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Title: Air Dispersion Modeling of Radioactive Releases During Proposed 236Z Rubble Pile Removal Activities

Technical Report ·
DOI:https://doi.org/10.2172/1604169· OSTI ID:1604169

This report is part of the planning process for the removal of the 236Z rubble remaining as of January 1, 2018, at the Plutonium Finishing Plant (PFP) on the Hanford Site. This report documents an analysis considering standard techniques for the removal of demolition rubble. It does not document any decisions about the removal approaches. This document is intended to guide the establishment of a boundary for the application of an air monitoring regime. Atmospheric dispersion modeling using estimated release rates has been conducted to provide information on the location and levels of radioactive contamination that may be expected as the result of rubble removal activities. Hourly meteorological data collected over a 6-year period (2004–2009) were used to examine the effects of wind speed, direction, and stability on projected concentrations of contaminants in air and deposited on nearby surfaces. The source terms modeled in this report were based on the residual transuranic contamination levels that are anticipated to remain in the 236Z rubble following building demolition. The potential airborne concentrations were established using the five-factor formula from DOE-HDBK-3010 (DOE 1994) considering material-at-risk, damage ratio, airborne release fraction, respirable fraction, and leak path factor. Radioactive contamination emissions were calculated by release mechanism and rubble pile area for on-shift and off-shift activities. The emissions from the applicable sources were combined to provide emissions estimates for each day from each cleanup area. The U.S. Environmental Protection Agency’s (EPA’s) AERMOD computer code was used to estimate atmospheric dispersion and deposition of the released radioactive materials in the immediate vicinity of the planned rubble removal activities Both airborne and surface concentrations were modeled with AERMOD. Hourly derived air concentrations (DAC) were modeled for an array of receptors covering the rubble pile site and surrounding area. Peak (95th and 99th percentile) values of time-integrated air concentrations at these receptor points are derived from these hourly values, with modeling results reported as total incremental air concentrations in DAC-hours occurring over the selected time period. Total accumulated deposition amounts were also evaluated with AERMOD using the same array of receptors, with results reported as disintegrations per minute (dpm) per 100 cm2. Each rubble pile was considered in terms of its size, location, and estimated contamination levels. The modeling was based on the assumed sequence of the rubble removal activities. The results in this report are based on cleanup schedules and methods proposed by CHPRC. As of January 1, 2018, there are broadly three large rubble piles (west, footprint, and east) remaining of the 236Z Building process cell. It is assumed that the overall cleanup will require either 1) 30 days over a 6-week period, or 2) 60 days over a 12-week period. Work was assumed to be performed during 10-hour day shifts. The analysis shows that some releases of radioactive material are to be anticipated during the cleanup of the 236Z rubble piles. The modeling results presented here are closely tied to the details of how the rubble removal is to be conducted. The results indicate that for the rubble removal, the radiological exposures from the planned activities are predicted to be well below the designated limits for air and soil exposures. The cleanup of the 236Z main process cell rubble is expected to release some alpha-emitting radionuclides. However, results based on 6 years of hourly climatological data, two representative cleanup periods, realistic mitigating actions, and a bounding source term indicate that concentrations at the fence line of the PFP facilities should remain well below 12 DAC-hours/week. The results presented in this report are a reevaluation of a subset of the results presented in PNNL-20173 Rev. 4.

Research Organization:
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
AC05-76RL01830
OSTI ID:
1604169
Report Number(s):
PNNL-27464-Rev.1; TRN: US2103889
Country of Publication:
United States
Language:
English