Linkage Effect in the Heterogenization of Cobalt Complexes by Doped Graphene for Electrocatalytic CO2 Reduction

Wang, J; Huang, X.; Xi, S.; Lee, J.; Wang, C.; Du, Y.; Wang, X.

doi:10.1002/anie.201906475

Linkage Effect in the Heterogenization of Cobalt Complexes by Doped Graphene for Electrocatalytic CO2 Reduction

Journal Article · 01 January 2022 · Angewandte Chemie (International Edition)

DOI:https://doi.org/10.1002/anie.201906475· OSTI ID:1689566

Wang, J; Huang, X.; Xi, S.; Lee, J.; Wang, C.; Du, Y.; Wang, X.

Research Organization:: Brookhaven National Lab. (BNL), Upton, NY (United States)

Sponsoring Organization:: ~OTHER

DOE Contract Number:: SC0012704

OSTI ID:: 1689566

Report Number(s):: BNL-220182-2020-JACI

Journal Information:: Angewandte Chemie (International Edition), Vol. 58, Issue 38

Country of Publication:: United States

Language:: English

References (56)

Electrochemical CO₂ Reduction on Metal Electrodes Hori, Y.; Vayenas, Constantinos G.; White, Ralph E. Modern Aspects of Electrochemistry, p. 89-189 https://doi.org/10.1007/978-0-387-49489-0_3	book	January 2008
Opportunities and prospects in the chemical recycling of carbon dioxide to fuels Centi, Gabriele; Perathoner, Siglinda Catalysis Today, Vol. 148, Issue 3-4 https://doi.org/10.1016/j.cattod.2009.07.075	journal	November 2009
The teraton challenge. A review of fixation and transformation of carbon dioxide Mikkelsen, Mette; Jørgensen, Mikkel; Krebs, Frederik C. Energy Environ. Sci., Vol. 3, Issue 1 https://doi.org/10.1039/B912904A	journal	January 2010
A review of catalysts for the electroreduction of carbon dioxide to produce low-carbon fuels Qiao, Jinli; Liu, Yuyu; Hong, Feng Chem. Soc. Rev., Vol. 43, Issue 2 https://doi.org/10.1039/C3CS60323G	journal	January 2014
Hydronium-Induced Switching between CO ₂ Electroreduction Pathways Seifitokaldani, Ali; Gabardo, Christine M.; Burdyny, Thomas Journal of the American Chemical Society, Vol. 140, Issue 11 https://doi.org/10.1021/jacs.7b13542	journal	February 2018
Mechanism of CO ₂ Reduction at Copper Surfaces: Pathways to C ₂ Products Garza, Alejandro J.; Bell, Alexis T.; Head-Gordon, Martin ACS Catalysis, Vol. 8, Issue 2 https://doi.org/10.1021/acscatal.7b03477	journal	January 2018
Understanding the Roadmap for Electrochemical Reduction of CO ₂ to Multi-Carbon Oxygenates and Hydrocarbons on Copper-Based Catalysts Zheng, Yao; Vasileff, Anthony; Zhou, Xianlong Journal of the American Chemical Society, Vol. 141, Issue 19 https://doi.org/10.1021/jacs.9b02124	journal	April 2019
General Techno-Economic Analysis of CO ₂ Electrolysis Systems Jouny, Matthew; Luc, Wesley; Jiao, Feng Industrial & Engineering Chemistry Research, Vol. 57, Issue 6 https://doi.org/10.1021/acs.iecr.7b03514	journal	February 2018
A comprehensive mechanism for the Fischer-Tropsch synthesis Rofer-DePoorter, Cheryl K. Chemical Reviews, Vol. 81, Issue 5 https://doi.org/10.1021/cr00045a002	journal	October 1981
Graphite-Conjugated Pyrazines as Molecularly Tunable Heterogeneous Electrocatalysts Fukushima, Tomohiro; Drisdell, Walter; Yano, Junko Journal of the American Chemical Society, Vol. 137, Issue 34 https://doi.org/10.1021/jacs.5b06737	journal	August 2015
A Local Proton Source Enhances CO ₂ Electroreduction to CO by a Molecular Fe Catalyst Costentin, Cyrille; Drouet, Samuel; Robert, Marc Science, Vol. 338, Issue 6103 https://doi.org/10.1126/science.1224581	journal	October 2012
Redox-inactive metal ions modulate the reactivity and oxygen release of mononuclear non-haem iron(III)–peroxo complexes Bang, Suhee; Lee, Yong-Min; Hong, Seungwoo Nature Chemistry, Vol. 6, Issue 10 https://doi.org/10.1038/nchem.2055	journal	September 2014
Understanding Immobilized Molecular Catalysts for Fuel-Forming Reactions through UV/Vis Spectroelectrochemistry Rosser, Timothy E.; Reisner, Erwin ACS Catalysis, Vol. 7, Issue 5 https://doi.org/10.1021/acscatal.7b00326	journal	March 2017
