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Title: Multifunctional Metal–Oxide Nanocomposite Thin Film with Plasmonic Au Nanopillars Embedded in Magnetic La 0.67Sr 0.33MnO 3 Matrix

Abstract

Searching for multifunctional materials with tunable magnetic and optical properties has been a critical task toward the implementation of future integrated optical devices. Vertically aligned nanocomposite (VAN) thin films provide a unique platform for multifunctional material designs. In this work, a new metal–oxide VAN has been designed with plasmonic Au nanopillars embedded in a ferromagnetic La 0.67Sr 0.33MnO 3 (LSMO) matrix. Such Au–LSMO nanocomposite presents intriguing plasmon resonance in the visible range and magnetic anisotropy property, which are functionalized by the Au and LSMO phase, respectively. Furthermore, the vertically aligned nanostructure of metal and dielectric oxide results in the hyperbolic property for near-field electromagnetic wave manipulation. Such optical and magnetic response could be further tailored by tuning the composition of Au and LSMO phases.

Authors:
 [1]; ORCiD logo [2];  [2];  [3];  [2];  [2];  [2]; ORCiD logo [2]
  1. Sun Yat-Sen Univ., Guangzhou (China)
  2. Purdue Univ., West Lafayette, IN (United States)
  3. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Publication Date:
Research Org.:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF); Guangdong Basic and Applied Research Foundation
OSTI Identifier:
1760432
Report Number(s):
SAND-2020-14121J
Journal ID: ISSN 1530-6984; 693046
Grant/Contract Number:  
AC04-94AL85000; SC0020077; DMR-1565822; DMR-1809520; 2019A1515111029; NA0003525
Resource Type:
Journal Article: Accepted Manuscript
Journal Name:
Nano Letters
Additional Journal Information:
Journal Name: Nano Letters; Journal ID: ISSN 1530-6984
Publisher:
American Chemical Society
Country of Publication:
United States
Language:
English
Subject:
Thin films; gold; nanocomposites; magnetic properties; optical properties

Citation Formats

Huang, Jijie, Wang, Han, Qi, Zhimin, Lu, Ping, Zhang, Di, Zhang, Bruce, He, Zihao, and Wang, Haiyan. Multifunctional Metal–Oxide Nanocomposite Thin Film with Plasmonic Au Nanopillars Embedded in Magnetic La0.67Sr0.33MnO3 Matrix. United States: N. p., 2021. Web. doi:10.1021/acs.nanolett.0c04213.
Huang, Jijie, Wang, Han, Qi, Zhimin, Lu, Ping, Zhang, Di, Zhang, Bruce, He, Zihao, & Wang, Haiyan. Multifunctional Metal–Oxide Nanocomposite Thin Film with Plasmonic Au Nanopillars Embedded in Magnetic La0.67Sr0.33MnO3 Matrix. United States. https://doi.org/10.1021/acs.nanolett.0c04213
Huang, Jijie, Wang, Han, Qi, Zhimin, Lu, Ping, Zhang, Di, Zhang, Bruce, He, Zihao, and Wang, Haiyan. Wed . "Multifunctional Metal–Oxide Nanocomposite Thin Film with Plasmonic Au Nanopillars Embedded in Magnetic La0.67Sr0.33MnO3 Matrix". United States. https://doi.org/10.1021/acs.nanolett.0c04213.
@article{osti_1760432,
title = {Multifunctional Metal–Oxide Nanocomposite Thin Film with Plasmonic Au Nanopillars Embedded in Magnetic La0.67Sr0.33MnO3 Matrix},
author = {Huang, Jijie and Wang, Han and Qi, Zhimin and Lu, Ping and Zhang, Di and Zhang, Bruce and He, Zihao and Wang, Haiyan},
abstractNote = {Searching for multifunctional materials with tunable magnetic and optical properties has been a critical task toward the implementation of future integrated optical devices. Vertically aligned nanocomposite (VAN) thin films provide a unique platform for multifunctional material designs. In this work, a new metal–oxide VAN has been designed with plasmonic Au nanopillars embedded in a ferromagnetic La0.67Sr0.33MnO3 (LSMO) matrix. Such Au–LSMO nanocomposite presents intriguing plasmon resonance in the visible range and magnetic anisotropy property, which are functionalized by the Au and LSMO phase, respectively. Furthermore, the vertically aligned nanostructure of metal and dielectric oxide results in the hyperbolic property for near-field electromagnetic wave manipulation. Such optical and magnetic response could be further tailored by tuning the composition of Au and LSMO phases.},
doi = {10.1021/acs.nanolett.0c04213},
url = {https://www.osti.gov/biblio/1760432}, journal = {Nano Letters},
issn = {1530-6984},
number = ,
volume = ,
place = {United States},
year = {2021},
month = {1}
}

Journal Article:
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This content will become publicly available on January 6, 2022
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