Probing many-body interactions in monolayer transition-metal dichalcogenides

Van Tuan, Dinh; Scharf, Benedikt; Wang, Zefang; Shan, Jie; Mak, Kin Fai; Žutić, Igor; Dery, Hanan

doi:10.1103/physrevb.99.085301

Title: Probing many-body interactions in monolayer transition-metal dichalcogenides

Journal Article · Fri Feb 01 00:00:00 EST 2019 · Physical Review B

DOI:https://doi.org/10.1103/physrevb.99.085301· OSTI ID:1610763

Van Tuan, Dinh ^[1]; Scharf, Benedikt ^[2]; Wang, Zefang ^[3]; Shan, Jie ^[3]; Mak, Kin Fai ^[3]; Žutić, Igor ^[4]; Dery, Hanan ^[1]

Univ. of Rochester, NY (United States)
State Univ. of New York (SUNY), Buffalo, NY (United States); Univ. of Regensburg (Germany); Univ. of Wurzburg (Germany)
Pennsylvania State Univ., University Park, PA (United States)
State Univ. of New York (SUNY), Buffalo, NY (United States)

Many-body interactions in monolayer transition-metal dichalcogenides are strongly affected by their unique band structure. We study these interactions by measuring the energy shift of neutral excitons (bound electron-hole pairs) in gated WSe₂ and MoSe₂. Surprisingly, while the blueshift of the neutral exciton X⁰ in electron-doped samples can be more than 10 meV, the blueshift in hole-doped samples is nearly absent. Taking into account dynamical screening and local-field effects, we present a transparent and analytical model that elucidates the crucial role played by intervalley plasmons in electron-doped conditions. Here, the energy shift of X⁰ as a function of charge density is computed showing agreement with experiment, where the renormalization of X⁰ by intervalley plasmons yields a stronger blueshift in MoSe₂ than in WSe₂ due to differences in their band ordering.

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Research Organization:: State Univ. of New York (SUNY), Albany, NY (United States); Univ. of South Florida, Tampa, FL (United States); Pennsylvania State Univ., University Park, PA (United States); Univ. of Rochester, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)

Grant/Contract Number:: SC0004890; SC0012635; SC0013883; SC0014349; DMR-1410407; DESC0013883

OSTI ID:: 1610763

Alternate ID(s):: OSTI ID: 1493105

Journal Information:: Physical Review B, Vol. 99, Issue 8; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 52 works

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Dynamical screening in monolayer transition-metal dichalcogenides and its manifestations in the exciton spectrum Scharf, Benedikt; Van Tuan, Dinh; Žutić, Igor Journal of Physics: Condensed Matter, Vol. 31, Issue 20 https://doi.org/10.1088/1361-648x/ab071f	journal	March 2019
Nonlinear excitonic spin Hall effect in monolayer transition metal dichalcogenides Taghizadeh, A.; Pedersen, T. G. 2D Materials, Vol. 7, Issue 1 https://doi.org/10.1088/2053-1583/ab4171	journal	October 2019
Magnetic field mixing and splitting of bright and dark excitons in monolayer MoSe ₂ Lu, Zhengguang; Rhodes, Daniel; Li, Zhipeng 2D Materials, Vol. 7, Issue 1 https://doi.org/10.1088/2053-1583/ab5614	journal	November 2019
Exciton states and absorption spectra in freestanding monolayer transition metal dichalcogenides: A variationally optimized diagonalization method Wu, Shudong; Cheng, Liwen; Wang, Qiang Physical Review B, Vol. 100, Issue 11 https://doi.org/10.1103/physrevb.100.115430	journal	September 2019
Multiphonon Raman scattering mediated by the exciton states in monolayer transition metal chalcogenides Wang, Zi-Wu; Xiao, Yao; Deng, Jia-Pei Physical Review B, Vol. 100, Issue 12 https://doi.org/10.1103/physrevb.100.125308	journal	September 2019
Excited-State Trions in Monolayer ${WS}_{2}$ Arora, Ashish; Deilmann, Thorsten; Reichenauer, Till Physical Review Letters, Vol. 123, Issue 16 https://doi.org/10.1103/PhysRevLett.123.167401	journal	October 2019
Coherent feedback control of two-dimensional excitons Rogers, Christopher; Gray, Dodd; Bogdanowicz, Nathan Physical Review Research, Vol. 2, Issue 1 https://doi.org/10.1103/physrevresearch.2.012029	journal	January 2020
Dynamical screening in monolayer transition-metal dichalcogenides and its manifestations in the exciton spectrum Scharf, Benedikt; Van Tuan, Dinh; Žutić, Igor arXiv https://doi.org/10.48550/arxiv.1801.06217	text	January 2018
Nonlinear excitonic spin Hall effect in monolayer transition metal dichalcogenides Taghizadeh, Alireza; Pedersen, T. G. arXiv https://doi.org/10.48550/arxiv.1812.02596	preprint	January 2018

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