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Title: Enabling high repetition rate nonlinear THz science with a kilowatt-class sub-100 fs laser source

Journal Article · · Optics Express
DOI:https://doi.org/10.1364/oe.389653· OSTI ID:1630379

Manipulating the atomic and electronic structure of matter with strong terahertz (THz) fields while probing the response with ultrafast pulses at x-ray free electron lasers (FELs) has offered unique insights into a multitude of physical phenomena in solid state and atomic physics. Recent upgrades of x-ray FEL facilities are pushing to much higher repetition rates, enabling unprecedented signal-to-noise ratio for pump probe experiments. This requires the development of suitable THz pump sources that are able to deliver intense pulses at compatible repetition rates. Here we present a high-power laser-driven THz source based on optical rectification in LiNbO3 using tilted pulse front pumping. Our source is driven by a kilowatt-level Yb:YAG amplifier system operating at 100 kHz repetition rate and employing nonlinear spectral broadening and recompression to achieve sub-100 fs pulses with pulse energies up to 7 mJ that are necessary for high THz conversion efficiency and peak field strength. We demonstrate a maximum of 144 mW average THz power (1.44 μJ pulse energy), consisting of single-cycle pulses centered at 0.6 THz with a peak electric field strength exceeding 150 kV/cm. These high field pulses open up a range of possibilities for nonlinear time-resolved THz experiments at unprecedented rates.

Research Organization:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States). Linac Coherent Light Source (LCLS)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-76SF00515; 2015-SLAC-100238
OSTI ID:
1630379
Alternate ID(s):
OSTI ID: 1647638
Journal Information:
Optics Express, Journal Name: Optics Express Vol. 28 Journal Issue: 11; ISSN 1094-4087
Publisher:
Optical Society of America (OSA)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 32 works
Citation information provided by
Web of Science

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