Splitting CO2 into CO and O2 by a single catalyst Chen, Z.; Concepcion, J. J.; Brennaman, M. K. Proceedings of the National Academy of Sciences, Vol. 109, Issue 39 https://doi.org/10.1073/pnas.1203122109	journal	June 2012
Mechanistic Contrasts between Manganese and Rhenium Bipyridine Electrocatalysts for the Reduction of Carbon Dioxide Riplinger, Christoph; Sampson, Matthew D.; Ritzmann, Andrew M. Journal of the American Chemical Society, Vol. 136, Issue 46 https://doi.org/10.1021/ja508192y	journal	November 2014
Catalysis of the Electrochemical Reduction of Carbon Dioxide by Iron(0) Porphyrins: Synergystic Effect of Weak Brönsted Acids Bhugun, Iqbal; Lexa, Doris; Savéant, Jean-Michel Journal of the American Chemical Society, Vol. 118, Issue 7 https://doi.org/10.1021/ja9534462	journal	January 1996
Noncovalent Immobilization of a Molecular Iron-Based Electrocatalyst on Carbon Electrodes for Selective, Efficient CO ₂ -to-CO Conversion in Water Maurin, Antoine; Robert, Marc Journal of the American Chemical Society, Vol. 138, Issue 8 https://doi.org/10.1021/jacs.5b12652	journal	February 2016
Electrons, Photons, Protons and Earth-Abundant Metal Complexes for Molecular Catalysis of CO ₂ Reduction Takeda, Hiroyuki; Cometto, Claudio; Ishitani, Osamu ACS Catalysis, Vol. 7, Issue 1 https://doi.org/10.1021/acscatal.6b02181	journal	November 2016
Covalent Attachment of Catalyst Molecules to Conductive Diamond: CO ₂ Reduction Using “Smart” Electrodes Yao, Shu A.; Ruther, Rose E.; Zhang, Linghong Journal of the American Chemical Society, Vol. 134, Issue 38 https://doi.org/10.1021/ja304783j	journal	September 2012
Homogeneous Catalysis--New Approaches to Catalyst Separation, Recovery, and Recycling Cole-Hamilton, David J. Science, Vol. 299, Issue 5613, p. 1702-1706 https://doi.org/10.1126/science.1081881	journal	March 2003
Activity boost of a biomimetic oxidation catalyst by immobilization onto a gold surface Berner, S.; Biela, S.; Ledung, G. Journal of Catalysis, Vol. 244, Issue 1 https://doi.org/10.1016/j.jcat.2006.08.017	journal	November 2006
Electrochemical CO2 reduction: Electrocatalyst, reaction mechanism, and process engineering Lu, Qi; Jiao, Feng Nano Energy, Vol. 29 https://doi.org/10.1016/j.nanoen.2016.04.009	journal	November 2016
Fundamentals and Challenges of Electrochemical CO2 Reduction Using Two-Dimensional Materials Sun, Zhenyu; Ma, Tao; Tao, Hengcong Chem, Vol. 3, Issue 4 https://doi.org/10.1016/j.chempr.2017.09.009	journal	October 2017
Distinguishing Homogeneous from Heterogeneous Catalysis in Electrode-Driven Water Oxidation with Molecular Iridium Complexes Schley, Nathan D.; Blakemore, James D.; Subbaiyan, Navaneetha K. Journal of the American Chemical Society, Vol. 133, Issue 27 https://doi.org/10.1021/ja2004522	journal	July 2011
Covalent Immobilization of a Molecular Catalyst on Cu ₂ O Photocathodes for CO ₂ Reduction Schreier, Marcel; Luo, Jingshan; Gao, Peng Journal of the American Chemical Society, Vol. 138, Issue 6 https://doi.org/10.1021/jacs.5b12157	journal	February 2016
Photoelectrochemical CO ₂ reduction using a Ru( ii )–Re( i ) multinuclear metal complex on a p-type semiconducting NiO electrode Sahara, Go; Abe, Ryu; Higashi, Masanobu Chemical Communications, Vol. 51, Issue 53 https://doi.org/10.1039/C5CC02403J	journal	January 2015
Noncovalent Immobilization of Electrocatalysts on Carbon Electrodes for Fuel Production Blakemore, James D.; Gupta, Ayush; Warren, Jeffrey J. Journal of the American Chemical Society, Vol. 135, Issue 49 https://doi.org/10.1021/ja4099609	journal	November 2013
Heterogeneous Electrocatalyst with Molecular Cobalt Ions Serving as the Center of Active Sites Wang, Jiong; Ge, Xiaoming; Liu, Zhaolin Journal of the American Chemical Society, Vol. 139, Issue 5 https://doi.org/10.1021/jacs.6b10307	journal	January 2017
