Efficient Electrochemical Water Oxidation by a Trinuclear Ru(bda) Macrocycle Immobilized on Multi;#8208;Walled Carbon Nanotube Electrodes

Schindler, Dorothee; Gil,; Sepulcre, Marcos; Lindner, Joachim O.; Stepanenko, Vladimir; Moonshiram, Dooshaye; Llobet, Antoni; Würthner, Frank

doi:10.1002/aenm.202002329

Title: Efficient Electrochemical Water Oxidation by a Trinuclear Ru(bda) Macrocycle Immobilized on Multi;#8208;Walled Carbon Nanotube Electrodes

Journal Article · Fri Nov 20 00:00:00 EST 2020 · Adv. Energy Mat.

DOI:https://doi.org/10.1002/aenm.202002329· OSTI ID:1718962

Schindler, Dorothee; Gil,; Sepulcre, Marcos; Lindner, Joachim O.; Stepanenko, Vladimir; Moonshiram, Dooshaye; Llobet, Antoni; Würthner, Frank ^[1]

Wurzburg

Cite

Export

Save

Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source (APS)

Sponsoring Organization:: FOREIGN

OSTI ID:: 1718962

Journal Information:: Adv. Energy Mat., Vol. 10, Issue (43) ; 11, 2020

Country of Publication:: United States

Language:: ENGLISH

References (51)

