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Title: A Coupled Experimental and Simulation Approach to Investigate the Impact of Grain Growth, Amorphization, and Grain Subdivision in Accident Tolerant U3Si2 Light Water Reactor Fuel

Abstract

Triuranium disilicide (U3Si2) is being considered as an alternative accident tolerant fuel (ATF) due to its higher thermal conductivity. However, there is uncertainty in its use due to a lack of irradiation data at light water reactor (LWR) conditions. In this project, we used an integrated experimental and simulation approach to answer two significant questions pertaining to U3Si2 that were not investigated by the Fuel Cycle Research and Development (FCRD) and Nuclear Energy Advanced Modeling and Simulation (NEAMS) programs: (1) Will grain growth in the hotter portions of the fuel significantly impact U3Si2 LWR fuel behavior? (2) Under what conditions do grain subdivision and amorphization occur in U3Si2 and will either occur at LWR conditions? Our approach to answer these questions used in situ ion irradiation and annealing to investigate grain growth, grain subdivision, and amorphization, along with mesoscale simulations using the MARMOT tool. We found that while the grain boundary mobility of U3Si2 is larger than that of UO2, grain growth in U3Si2 fuel pellets will be less than in UO2 and may be neglected due to the lower thermal conductivity and thus lower centerline temperature. We also found that amorphization will not occur in U3Si2 above 600 K,more » such that it is not likely to occur at typical LWR operating conditions. Grain subdivision will occur at LWR conditions and will likely occur at lower burnups than in UO2.« less

Authors:
 [1]; ORCiD logo [2];  [3];  [4];  [5]
  1. Pennsylvania State Univ., University Park, PA (United States)
  2. Univ. of Florida, Gainesville, FL (United States)
  3. Rennselaer Polytechnic University, Troy, NY (United States)
  4. Univ. of Wisconsin, Madison, WI (United States)
  5. Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Publication Date:
Research Org.:
Pennsylvania State Univ., University Park, PA (United States)
Sponsoring Org.:
USDOE Office of Nuclear Energy (NE)
OSTI Identifier:
1607368
Report Number(s):
DOE-PSU-08564
16-10667; TRN: US2103848
DOE Contract Number:  
NE0008564
Resource Type:
Technical Report
Country of Publication:
United States
Language:
English
Subject:
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS; U3Si2; Grain growth; Grain Subdivision; Amorphization

Citation Formats

Walters, William, Tonks, Michael R., Lian, Jie, Zhang, Yongfeng, and Harp, Jason. A Coupled Experimental and Simulation Approach to Investigate the Impact of Grain Growth, Amorphization, and Grain Subdivision in Accident Tolerant U3Si2 Light Water Reactor Fuel. United States: N. p., 2020. Web. doi:10.2172/1607368.
Walters, William, Tonks, Michael R., Lian, Jie, Zhang, Yongfeng, & Harp, Jason. A Coupled Experimental and Simulation Approach to Investigate the Impact of Grain Growth, Amorphization, and Grain Subdivision in Accident Tolerant U3Si2 Light Water Reactor Fuel. United States. https://doi.org/10.2172/1607368
Walters, William, Tonks, Michael R., Lian, Jie, Zhang, Yongfeng, and Harp, Jason. 2020. "A Coupled Experimental and Simulation Approach to Investigate the Impact of Grain Growth, Amorphization, and Grain Subdivision in Accident Tolerant U3Si2 Light Water Reactor Fuel". United States. https://doi.org/10.2172/1607368. https://www.osti.gov/servlets/purl/1607368.
@article{osti_1607368,
title = {A Coupled Experimental and Simulation Approach to Investigate the Impact of Grain Growth, Amorphization, and Grain Subdivision in Accident Tolerant U3Si2 Light Water Reactor Fuel},
author = {Walters, William and Tonks, Michael R. and Lian, Jie and Zhang, Yongfeng and Harp, Jason},
abstractNote = {Triuranium disilicide (U3Si2) is being considered as an alternative accident tolerant fuel (ATF) due to its higher thermal conductivity. However, there is uncertainty in its use due to a lack of irradiation data at light water reactor (LWR) conditions. In this project, we used an integrated experimental and simulation approach to answer two significant questions pertaining to U3Si2 that were not investigated by the Fuel Cycle Research and Development (FCRD) and Nuclear Energy Advanced Modeling and Simulation (NEAMS) programs: (1) Will grain growth in the hotter portions of the fuel significantly impact U3Si2 LWR fuel behavior? (2) Under what conditions do grain subdivision and amorphization occur in U3Si2 and will either occur at LWR conditions? Our approach to answer these questions used in situ ion irradiation and annealing to investigate grain growth, grain subdivision, and amorphization, along with mesoscale simulations using the MARMOT tool. We found that while the grain boundary mobility of U3Si2 is larger than that of UO2, grain growth in U3Si2 fuel pellets will be less than in UO2 and may be neglected due to the lower thermal conductivity and thus lower centerline temperature. We also found that amorphization will not occur in U3Si2 above 600 K, such that it is not likely to occur at typical LWR operating conditions. Grain subdivision will occur at LWR conditions and will likely occur at lower burnups than in UO2.},
doi = {10.2172/1607368},
url = {https://www.osti.gov/biblio/1607368}, journal = {},
number = ,
volume = ,
place = {United States},
year = {Mon Mar 30 00:00:00 EDT 2020},
month = {Mon Mar 30 00:00:00 EDT 2020}
}