Anisotropic ultraviolet-plasmon dispersion in black phosphorus

Nicotra, Giuseppe; van Veen, Edo; Deretzis, Ioannis; Wang, Lin; Hu, Jin; Mao, Zhiqiang; Fabio, Vito; Spinella, Corrado; Chiarello, Gennaro; Rudenko, Alexander; Yuan, Shengjun; Politano, Antonio

doi:10.1039/c8nr05502e

Title: Anisotropic ultraviolet-plasmon dispersion in black phosphorus

Journal Article · Mon Nov 12 00:00:00 EST 2018 · Nanoscale

DOI:https://doi.org/10.1039/c8nr05502e· OSTI ID:1612107

Nicotra, Giuseppe ^[1]; van Veen, Edo ^[2];

^[1]; Wang, Lin ^[3]; Hu, Jin ^[4]; Mao, Zhiqiang ^[5]; Fabio, Vito ^[6]; Spinella, Corrado ^[1]; Chiarello, Gennaro ^[6]; Rudenko, Alexander ^[2]; Yuan, Shengjun ^[2];

^[7]

Consiglio Nazionale delle Ricerche (CNR), Catania (Italy). Istituto per la Microelettronica e Microsistemi (IMM)
Wuhan Univ. (China); Radboud Univ., Nijmegen (Netherlands)
Chinese Academy of Sciences (CAS), Shanghai (China). State Key Laboratory of Infrared Physics, ;Institute of Technical Physics; Univ. of Science and Technology of China, Hefei (China)
Univ. of Arkansas, Fayetteville, AR (United States)
Tulane Univ., New Orleans, LA (United States)
University of Calabria (Italy)
Graphene Labs, Genova (Italy); University of L'Aquila (Italy)

Via momentum-resolved electron energy loss spectroscopy (EELS) coupled with scanning transmission electron microscopy, we have studied the dispersion relation of interband plasmonic modes in the ultraviolet in black phosphorus. We find that the dispersion of the interband plasmons is anisotropic. Experimental results are reproduced by density functional theory, by taking into account both the anisotropy of the single-particle response function, arising from the anisotropic band structure, and the damping. Moreover, our theoretical model also indicates the presence of low-energy excitations in the near-infrared that are selectively active in the armchair direction, whose existence has been experimentally validated by high-resolution EELS (HREELS) in reflection mode.

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Research Organization:: Tulane Univ., New Orleans, LA (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: SC0014208

OSTI ID:: 1612107

Alternate ID(s):: OSTI ID: 1483008

Journal Information:: Nanoscale, Vol. 10, Issue 46; ISSN 2040-3364

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 16 works

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Energy loss spectrum and surface modes of two-dimensional black phosphorus Xu, Peng; Zheng, Dingguo; Zhu, Chunhui Journal of Physics: Materials, Vol. 2, Issue 4 https://doi.org/10.1088/2515-7639/ab27e9	journal	July 2019
The Optical Properties and Plasmonics of Anisotropic 2D Materials Wang, Chong; Zhang, Guowei; Huang, Shenyang Advanced Optical Materials, Vol. 8, Issue 5 https://doi.org/10.1002/adom.201900996	journal	September 2019
Rapid exfoliation for few-layer enriched black phosphorus dispersion via a superhydrophobic silicon-nanowire-embedded microfluidic process Choi, Chang-Ho; Ko, Dong-Hyeon; Jun, Ho Young Green Chemistry, Vol. 22, Issue 3 https://doi.org/10.1039/c9gc02337b	journal	January 2020
Effect of mechanical strain on the optical properties of nodal-line semimetal ZrSiS Zhou, Weiqing; Rudenko, A. N.; Yuan, Shengjun arXiv https://doi.org/10.48550/arxiv.1908.08789	text	January 2019
Momentum-Resolved Dielectric Response of Free-Standing Mono-, Bi-, and Trilayer Black Phosphorus Gaufrès, Etienne; Fossard, Frédéric; Gosselin, Vincent Nano Letters, Vol. 19, Issue 11 https://doi.org/10.1021/acs.nanolett.9b03928	journal	September 2019

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