Phase control of coherent acoustic phonons in gold bipyramids for optical memory and manipulating plasmon–exciton coupling

Kirschner, Matthew S.; Lin, Xiao-Min; Chen, Lin X.; Schaller, Richard D.

doi:10.1063/5.0004209

Title: Phase control of coherent acoustic phonons in gold bipyramids for optical memory and manipulating plasmon–exciton coupling

Journal Article · Mon Apr 13 00:00:00 EDT 2020 · Applied Physics Letters

DOI:https://doi.org/10.1063/5.0004209· OSTI ID:1632826

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Northwestern Univ., Evanston, IL (United States)
Argonne National Lab. (ANL), Lemont, IL (United States). Center for Nanoscale Materials
Northwestern Univ., Evanston, IL (United States); Argonne National Lab. (ANL), Lemont, IL (United States). Center for Nanoscale Materials

Recent efforts have targeted manipulation of nanomaterial vibrational modes in applications such as chemical/mass sensing, optical switching, and phonon-driven photochemistry. While impulsive photoexcitation can generate coherent phonons, multiple excitation pulses offer the prospect of control and manipulation of coherent phonon modes for functions of optical memory and logic. In this work, we use such an approach to inject an arbitrary coherent phonon phase into a colloidal ensemble of highly monodisperse gold bipyramids. We then demonstrate that this technique can be applied to a system that exhibits plasmon-exciton coupling to further manipulate the hybridization of the system. This ability to manipulate acoustic phonons and hybridization can enable optical logic applications of acoustic phonons in addition to optical memory.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States). Center for Nanoscale Materials (CNM)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1632826

Alternate ID(s):: OSTI ID: 1632961

Journal Information:: Applied Physics Letters, Vol. 116, Issue 15; ISSN 0003-6951

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 1 work

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Title: Phase control of coherent acoustic phonons in gold bipyramids for optical memory and manipulating plasmon–exciton coupling

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