skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Molecular beam epitaxy of the magnetic Kagome metal FeSn on LaAlO3 (111)

Journal Article · · AIP Advances
DOI:https://doi.org/10.1063/5.0001909· OSTI ID:1671751
 [1];  [1];  [2];  [3];  [1];  [2]; ORCiD logo [1]
  1. Argonne National Lab. (ANL), Argonne, IL (United States)
  2. Univ. of Illinois at Urbana-Champaign, IL (United States)
  3. Argonne National Lab. (ANL), Argonne, IL (United States). Center for Nanoscale Materials

Materials with Kagome layers are expected to give rise to rich physics arising from band structures with topological properties, spin liquid behavior, and the formation of Skyrmions. Until now, most work on Kagome materials has been performed on bulk samples due to difficulties in thin film synthesis. Here, by using molecular beam epitaxy, layered Kagome-structured FeSn films are synthesized on the (111) oriented LaAlO3 substrate. Both in situ and ex situ characterizations indicate that these films are highly crystalline and c-axis oriented, with atomically smooth surfaces. The films grow as disconnected islands, with lateral dimensions on the micron meter scale. By patterning Pt electrodes using a focused electron beam, the longitudinal and transverse resistance of single islands have been measured in magnetic fields. Our work opens a pathway for exploring mesoscale transport properties in thin films of Kagome materials and related devices.

Research Organization:
Argonne National Lab. (ANL), Argonne, IL (United States). Center for Nanoscale Materials; Energy Frontier Research Centers (EFRC) (United States). Center for the Advancement of Topological Semimetals (CATS)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-06CH11357
OSTI ID:
1671751
Alternate ID(s):
OSTI ID: 1671848
Journal Information:
AIP Advances, Vol. 10, Issue 10; ISSN 2158-3226
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English

References (18)

Evidence for magnetic Weyl fermions in a correlated metal journal September 2017
Unconventional superconductivity in magic-angle graphene superlattices journal March 2018
Large anomalous Hall effect in a non-collinear antiferromagnet at room temperature journal October 2015
Gate-tunable negative longitudinal magnetoresistance in the predicted type-II Weyl semimetal WTe2 journal October 2016
Electronics and optoelectronics of two-dimensional transition metal dichalcogenides journal November 2012
Epitaxial growth of ultraflat stanene with topological band inversion journal November 2018
Observation of a three-dimensional topological Dirac semimetal phase in high-mobility Cd3As2 journal May 2014
Massive Dirac fermions in a ferromagnetic kagome metal journal March 2018
Epitaxial growth of Bi 2 Se 3 topological insulator thin films on Si (111) journal May 2011
Large anomalous Hall effect driven by a nonvanishing Berry curvature in the noncolinear antiferromagnet Mn 3 Ge journal April 2016
Dirac fermions and flat bands in the ideal kagome metal FeSn journal December 2019
Correlated insulator behaviour at half-filling in magic-angle graphene superlattices journal March 2018
Observation of Various and Spontaneous Magnetic Skyrmionic Bubbles at Room Temperature in a Frustrated Kagome Magnet with Uniaxial Magnetic Anisotropy journal June 2017
Topological metal at the surface of an ultrathin Bi 1 x Sb x alloy film journal April 2010
Topological Insulator Thin Films of Bi2Te3 with Controlled Electronic Structure journal May 2011
Topological Weyl semimetals in the chiral antiferromagnetic materials Mn 3 Ge and Mn 3 Sn journal January 2017
Molecular beam epitaxy growth of antiferromagnetic Kagome metal FeSn journal August 2019
Giant and anisotropic many-body spin–orbit tunability in a strongly correlated kagome magnet journal September 2018

Similar Records

Giant Periodic Pseudomagnetic Fields in Strained Kagome Magnet FeSn Epitaxial Films on SrTiO 3 (111) Substrate
Journal Article · Mon Mar 13 00:00:00 EDT 2023 · Nano Letters · OSTI ID:1671751

Visualizing symmetry-breaking electronic orders in epitaxial Kagome magnet FeSn films
Journal Article · Wed Oct 04 00:00:00 EDT 2023 · Nature Communications · OSTI ID:1671751

Atomic layer epitaxy of kagome magnet Fe3Sn2 and Sn-modulated heterostructures
Journal Article · Fri Jun 24 00:00:00 EDT 2022 · APL Materials · OSTI ID:1671751