Powering the future of molecular artificial photosynthesis with light-harvesting metallosupramolecular dye assemblies Frischmann, Peter D.; Mahata, Kingsuk; Würthner, Frank Chem. Soc. Rev., Vol. 42, Issue 4 https://doi.org/10.1039/C2CS35223K	journal	January 2013
Molecular artificial photosynthesis Berardi, Serena; Drouet, Samuel; Francàs, Laia Chem. Soc. Rev., Vol. 43, Issue 22 https://doi.org/10.1039/C3CS60405E	journal	January 2014
Artificial photosynthesis: opportunities and challenges of molecular catalysts Zhang, Biaobiao; Sun, Licheng Chemical Society Reviews, Vol. 48, Issue 7 https://doi.org/10.1039/C8CS00897C	journal	January 2019
Solar Water Splitting Cells Walter, Michael G.; Warren, Emily L.; McKone, James R. Chemical Reviews, Vol. 110, Issue 11, p. 6446-6473 https://doi.org/10.1021/cr1002326	journal	November 2010
Towards a Bioinspired-Systems Approach for Solar Fuel Devices Detz, Remko J.; Sakai, Ken; Spiccia, Leone ChemPlusChem, Vol. 81, Issue 10 https://doi.org/10.1002/cplu.201600446	journal	October 2016
Toward a Low‐Cost Artificial Leaf: Driving Carbon‐Based and Bifunctional Catalyst Electrodes with Solution‐Processed Perovskite Photovoltaics Sharifi, Tiva; Larsen, Christian; Wang, Jia Advanced Energy Materials, Vol. 6, Issue 20 https://doi.org/10.1002/aenm.201600738	journal	July 2016
Chemistry Future: Priorities and Opportunities from the Sustainability Perspective Beller, Matthias; Centi, Gabriele; Sun, Licheng ChemSusChem, Vol. 10, Issue 1 https://doi.org/10.1002/cssc.201601739	journal	December 2016
Hydrogen Bockris, John O’M. Materials, Vol. 4, Issue 12 https://doi.org/10.3390/ma4122073	journal	November 2011
Solar-to-Hydrogen Energy Conversion Based on Water Splitting Qi, Jing; Zhang, Wei; Cao, Rui Advanced Energy Materials, Vol. 8, Issue 5 https://doi.org/10.1002/aenm.201701620	journal	October 2017
Will Solar-Driven Water-Splitting Devices See the Light of Day? McKone, James R.; Lewis, Nathan S.; Gray, Harry B. Chemistry of Materials, Vol. 26, Issue 1 https://doi.org/10.1021/cm4021518	journal	September 2013
Rational Design Rules for Molecular Water Oxidation Catalysts based on Scaling Relationships Hessels, Joeri; Detz, Remko J.; Koper, Marc T. M. Chemistry - A European Journal, Vol. 23, Issue 65 https://doi.org/10.1002/chem.201702850	journal	November 2017
Heterogeneous photocatalyst materials for water splitting Kudo, Akihiko; Miseki, Yugo Chem. Soc. Rev., Vol. 38, Issue 1 https://doi.org/10.1039/B800489G	journal	January 2009
Water Oxidation Catalysts for Artificial Photosynthesis Ye, Sheng; Ding, Chunmei; Liu, Mingyao Advanced Materials, Vol. 31, Issue 50 https://doi.org/10.1002/adma.201902069	journal	July 2019
Mechanism of Catalytic Water Oxidation by the Ruthenium Blue Dimer Catalyst: Comparative Study in D2O versus H2O Moonshiram, Dooshaye; Purohit, Vatsal; Concepcion, Javier Materials, Vol. 6, Issue 2 https://doi.org/10.3390/ma6020392	journal	January 2013
Ru-bda: Unique Molecular Water-Oxidation Catalysts with Distortion Induced Open Site and Negatively Charged Ligands Zhang, Biaobiao; Sun, Licheng Journal of the American Chemical Society, Vol. 141, Issue 14 https://doi.org/10.1021/jacs.8b12862	journal	March 2019
Catalytic Oxidation of Water to Dioxygen by Mononuclear Ru Complexes Bearing a 2,6‐Pyridinedicarboxylato Ligand Hoque, Md Asmaul; Benet‐Buchholz, Jordi; Llobet, Antoni ChemSusChem, Vol. 12, Issue 9 https://doi.org/10.1002/cssc.201802996	journal	November 2018
Redox‐Active Ligand Assisted Catalytic Water Oxidation by a Ru ^IV =O Intermediate Shi, Jing; Guo, Yu‐Hua; Xie, Fei Angewandte Chemie International Edition, Vol. 59, Issue 10 https://doi.org/10.1002/anie.201910614	journal	January 2020
A molecular ruthenium catalyst with water-oxidation activity comparable to that of photosystem II Duan, Lele; Bozoglian, Fernando; Mandal, Sukanta Nature Chemistry, Vol. 4, Issue 5 https://doi.org/10.1038/nchem.1301	journal	March 2012
Molecular water-oxidation catalysts for photoelectrochemical cells Brimblecombe, Robin; Dismukes, G. Charles; Swiegers, Gerhard F. Dalton Transactions, Issue 43 https://doi.org/10.1039/b912669d	journal	January 2009
Single-Site, Catalytic Water Oxidation on Oxide Surfaces Chen, Zuofeng; Concepcion, Javier J.; Jurss, Jonah W. Journal of the American Chemical Society, Vol. 131, Issue 43, p. 15580-15581 https://doi.org/10.1021/ja906391w	journal	November 2009
Molecular Engineering of a 3D Self‐Supported Electrode for Oxygen Electrocatalysis in Neutral Media Xie, Lisi; Li, Xialiang; Wang, Bin Angewandte Chemie International Edition, Vol. 58, Issue 52 https://doi.org/10.1002/anie.201911441	journal	December 2019
Hybrid Photoelectrochemical Water Splitting Systems: From Interface Design to System Assembly Niu, Fujun; Wang, Degao; Li, Fei Advanced Energy Materials, Vol. 10, Issue 11 https://doi.org/10.1002/aenm.201900399	journal	June 2019
Ru‐Hbpp‐Based Water‐Oxidation Catalysts Anchored on Conducting Solid Supports Mola, Joaquim; Mas‐Marza, Elena; Sala, Xavier Angewandte Chemie International Edition, Vol. 47, Issue 31 https://doi.org/10.1002/anie.200704912	journal	July 2008
Visible Light Driven Water Splitting in a Molecular Device with Unprecedentedly High Photocurrent Density Gao, Yan; Ding, Xin; Liu, Jianhui Journal of the American Chemical Society, Vol. 135, Issue 11 https://doi.org/10.1021/ja400402d	journal	March 2013
Visible light-driven water oxidation with a subporphyrin sensitizer and a water oxidation catalyst Yamamoto, Masanori; Nishizawa, Yusuke; Chábera, Pavel Chemical Communications, Vol. 52, Issue 94 https://doi.org/10.1039/C6CC07877J	journal	January 2016
High-Performance Photoelectrochemical Cells Based on a Binuclear Ruthenium Catalyst for Visible-Light-Driven Water Oxidation Zhang, Linlin; Gao, Yan; Ding, Xin ChemSusChem, Vol. 7, Issue 10 https://doi.org/10.1002/cssc.201402561	journal	August 2014
Immobilizing Ru(bda) Catalyst on a Photoanode via Electrochemical Polymerization for Light-Driven Water Splitting Li, Fusheng; Fan, Ke; Wang, Lei ACS Catalysis, Vol. 5, Issue 6 https://doi.org/10.1021/cs502115f	journal	May 2015
