Pathways to excitation of atoms with bicircular laser pulses

Venzke, J.; Gebre, Y.; Becker, A.; Jarón-Becker, A.

doi:10.1103/physreva.101.053425

Title: Pathways to excitation of atoms with bicircular laser pulses

Journal Article · Thu May 14 00:00:00 EDT 2020 · Physical Review A

DOI:https://doi.org/10.1103/physreva.101.053425· OSTI ID:1712954

^[1];

^[1]; Jarón-Becker, A. ^[1]

Univ. of Colorado, Boulder, CO (United States)

We study the excitation of the hydrogen atom by bichromatic circularly polarized laser pulses using numerical solutions of the time-dependent Schrödinger equation. The results are in agreement with the selection rules for multiphoton processes in such fields, namely, excited states are populated in which orbital angular momentum and magnetic quantum numbers are either both odd or both even, independent of the relative helicity, peak intensity, and pulse duration of the pulses. For co-rotating pulses the results show that excitation predominantly proceeds to states with magnetic quantum number of the same helicity as the laser pulses. Besides pathways via direct photon absorption from the ground state our results indicate that a transfer of population among the Rydberg states occurs via Λ-type transitions. In the case of counter-rotating pulses the largest excitation probability is found for Rydberg states that differ in magnetic quantum number by Δm=±3. This pattern allows us to estimate how many photons from each of the two bichromatic fields have been absorbed. Finally, we confirm that a population in Rydberg states beyond a maximum orbital angular quantum number is unlikely.

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Research Organization:: Univ. of Colorado, Boulder, CO (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division; National Science Foundation (NSF)

Grant/Contract Number:: SC0001771; PHY-1734006

OSTI ID:: 1712954

Journal Information:: Physical Review A, Vol. 101, Issue 5; ISSN 2469-9926

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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