Magnetic field-tuned Fermi liquid in a Kondo insulator

Kushwaha, Satya K.; Chan, Mun K.; Park, Joonbum; Thomas, S. M.; Bauer, Eric D.; Thompson, J. D.; Ronning, F.; Rosa, Priscila F. S.; Harrison, Neil

doi:10.1038/s41467-019-13421-w

Title: Magnetic field-tuned Fermi liquid in a Kondo insulator

Journal Article · Mon Dec 02 00:00:00 EST 2019 · Nature Communications

DOI:https://doi.org/10.1038/s41467-019-13421-w· OSTI ID:1619599

;

; Park, Joonbum;

;

; Thompson, J. D.; Ronning, F.; Rosa, Priscila F. S.; Harrison, Neil

Kondo insulators are expected to transform into metals under a sufficiently strong magnetic field. The closure of the insulating gap stems from the coupling of a magnetic field to the electron spin, yet the required strength of the magnetic field–typically of order 100 T–means that very little is known about this insulator-metal transition. Here we show that Ce₃Bi₄Pd₃, owing to its fortuitously small gap, provides an ideal Kondo insulator for this investigation. A metallic Fermi liquid state is established above a critical magnetic field of only B_c ≈ 11 T. A peak in the strength of electronic correlations near B_c, which is evident in transport and susceptibility measurements, suggests that Ce₃Bi₄Pd₃ may exhibit quantum criticality analogous to that reported in Kondo insulators under pressure. Metamagnetism and the breakdown of the Kondo coupling are also discussed.

View Journal Article

Cite

Export

Save

Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Laboratory Directed Research and Development (LDRD) Program; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; State of Florida

Grant/Contract Number:: 89233218CNA000001

OSTI ID:: 1619599

Alternate ID(s):: OSTI ID: 1603991; OSTI ID: 1779668

Report Number(s):: LA-UR-19-25216; LA-UR-19-25217; 5487; PII: 13421

Journal Information:: Nature Communications, Journal Name: Nature Communications Vol. 10 Journal Issue: 1; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United Kingdom

Language:: English

Citation Metrics:

Cited by: 14 works

Citation information provided by
Web of Science

References (53)