Pt-free tandem molecular photoelectrochemical cells for water splitting driven by visible light Fan, Ke; Li, Fusheng; Wang, Lei Phys. Chem. Chem. Phys., Vol. 16, Issue 46 https://doi.org/10.1039/C4CP04489D	journal	January 2014
Chasing the Achilles’ Heel in Hybrid Systems of Diruthenium Water Oxidation Catalysts Anchored on Indium Tin Oxide: The Stability of the Anchor Odrobina, Jann; Scholz, Julius; Risch, Marcel ACS Catalysis, Vol. 7, Issue 9 https://doi.org/10.1021/acscatal.7b01883	journal	August 2017
Highly Efficient Oxidation of Water by a Molecular Catalyst Immobilized on Carbon Nanotubes Li, Fei; Zhang, Biaobiao; Li, Xiaona Angewandte Chemie International Edition, Vol. 50, Issue 51 https://doi.org/10.1002/anie.201105044	journal	October 2011
A Million Turnover Molecular Anode for Catalytic Water Oxidation Creus, Jordi; Matheu, Roc; Peñafiel, Itziar Angewandte Chemie International Edition, Vol. 55, Issue 49 https://doi.org/10.1002/anie.201609167	journal	November 2016
Current Progress on the Chemical Modification of Carbon Nanotubes Karousis, Nikolaos; Tagmatarchis, Nikos; Tasis, Dimitrios Chemical Reviews, Vol. 110, Issue 9 https://doi.org/10.1021/cr100018g	journal	September 2010
Efficient Energy-Conversion Materials for the Future: Understanding and Tailoring Charge-Transfer Processes in Carbon Nanostructures Strauss, Volker; Roth, Alexandra; Sekita, Michael Chem, Vol. 1, Issue 4 https://doi.org/10.1016/j.chempr.2016.09.001	journal	October 2016
Carbon nanotubes—electronic/electrochemical properties and application for nanoelectronics and photonics Sgobba, Vito; Guldi, Dirk M. Chem. Soc. Rev., Vol. 38, Issue 1 https://doi.org/10.1039/B802652C	journal	January 2009
Carbon nanotube-modified electrodes for solar energy conversion Umeyama, Tomokazu; Imahori, Hiroshi Energy & Environmental Science, Vol. 1, Issue 1 https://doi.org/10.1039/b805419n	journal	January 2008
Carbon Nanotubes with Cobalt Corroles for Hydrogen and Oxygen Evolution in pH 0-14 Solutions Li, Xialiang; Lei, Haitao; Liu, Jieyu Angewandte Chemie International Edition, Vol. 57, Issue 46 https://doi.org/10.1002/anie.201807996	journal	October 2018
Attaching Cobalt Corroles onto Carbon Nanotubes: Verification of Four-Electron Oxygen Reduction by Mononuclear Cobalt Complexes with Significantly Improved Efficiency Meng, Jia; Lei, Haitao; Li, Xialiang ACS Catalysis, Vol. 9, Issue 5 https://doi.org/10.1021/acscatal.9b00213	journal	April 2019
Molecular Water Oxidation Mechanisms Followed by Transition Metals: State of the Art Sala, Xavier; Maji, Somnath; Bofill, Roger Accounts of Chemical Research, Vol. 47, Issue 2 https://doi.org/10.1021/ar400169p	journal	December 2013
Electronic, mechanistic, and structural factors that influence the performance of molecular water oxidation catalysts anchored on electrode surfaces Garrido-Barros, Pablo; Matheu, Roc; Gimbert-Suriñach, Carolina Current Opinion in Electrochemistry, Vol. 15 https://doi.org/10.1016/j.coelec.2019.04.027	journal	June 2019
Behavior of the Ru-bda Water Oxidation Catalyst Covalently Anchored on Glassy Carbon Electrodes Matheu, Roc; Francàs, Laia; Chernev, Petko ACS Catalysis, Vol. 5, Issue 6 https://doi.org/10.1021/acscatal.5b00132	journal	May 2015
Foot of the Wave Analysis for Mechanistic Elucidation and Benchmarking Applications in Molecular Water Oxidation Catalysis Matheu, Roc; Neudeck, Sven; Meyer, Franc ChemSusChem, Vol. 9, Issue 23 https://doi.org/10.1002/cssc.201601286	journal	November 2016
O–O bond formation in ruthenium-catalyzed water oxidation: single-site nucleophilic attack vs. O–O radical coupling Shaffer, David W.; Xie, Yan; Concepcion, Javier J. Chemical Society Reviews, Vol. 46, Issue 20 https://doi.org/10.1039/C7CS00542C	journal	January 2017
A supramolecular ruthenium macrocycle with high catalytic activity for water oxidation that mechanistically mimics photosystem II Schulze, Marcus; Kunz, Valentin; Frischmann, Peter D. Nature Chemistry, Vol. 8, Issue 6 https://doi.org/10.1038/nchem.2503	journal	May 2016
Supramolecular Approaches to Improve the Performance of Ruthenium-Based Water Oxidation Catalysts Kunz, Valentin; Schmidt, David; Röhr, Merle I. S. Advanced Energy Materials, Vol. 7, Issue 16 https://doi.org/10.1002/aenm.201602939	journal	June 2017
Intramolecular Proton Transfer Boosts Water Oxidation Catalyzed by a Ru Complex Matheu, Roc; Ertem, Mehmed Z.; Benet-Buchholz, Jordi Journal of the American Chemical Society, Vol. 137, Issue 33 https://doi.org/10.1021/jacs.5b06541	journal	August 2015
Turnover Numbers, Turnover Frequencies, and Overpotential in Molecular Catalysis of Electrochemical Reactions. Cyclic Voltammetry and Preparative-Scale Electrolysis Costentin, Cyrille; Drouet, Samuel; Robert, Marc Journal of the American Chemical Society, Vol. 134, Issue 27, p. 11235-11242 https://doi.org/10.1021/ja303560c	journal	June 2012
A Local Proton Source Enhances CO ₂ Electroreduction to CO by a Molecular Fe Catalyst Costentin, Cyrille; Drouet, Samuel; Robert, Marc Science, Vol. 338, Issue 6103 https://doi.org/10.1126/science.1224581	journal	October 2012
Toward the rational benchmarking of homogeneous H ₂ -evolving catalysts Artero, Vincent; Saveant, Jean-Michel Energy Environ. Sci., Vol. 7, Issue 11 https://doi.org/10.1039/C4EE01709A	journal	January 2014
Multielectron, Multistep Molecular Catalysis of Electrochemical Reactions: Benchmarking of Homogeneous Catalysts Costentin, Cyrille; Savéant, Jean-Michel ChemElectroChem, Vol. 1, Issue 7 https://doi.org/10.1002/celc.201300263	journal	June 2014
Molecular Catalysis of H ₂ Evolution: Diagnosing Heterolytic versus Homolytic Pathways Costentin, Cyrille; Dridi, Hachem; Savéant, Jean-Michel Journal of the American Chemical Society, Vol. 136, Issue 39 https://doi.org/10.1021/ja505845t	journal	September 2014
Benchmarking of Homogeneous Electrocatalysts: Overpotential, Turnover Frequency, Limiting Turnover Number Costentin, Cyrille; Passard, Guillaume; Savéant, Jean-Michel Journal of the American Chemical Society, Vol. 137, Issue 16 https://doi.org/10.1021/jacs.5b00914	journal	April 2015