A Water-Soluble Cu Complex as Molecular Catalyst for Electrocatalytic CO ₂ Reduction on Graphene-Based Electrodes Wang, Jiong; Gan, Liyong; Zhang, Qianwen Advanced Energy Materials, Vol. 9, Issue 3 https://doi.org/10.1002/aenm.201803151	journal	November 2018
Strong Electronic Coupling of Molecular Sites to Graphitic Electrodes via Pyrazine Conjugation Jackson, Megan N.; Oh, Seokjoon; Kaminsky, Corey J. Journal of the American Chemical Society, Vol. 140, Issue 3 https://doi.org/10.1021/jacs.7b10723	journal	January 2018
Highly selective and active CO2 reduction electrocatalysts based on cobalt phthalocyanine/carbon nanotube hybrid structures Zhang, Xing; Wu, Zishan; Zhang, Xiao Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/ncomms14675	journal	March 2017
Bioinspired catalytic materials for energy-relevant conversions Artero, Vincent Nature Energy, Vol. 2, Issue 9 https://doi.org/10.1038/nenergy.2017.131	journal	August 2017
Catalytic reduction of carbon dioxide at carbon electrodes modified with cobalt phthalocyanine Lieber, Charles M.; Lewis, Nathan S. Journal of the American Chemical Society, Vol. 106, Issue 17 https://doi.org/10.1021/ja00329a082	journal	August 1984
Covalent organic frameworks comprising cobalt porphyrins for catalytic CO ₂ reduction in water Lin, Song; Diercks, Christian S.; Zhang, Yue-Biao Science, Vol. 349, Issue 6253 https://doi.org/10.1126/science.aac8343	journal	August 2015
Metal–Organic Frameworks for Electrocatalytic Reduction of Carbon Dioxide Kornienko, Nikolay; Zhao, Yingbo; Kley, Christopher S. Journal of the American Chemical Society, Vol. 137, Issue 44 https://doi.org/10.1021/jacs.5b08212	journal	October 2015
Selective CO ₂ Conversion to Formate Conjugated with H ₂ O Oxidation Utilizing Semiconductor/Complex Hybrid Photocatalysts Sato, Shunsuke; Arai, Takeo; Morikawa, Takeshi Journal of the American Chemical Society, Vol. 133, Issue 39 https://doi.org/10.1021/ja204881d	journal	October 2011
Electrochemical CO ₂ Reduction to Hydrocarbons on a Heterogeneous Molecular Cu Catalyst in Aqueous Solution Weng, Zhe; Jiang, Jianbing; Wu, Yueshen Journal of the American Chemical Society, Vol. 138, Issue 26 https://doi.org/10.1021/jacs.6b04746	journal	June 2016
Selective electroacatalysis for CO2 reduction in the aqueous phase using cobalt phthalocyanine/poly-4-vinylpyridine modified electrodes Yoshida, Tsukasa; Kamato, Kazuhiro; Tsukamoto, Masaaki Journal of Electroanalytical Chemistry, Vol. 385, Issue 2 https://doi.org/10.1016/0022-0728(94)03762-R	journal	April 1995
Factors affecting selective electrocatalytic co2 reduction with cobalt phthalocyanine incorporated in a polyvinylpyridine membrane coated on a graphite electrode Abe, Toshiyuki; Yoshida, Tsukasa; Tokita, Sumio Journal of Electroanalytical Chemistry, Vol. 412, Issue 1-2 https://doi.org/10.1016/0022-0728(96)04631-1	journal	August 1996
Elucidating the Reactivity and Mechanism of CO ₂ Electroreduction at Highly Dispersed Cobalt Phthalocyanine Zhu, Minghui; Ye, Ruquan; Jin, Kyoungsuk ACS Energy Letters, Vol. 3, Issue 6 https://doi.org/10.1021/acsenergylett.8b00519	journal	May 2018
The Surface Trans Effect: Influence of Axial Ligands on the Surface Chemical Bonds of Adsorbed Metalloporphyrins Hieringer, Wolfgang; Flechtner, Ken; Kretschmann, Andreas Journal of the American Chemical Society, Vol. 133, Issue 16 https://doi.org/10.1021/ja1093502	journal	April 2011
Electrochemistry of redox-active self-assembled monolayers Eckermann, Amanda L.; Feld, Daniel J.; Shaw, Justine A. Coordination Chemistry Reviews, Vol. 254, Issue 15-16 https://doi.org/10.1016/j.ccr.2009.12.023	journal	August 2010
Hopping versus Tunneling Mechanism for Long-Range Electron Transfer in Porphyrin Oligomer Bridged Donor–Acceptor Systems Gilbert Gatty, Mélina; Kahnt, Axel; Esdaile, Louisa J. The Journal of Physical Chemistry B, Vol. 119, Issue 24 https://doi.org/10.1021/jp5115064	journal	December 2014
