Simulating Oxidation of Carbon Surfaces by Atomic Oxygen Coupled with a Finite Rate Oxidation Model

Kirmanoglu, Kaan K.; Anderson, Nicholas A.; Panerai, Francesco; Stephani, Kelly A.; Ferguson, Joseph C.; Close, Sigrid

doi:10.2514/6.2022-0674

Simulating Oxidation of Carbon Surfaces by Atomic Oxygen Coupled with a Finite Rate Oxidation Model

Conference · 29 December 2021 · AIAA SCITECH 2022 Forum

DOI:https://doi.org/10.2514/6.2022-0674· OSTI ID:1844238

Kirmanoglu, Kaan K. ^[1]; Anderson, Nicholas A. ^[2]; Panerai, Francesco ^[2]; Stephani, Kelly A. ^[2]; Ferguson, Joseph C. ^[3]; Close, Sigrid ^[3]

Univ. of Illinois at Urbana-Champaign, IL (United States); University of Illinois
Univ. of Illinois at Urbana-Champaign, IL (United States)
Stanford Univ., CA (United States)

Oxidation is a prominent factor in degradation of carbon based ablative materials at high temperatures, resulting in mass loss and material recession through chemical and mechanical erosion. In this paper, a finite rate carbon oxidation model coupled with surface recession is implemented in the Porous Ablation and Thermal Response (Panther) software to investigate carbon oxidation by atomic oxygen over a range of temperatures and pressures. Panther is utilized to investigate the finite rate oxidation model proposed by Swaminathan-Gopalan et al. at conditions of higher pressure and flux relative to the experiments it was built on.

View Conference

Research Organization:: Univ. of Illinois at Urbana-Champaign, IL (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

DOE Contract Number:: NA0003963;

OSTI ID:: 1844238

Resource Type:: Conference paper

Conference Information:: Journal Name: AIAA SCITECH 2022 Forum

Country of Publication:: United States

Language:: English

References (24)