Similar Records

Enhancement of the efficiency of dye-sensitized solar cell with multi-wall carbon nanotubes/polypyrrole composite counter electrodes prepared by electrophoresis/electrochemical polymerization

Journal Article · Fri Mar 15 00:00:00 EDT 2013 · Materials Research Bulletin · OSTI ID:1718962

Luo, Jun; Niu, Hai-jun; Wen, Hai-lin; +5 more

Behavior of the Ru-bda water oxidation catalyst covalently anchored on glassy carbon electrodes

Journal Article · Thu May 07 00:00:00 EDT 2015 · ACS Catalysis · OSTI ID:1718962

Matheu, Roc; Francàs, Laia; Chernev, Petko; +5 more

Immobilization of ruthenium phthalocyanine on silica-coated multi-wall partially oriented carbon nanotubes: Electrochemical detection of fenitrothion pesticide

Journal Article · Fri Apr 15 00:00:00 EDT 2016 · Materials Research Bulletin · OSTI ID:1718962

Prado, Thiago M.; Cincotto, Fernando H.; Machado, Sergio A.S.

Title: Efficient Electrochemical Water Oxidation by a Trinuclear Ru(bda) Macrocycle Immobilized on Multi;#8208;Walled Carbon Nanotube Electrodes

Citation Formats

References (51)

Similar Records

Related Subjects