Advanced Carbon Electrode Materials for Molecular Electrochemistry McCreery, Richard L. Chemical Reviews, Vol. 108, Issue 7, p. 2646-2687 https://doi.org/10.1021/cr068076m	journal	July 2008
The Potential of Perylene Bisimide Derivatives for the Solubilization of Carbon Nanotubes and Graphene Backes, Claudia; Hauke, Frank; Hirsch, Andreas Advanced Materials, Vol. 23, Issue 22-23 https://doi.org/10.1002/adma.201100300	journal	April 2011
Polymer coordination promotes selective CO ₂ reduction by cobalt phthalocyanine Kramer, W. W.; McCrory, C. C. L. Chemical Science, Vol. 7, Issue 4 https://doi.org/10.1039/C5SC04015A	journal	January 2016
Modulating the mechanism of electrocatalytic CO2 reduction by cobalt phthalocyanine through polymer coordination and encapsulation Liu, Yingshuo; McCrory, Charles C. L. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-09626-8	journal	April 2019
Molecular Spectroscopy by Means of ESCA II. Sulfur compounds. Correlation of electron binding energy with structure Lindberg, B. J.; Hamrin, K.; Johansson, G. Physica Scripta, Vol. 1, Issue 5-6 https://doi.org/10.1088/0031-8949/1/5-6/020	journal	May 1970
Nitrogen-Doped Graphene Sheets Grown by Chemical Vapor Deposition: Synthesis and Influence of Nitrogen Impurities on Carrier Transport Lu, Yu-Fen; Lo, Shun-Tsung; Lin, Jheng-Cyuan ACS Nano, Vol. 7, Issue 8 https://doi.org/10.1021/nn402102y	journal	July 2013
Tuning the Acid/Base Properties of Nanocarbons by Functionalization via Amination Arrigo, Rosa; Hävecker, Michael; Wrabetz, Sabine Journal of the American Chemical Society, Vol. 132, Issue 28 https://doi.org/10.1021/ja910169v	journal	July 2010
Redox transitions of chromium, manganese, iron, cobalt and nickel protoporphyrins in aqueous solution de Groot, Matheus T.; Koper, Marc T. M. Phys. Chem. Chem. Phys., Vol. 10, Issue 7 https://doi.org/10.1039/B714727A	journal	January 2008
Redox potential and electrocatalysis of O2 reduction on transition metal chelates van der Putten, A.; Elzing, A.; Visscher, W. Journal of Electroanalytical Chemistry and Interfacial Electrochemistry, Vol. 221, Issue 1-2 https://doi.org/10.1016/0022-0728(87)80248-6	journal	April 1987
The use of linear potential sweep voltammetry and of a.c. voltammetry for the study of the surface electrochemical reaction of strongly adsorbed systems and of redox modified electrodes Laviron, E. Journal of Electroanalytical Chemistry and Interfacial Electrochemistry, Vol. 100, Issue 1-2 https://doi.org/10.1016/S0022-0728(79)80167-9	journal	June 1979
Understanding the Difference between Inner- and Outer-Sphere Mechanisms: An Electrochemical Experiment Torres, Luz María; Gil, Adrián F.; Galicia, Laura Journal of Chemical Education, Vol. 73, Issue 8 https://doi.org/10.1021/ed073p808	journal	August 1996
Electron transfer kinetics on composite diamond (sp3)–graphite (sp2) electrodes Duo, I.; Fujishima, A.; Comninellis, Ch Electrochemistry Communications, Vol. 5, Issue 8 https://doi.org/10.1016/S1388-2481(03)00169-3	journal	August 2003
Voltammetry at graphite electrodes: The oxidation of hexacyanoferrate (II) (ferrocyanide) does not exhibit pure outer-sphere electron transfer kinetics and is sensitive to pre-exposure of the electrode to organic solvents Xiong, Linhongjia; Batchelor-McAuley, Christopher; Ward, Kristopher R. Journal of Electroanalytical Chemistry, Vol. 661, Issue 1 https://doi.org/10.1016/j.jelechem.2011.07.028	journal	October 2011

Similar Records

Synergistic Effect of Diatomic Mo-B Site Confined in Graphene-Like C₂N Enables Electrocatalytic Nitrogen Reduction via Novel Mechanism

Journal Article · 2022 · Journal of Chemical Physics · OSTI ID:1897685

Li, Yang; An, Wei

Related Subjects

99 GENERAL AND MISCELLANEOUS

Linkage Effect in the Heterogenization of Cobalt Complexes by Doped Graphene for Electrocatalytic CO2 Reduction

Citation Formats

References (56)

Similar Records

Related Subjects