Closing the spin gap in the Kondo insulator Ce3Bi4Pt3 at high magnetic fields Jaime, Marcelo; Movshovich, Roman; Stewart, Gregory R. Nature, Vol. 405, Issue 6783 https://doi.org/10.1038/35012027	journal	May 2000
Topological Kondo Insulators Dzero, Maxim; Sun, Kai; Galitski, Victor Physical Review Letters, Vol. 104, Issue 10 https://doi.org/10.1103/PhysRevLett.104.106408	journal	March 2010
Hall effect in the doped Kondo insulator (Ce1−xLax)3Bi4Pt3 Pietrus, T.; Löhneysen, H. Von; Steinbach, B. Physica B: Condensed Matter, Vol. 281-282 https://doi.org/10.1016/S0921-4526(99)01231-4	journal	June 2000
Mixed valence properties of YbB12 Kasaya, M.; Iga, F.; Takigawa, M. Journal of Magnetism and Magnetic Materials, Vol. 47-48 https://doi.org/10.1016/0304-8853(85)90458-5	journal	February 1985
Magnetic-Field-Induced Kondo Metal Realized in ${YbB}_{12}$ Terashima, Taku T.; Matsuda, Yasuhiro H.; Kohama, Yoshimitsu Physical Review Letters, Vol. 120, Issue 25 https://doi.org/10.1103/PhysRevLett.120.257206	journal	June 2018
Two-dimensional Fermi surfaces in Kondo insulator SmB ₆ Li, G.; Xiang, Z.; Yu, F. Science, Vol. 346, Issue 6214 https://doi.org/10.1126/science.1250366	journal	December 2014
Low-temperature conducting state in two candidate topological Kondo insulators: ${SmB}_{6}$ and ${Ce}_{3} {Bi}_{4} {Pt}_{3}$ Wakeham, N.; Rosa, P. F. S.; Wang, Y. Q. Physical Review B, Vol. 94, Issue 3 https://doi.org/10.1103/PhysRevB.94.035127	journal	July 2016
Sm $B_{6}$ : Kondo Insulator or Exotic Metal? Cooley, J. C.; Aronson, M. C.; Fisk, Z. Physical Review Letters, Vol. 74, Issue 9 https://doi.org/10.1103/PhysRevLett.74.1629	journal	February 1995
Highly Asymmetric Nodal Semimetal in Bulk ${SmB}_{6}$ Harrison, N. Physical Review Letters, Vol. 121, Issue 2 https://doi.org/10.1103/PhysRevLett.121.026602	journal	July 2018
Quantum criticality Sachdev, Subir; Keimer, Bernhard Physics Today, Vol. 64, Issue 2 https://doi.org/10.1063/1.3554314	journal	February 2011
Unconventional Fermi surface in an insulating state Tan, B. S.; Hsu, Y. - T.; Zeng, B. Science, Vol. 349, Issue 6245 https://doi.org/10.1126/science.aaa7974	journal	July 2015
Magnetization of ${UBe}_{13}$ to 60 T Detwiler, J. A.; Schmiedeshoff, G. M.; Harrison, N. Physical Review B, Vol. 61, Issue 1 https://doi.org/10.1103/PhysRevB.61.402	journal	January 2000
Magnetic-field-driven metal-insulator transition in Kondo insulators de Oliveira, N. A.; Tovar Costa, Marcus V.; Troper, A. Physical Review B, Vol. 60, Issue 3 https://doi.org/10.1103/PhysRevB.60.1444	journal	July 1999
Antiferromagnetic Kondo lattice in the layered compound ${CePd}_{1 - x} {Bi}_{2}$ and comparison to the superconductor ${LaPd}_{1 - x} {Bi}_{2}$ Han, Fei; Wan, Xiangang; Phelan, Daniel Physical Review B, Vol. 92, Issue 4 https://doi.org/10.1103/PhysRevB.92.045112	journal	July 2015
SmB ₆ : A Promising Candidate for a Topological Insulator Takimoto, Tetsuya Journal of the Physical Society of Japan, Vol. 80, Issue 12 https://doi.org/10.1143/JPSJ.80.123710	journal	December 2011
Low-temperature surface conduction in the Kondo insulator SmB $_{6}$ Wolgast, Steven; Kurdak, Çağlıyan; Sun, Kai Physical Review B, Vol. 88, Issue 18 https://doi.org/10.1103/PhysRevB.88.180405	journal	November 2013
Pressure-induced Fermi-liquid behavior in the Kondo insulator ${SmB}_{6} :$ Possible transition through a quantum critical point Gabáni, S.; Bauer, E.; Berger, S. Physical Review B, Vol. 67, Issue 17 https://doi.org/10.1103/PhysRevB.67.172406	journal	May 2003
Kondo Insulator to Semimetal Transformation Tuned by Spin-Orbit Coupling Dzsaber, S.; Prochaska, L.; Sidorenko, A. Physical Review Letters, Vol. 118, Issue 24 https://doi.org/10.1103/PhysRevLett.118.246601	journal	June 2017
Volume magnetostriction of rare-earth metals with unstable 4f shells Zieglowski, J.; Hafner, H. U.; Wohlleben, D. Physical Review Letters, Vol. 56, Issue 2 https://doi.org/10.1103/PhysRevLett.56.193	journal	January 1986
Quantum phase transition and destruction of Kondo effect in pressurized SmB6 Zhou, Yazhou; Wu, Qi; Rosa, Priscila F. S. Science Bulletin, Vol. 62, Issue 21 https://doi.org/10.1016/j.scib.2017.10.008	journal	November 2017
Topological Kondo Insulators Dzero, Maxim; Xia, Jing; Galitski, Victor Annual Review of Condensed Matter Physics, Vol. 7, Issue 1 https://doi.org/10.1146/annurev-conmatphys-031214-014749	journal	March 2016
Quantum oscillations of electrical resistivity in an insulator Xiang, Z.; Kasahara, Y.; Asaba, T. Science, Vol. 362, Issue 6410 https://doi.org/10.1126/science.aap9607	journal	August 2018
Continuous Evolution of the Fermi Surface of ${CeRu}_{2} {Si}_{2}$ across the Metamagnetic Transition Daou, R.; Bergemann, C.; Julian, S. R. Physical Review Letters, Vol. 96, Issue 2 https://doi.org/10.1103/PhysRevLett.96.026401	journal	January 2006