Über die von der molekularkinetischen Theorie der Wärme geforderte Bewegung von in ruhenden Flüssigkeiten suspendierten Teilchen Einstein, A. Annalen der Physik, Vol. 322, Issue 8 https://doi.org/10.1002/andp.19053220806	journal	January 1905
High temperature oxidation of carbon by atomic oxygen Rosner, D. E.; Allendorf, H. D. Carbon, Vol. 3, Issue 2 https://doi.org/10.1016/0008-6223(65)90042-4	journal	October 1965
Ordinary, transition, and Knudsen regime diffusion in random capillary structures Tomadakis, Manolis M.; Sotirchos, Stratis V. Chemical Engineering Science, Vol. 48, Issue 19 https://doi.org/10.1016/0009-2509(93)80149-K	journal	October 1993
Volume of fluid (VOF) method for the dynamics of free boundaries Hirt, C. W.; Nichols, B. D. Journal of Computational Physics, Vol. 39, Issue 1 https://doi.org/10.1016/0021-9991(81)90145-5	journal	January 1981
The sticking probabilities of gases chemisorbed on the surfaces of solids Kisliuk, P. Journal of Physics and Chemistry of Solids, Vol. 3, Issue 1-2 https://doi.org/10.1016/0022-3697(57)90054-9	journal	January 1957
Modeling the oxidation of low-density carbon fiber material based on micro-tomography Ferguson, Joseph C.; Panerai, Francesco; Lachaud, Jean Carbon, Vol. 96 https://doi.org/10.1016/j.carbon.2015.08.113	journal	January 2016
Theoretical study on the micro-scale oxidation of resin-infused carbon ablators Ferguson, Joseph C.; Panerai, Francesco; Lachaud, Jean Carbon, Vol. 121 https://doi.org/10.1016/j.carbon.2017.06.013	journal	September 2017
Development and validation of a finite-rate model for carbon oxidation by atomic oxygen Swaminathan-Gopalan, Krishnan; Borner, Arnaud; Murray, Vanessa J. Carbon, Vol. 137 https://doi.org/10.1016/j.carbon.2018.04.088	journal	October 2018
Oxidation and nitridation of vitreous carbon at high temperatures Murray, Vanessa J.; Recio, Pedro; Caracciolo, Adriana Carbon, Vol. 167 https://doi.org/10.1016/j.carbon.2020.05.076	journal	October 2020
A Brownian motion technique to simulate gasification and its application to C/C composite ablation Lachaud, J.; Vignoles, G. L. Computational Materials Science, Vol. 44, Issue 4 https://doi.org/10.1016/j.commatsci.2008.07.015	journal	February 2009
Micro-tomography based analysis of thermal conductivity, diffusivity and oxidation behavior of rigid and flexible fibrous insulators Panerai, Francesco; Ferguson, Joseph C.; Lachaud, Jean International Journal of Heat and Mass Transfer, Vol. 108 https://doi.org/10.1016/j.ijheatmasstransfer.2016.12.048	journal	May 2017
PuMA: the Porous Microstructure Analysis software Ferguson, Joseph C.; Panerai, Francesco; Borner, Arnaud SoftwareX, Vol. 7 https://doi.org/10.1016/j.softx.2018.03.001	journal	January 2018
Update 3.0 to “PuMA: The Porous Microstructure Analysis software”, (PII:S2352711018300281) Ferguson, Joseph C.; Semeraro, Federico; Thornton, John M. SoftwareX, Vol. 15 https://doi.org/10.1016/j.softx.2021.100775	journal	July 2021
Inelastic and Reactive Scattering Dynamics of Hyperthermal O and O ₂ on Hot Vitreous Carbon Surfaces Murray, Vanessa J.; Marshall, Brooks C.; Woodburn, Philip J. The Journal of Physical Chemistry C, Vol. 119, Issue 26 https://doi.org/10.1021/acs.jpcc.5b00924	journal	April 2015
Surface Precursors and Reaction Mechanisms for the Thermal Reduction of Graphene Basal Surfaces Oxidized by Atomic Oxygen Sun, Tao; Fabris, Stefano; Baroni, Stefano The Journal of Physical Chemistry C, Vol. 115, Issue 11 https://doi.org/10.1021/jp111372k	journal	February 2011
An Inverse Method for The Generation of Random Normal Deviates on Large-Scale Computers Muller, Mervin E. Mathematical Tables and Other Aids to Computation, Vol. 12, Issue 63 https://doi.org/10.2307/2002017	journal	July 1958
Multiscale Approach to Ablation Modeling of Phenolic Impregnated Carbon Ablators Lachaud, Jean; Cozmuta, Ioana; Mansour, Nagi N. Journal of Spacecraft and Rockets, Vol. 47, Issue 6 https://doi.org/10.2514/1.42681	journal	November 2010
Molecular Simulation of Carbon Ablation Using Beam Experiments and Resolved Microstructure Poovathingal, Savio; Schwartzentruber, Thomas E.; Murray, Vanessa J. AIAA Journal, Vol. 54, Issue 3 https://doi.org/10.2514/1.J054562	journal	March 2016
Finite-Rate Oxidation Model for Carbon Surfaces from Molecular Beam Experiments Poovathingal, Savio; Schwartzentruber, Thomas E.; Murray, Vanessa J. AIAA Journal, Vol. 55, Issue 5 https://doi.org/10.2514/1.J055371	journal	May 2017
Air–Carbon Ablation Model for Hypersonic Flight from Molecular-Beam Data Prata, Krishna Sandeep; Schwartzentruber, Thomas E.; Minton, Timothy K. AIAA Journal, Vol. 60, Issue 2 https://doi.org/10.2514/1.J060516	journal	February 2022
Viscous Shock-Layer Simulation of Airflow past Ablating Blunt Body with Carbon Surface Zhluktov, Sergey V.; Abe, Takashi Journal of Thermophysics and Heat Transfer, Vol. 13, Issue 1 https://doi.org/10.2514/2.6400	journal	January 1999
Comparative studies of the attack of pyrolytic and isotropic graphite by atomic and molecular oxygen at high temperatures. Rosner, Daniel E.; Allendor, H. Donald AIAA Journal, Vol. 6, Issue 4 https://doi.org/10.2514/3.4558	journal	April 1968
Effects of atomic oxygen on graphite ablation Park, Chul AIAA Journal, Vol. 14, Issue 11 https://doi.org/10.2514/3.7267	journal	November 1976
Development of a Detailed Surface Chemistry Framework in DSMC Swaminathan Gopalan, Krishnan; Stephani, Kelly A. 2018 AIAA Aerospace Sciences Meeting, 2018 AIAA Aerospace Sciences Meeting https://doi.org/10.2514/6.2018-0494	conference	January 2018

Similar Records

Erosion-oxidation of carbon steel in the convection section of an industrial boiler cofiring coal-water fuel and natural gas

Journal Article · 1997 · Journal of Engineering for Gas Turbines and Power · OSTI ID:533054

Oxidation kinetics of a continuous carbon phase in a nonreactive matrix

Journal Article · 1995 · Journal of the American Ceramic Society · OSTI ID:82590

A comparison of carbon depletion on STS-8 with atmospheric atomic oxygen flux

Journal Article · 1996 · AIP Conference Proceedings · OSTI ID:385424

Simulating Oxidation of Carbon Surfaces by Atomic Oxygen Coupled with a Finite Rate Oxidation Model

Citation Formats

References (24)

Similar Records

Related Subjects