695	journal	July 2020
B‐MWW Zeolite: The Case Against Single‐Site Catalysis Altvater, Natalie R.; Dorn, Rick W.; Cendejas, Melissa C. Angewandte Chemie International Edition, Vol. 59, Issue 16 https://doi.org/10.1002/anie.201914696	journal	April 2020
On the Structure of Vanadium Oxide Supported on Aluminas: UV and Visible Raman Spectroscopy, UV−Visible Diffuse Reflectance Spectroscopy, and Temperature-Programmed Reduction Studies Wu, Zili; Kim, Hack-Sung; Stair, Peter C. The Journal of Physical Chemistry B, Vol. 109, Issue 7 https://doi.org/10.1021/jp046011m	journal	February 2005
Propane oxidative dehydrogenation over highly selective hexagonal boron nitride catalysts: The role of oxidative coupling of methyl Tian, Jinshu; Tan, Jiangqiao; Xu, Mingliang Science Advances, Vol. 5, Issue 3 https://doi.org/10.1126/sciadv.aav8063	journal	March 2019
Selective oxidative dehydrogenation of propane over V$z.sbnd;Mg$z.sbnd;O catalysts Chaar, M. Journal of Catalysis, Vol. 109, Issue 2 https://doi.org/10.1016/0021-9517(88)90226-6	journal	February 1988
Probing the Transformation of Boron Nitride Catalysts under Oxidative Dehydrogenation Conditions Love, Alyssa M.; Thomas, Brijith; Specht, Sarah E. Journal of the American Chemical Society, Vol. 141, Issue 1 https://doi.org/10.1021/jacs.8b08165	journal	November 2018
Nature of Silicon−Boron Mixing in Sodium Borosilicate Glasses: A High-Resolution ¹¹ B and ¹⁷ O NMR Study Du, Lin-Shu; Stebbins, Jonathan F. The Journal of Physical Chemistry B, Vol. 107, Issue 37 https://doi.org/10.1021/jp034048l	journal	September 2003
The Partial Oxidation of Ethane over a B ₂ O ₃ –Al ₂ O ₃ Catalyst Murakami, Yasushi; Otsuka, Kiyoshi; Wada, Yuji Bulletin of the Chemical Society of Japan, Vol. 63, Issue 2 https://doi.org/10.1246/bcsj.63.340	journal	February 1990
Boron Sites in Borosilicate Zeolites at Various Stages of Hydration Studied by Solid State NMR Spectroscopy Hwang, Son-Jong; Chen, Cong-Yan; Zones, Stacey I. The Journal of Physical Chemistry B, Vol. 108, Issue 48 https://doi.org/10.1021/jp0476904	journal	December 2004
Reactions of Laser-Ablated Boron Atoms with Ethylene and Ethane. Infrared Spectra and DFT Calculations for Several Novel BC ₂ H _x ( x = 1, 2, 3, 4, 5) Molecules Andrews, Lester; Lanzisera, Dominick V.; Hassanzadeh, Parviz The Journal of Physical Chemistry A, Vol. 102, Issue 19 https://doi.org/10.1021/jp980437h	journal	April 1998
Radical Chemistry and Reaction Mechanisms of Propane Oxidative Dehydrogenation over Hexagonal Boron Nitride Catalysts Zhang, Xuanyu; You, Rui; Wei, Zeyue Angewandte Chemie International Edition, Vol. 59, Issue 21 https://doi.org/10.1002/anie.202002440	journal	April 2020
Cross-Coupling Reactions Of Organoboranes: An Easy Way To Construct CC Bonds (Nobel Lecture) Suzuki, Akira Angewandte Chemie International Edition, Vol. 50, Issue 30 https://doi.org/10.1002/anie.201101379	journal	May 2011
VO _x /SiO ₂ Catalyst Prepared by Grafting VOCl ₃ on Silica for Oxidative Dehydrogenation of Propane Zhu, Haibo; Ould-Chikh, Samy; Dong, Hailin ChemCatChem, Vol. 7, Issue 20 https://doi.org/10.1002/cctc.201500607	journal	September 2015

Similar Records

Identifying Boron Active Sites for the Oxidative Dehydrogenation of Propane

Journal Article · 2021 · ACS Catalysis · OSTI ID:2482452

Dynamically Formed Active Sites on Liquid Boron Oxide for Selective Oxidative Dehydrogenation of Propane

Journal Article · 2023 · ACS Catalysis · OSTI ID:1988427

The Influence of Reactor Parameters on the Boron Nitride-Catalyzed Oxidative Dehydrogenation of Propane

Journal Article · 2018 · Organic Process Research & Development · OSTI ID:1612786

Related Subjects

Chemistry

Identifying Boron Active Sites for the Oxidative Dehydrogenation of Propane

Citation Formats

References (33)

Similar Records

Related Subjects