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Title: In situ X-ray spatial profiling reveals uneven compression of electrode assemblies and steep lateral gradients in lithium-ion coin cells

Abstract

In situ X-ray diffraction profilometry reveals radially nonuniform compression of the electrode assembly leading to large lateral heterogeneity of lithium intercalation and plating in the standard Li-ion coin cells in fast charge regimes.

Authors:
ORCiD logo [1]; ORCiD logo [2];  [1]; ORCiD logo [2]; ORCiD logo [3]; ORCiD logo [2]; ORCiD logo [2]
  1. X-ray Science Division, Advanced Photon Source, Argonne National Laboratory, Lemont, USA
  2. Chemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, USA
  3. Chemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, USA, Department of Electrical Engineering
Publication Date:
Sponsoring Org.:
USDOE Office of Science (SC), Workforce Development for Teachers and Scientists (WDTS); USDOE Office of Energy Efficiency and Renewable Energy (EERE), Transportation Office. Vehicle Technologies Office
OSTI Identifier:
1665906
Grant/Contract Number:  
AC02-06CH11357; SC0014664
Resource Type:
Journal Article: Publisher's Accepted Manuscript
Journal Name:
Physical Chemistry Chemical Physics. PCCP (Print)
Additional Journal Information:
Journal Name: Physical Chemistry Chemical Physics. PCCP (Print) Journal Volume: 22 Journal Issue: 38; Journal ID: ISSN 1463-9076
Publisher:
Royal Society of Chemistry (RSC)
Country of Publication:
United Kingdom
Language:
English

Citation Formats

Okasinski, John S., Shkrob, Ilya A., Chuang, Andrew, Rodrigues, Marco-Tulio Fonseca, Raj, Abhi, Dees, Dennis W., and Abraham, Daniel P. In situ X-ray spatial profiling reveals uneven compression of electrode assemblies and steep lateral gradients in lithium-ion coin cells. United Kingdom: N. p., 2020. Web. doi:10.1039/D0CP04436A.
Okasinski, John S., Shkrob, Ilya A., Chuang, Andrew, Rodrigues, Marco-Tulio Fonseca, Raj, Abhi, Dees, Dennis W., & Abraham, Daniel P. In situ X-ray spatial profiling reveals uneven compression of electrode assemblies and steep lateral gradients in lithium-ion coin cells. United Kingdom. doi:10.1039/D0CP04436A.
Okasinski, John S., Shkrob, Ilya A., Chuang, Andrew, Rodrigues, Marco-Tulio Fonseca, Raj, Abhi, Dees, Dennis W., and Abraham, Daniel P. Wed . "In situ X-ray spatial profiling reveals uneven compression of electrode assemblies and steep lateral gradients in lithium-ion coin cells". United Kingdom. doi:10.1039/D0CP04436A.
@article{osti_1665906,
title = {In situ X-ray spatial profiling reveals uneven compression of electrode assemblies and steep lateral gradients in lithium-ion coin cells},
author = {Okasinski, John S. and Shkrob, Ilya A. and Chuang, Andrew and Rodrigues, Marco-Tulio Fonseca and Raj, Abhi and Dees, Dennis W. and Abraham, Daniel P.},
abstractNote = {In situ X-ray diffraction profilometry reveals radially nonuniform compression of the electrode assembly leading to large lateral heterogeneity of lithium intercalation and plating in the standard Li-ion coin cells in fast charge regimes.},
doi = {10.1039/D0CP04436A},
journal = {Physical Chemistry Chemical Physics. PCCP (Print)},
issn = {1463-9076},
number = 38,
volume = 22,
place = {United Kingdom},
year = {2020},
month = {10}
}

Journal Article:
Free Publicly Available Full Text
This content will become publicly available on September 15, 2021
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