Physical Properties of Sm $B_{6}$ Nickerson, J. C.; White, R. M.; Lee, K. N. Physical Review B, Vol. 3, Issue 6 https://doi.org/10.1103/PhysRevB.3.2030	journal	March 1971
Quantum Oscillations in Flux-Grown ${SmB}_{6}$ with Embedded Aluminum Thomas, S. M.; Ding, Xiaxin; Ronning, F. Physical Review Letters, Vol. 122, Issue 16 https://doi.org/10.1103/PhysRevLett.122.166401	journal	April 2019
High-Pressure Ground State of ${SmB}_{6}$ : Electronic Conduction and Long Range Magnetic Order Barla, A.; Derr, J.; Sanchez, J. P. Physical Review Letters, Vol. 94, Issue 16 https://doi.org/10.1103/PhysRevLett.94.166401	journal	April 2005
Magnetic Field-Tuned Quantum Criticality in the Metallic Ruthenate Sr3Ru2O7 Grigera, S. A. Science, Vol. 294, Issue 5541 https://doi.org/10.1126/science.1063539	journal	October 2001
Field suppression of the heavy-fermion state in ${CeRu}_{2}$ ${Si}_{2}$ van der Meulen, H. P.; de Visser, A.; Franse, J. J. M. Physical Review B, Vol. 44, Issue 2 https://doi.org/10.1103/PhysRevB.44.814	journal	July 1991
Transition of f electron nature from itinerant to localized: Metamagnetic transition in ${CeRu}_{2}$ ${Si}_{2}$ studied via the de Haas–van Alphen effect Aoki, H.; Uji, S.; Albessard, A. K. Physical Review Letters, Vol. 71, Issue 13 https://doi.org/10.1103/PhysRevLett.71.2110	journal	September 1993
Topological surface state in the Kondo insulator samarium hexaboride Kim, D. J.; Xia, J.; Fisk, Z. Nature Materials, Vol. 13, Issue 5 https://doi.org/10.1038/nmat3913	journal	March 2014
Heavy fermions in a high magnetic field Aoki, Dai; Knafo, William; Sheikin, Ilya Comptes Rendus Physique, Vol. 14, Issue 1 https://doi.org/10.1016/j.crhy.2012.11.004	journal	January 2013
Surface Hall Effect and Nonlocal Transport in SmB6: Evidence for Surface Conduction Kim, D. J.; Thomas, S.; Grant, T. Scientific Reports, Vol. 3, Issue 1 https://doi.org/10.1038/srep03150	journal	November 2013
Excitons in topological Kondo insulators: Theory of thermodynamic and transport anomalies in ${SmB}_{6}$ Knolle, Johannes; Cooper, Nigel R. Physical Review Letters, Vol. 118, Issue 9 https://doi.org/10.1103/PhysRevLett.118.096604	journal	March 2017
Field-Induced Metallic State in YbB ₁₂ under High Magnetic Field Sugiyama, Kiyohiro; Iga, Fumitoshi; Kasaya, Mitsuo Journal of the Physical Society of Japan, Vol. 57, Issue 11 https://doi.org/10.1143/JPSJ.57.3946	journal	November 1988
Magnetic and Semiconducting Properties of Sm $B_{6}$ Menth, A.; Buehler, E.; Geballe, T. H. Physical Review Letters, Vol. 22, Issue 7 https://doi.org/10.1103/PhysRevLett.22.295	journal	February 1969
Rare-earth compounds with mixed valencies Mott, N. F. Philosophical Magazine, Vol. 30, Issue 2 https://doi.org/10.1080/14786439808206566	journal	August 1974
Structure and properties of Ce3Pd3Bi4, CePdBi, and CePd2Zn3 Hermes, Wilfried; Linsinger, Stefan; Mishra, Ratikanta Monatshefte für Chemie - Chemical Monthly, Vol. 139, Issue 10 https://doi.org/10.1007/s00706-008-0914-4	journal	May 2008
Locally critical quantum phase transitions in strongly correlated metals Si, Qimiao; Rabello, Silvio; Ingersent, Kevin Nature, Vol. 413, Issue 6858 https://doi.org/10.1038/35101507	journal	October 2001
Nonmagnetic $4 f$ Shell in the High-Pressure Phase of SmS Maple, M. B.; Wohlleben, D. Physical Review Letters, Vol. 27, Issue 8 https://doi.org/10.1103/PhysRevLett.27.511	journal	August 1971
Heavy fermion semiconductors Riseborough, Peter S. Advances in Physics, Vol. 49, Issue 3 https://doi.org/10.1080/000187300243345	journal	May 2000
Heavy fermions in high magnetic fields Edwards, D. M.; Green, A. C. M. Zeitschrift für Physik B Condensed Matter, Vol. 103, Issue 2 https://doi.org/10.1007/s002570050367	journal	June 1996
Hybridization gap in ${Ce}_{3}$ ${Bi}_{4}$ ${Pt}_{3}$ Hundley, M. F.; Canfield, P. C.; Thompson, J. D. Physical Review B, Vol. 42, Issue 10 https://doi.org/10.1103/PhysRevB.42.6842	journal	October 1990
Interpretation of Kondo experiments in a magnetic field Schotte, K. D.; Schotte, U. Physics Letters A, Vol. 55, Issue 1 https://doi.org/10.1016/0375-9601(75)90386-2	journal	November 1975
Quantum Critical $5 f$ Electrons Avoid Singularities in $U (Ru, Rh)_{2} {Si}_{2}$ Silhanek, A. V.; Harrison, N.; Batista, C. D. Physical Review Letters, Vol. 95, Issue 2 https://doi.org/10.1103/PhysRevLett.95.026403	journal	July 2005
Studies of the Kondo insulator Ce3Bi4Pt3 in 61 T pulsed magnetic fields Boebinger, G. S.; Passner, A.; Canfield, P. C. Physica B: Condensed Matter, Vol. 211, Issue 1-4 https://doi.org/10.1016/0921-4526(94)00992-5	journal	May 1995
Crystal Growth and Characterization of the Kondo Semimetal CeNiSn Nakamoto, Go; Takabatake, Toshiro; Fujii, Hironobu Journal of the Physical Society of Japan, Vol. 64, Issue 12 https://doi.org/10.1143/JPSJ.64.4834	journal	December 1995
Multiscale fluctuations near a Kondo breakdown quantum critical point Paul, I.; Pépin, C.; Norman, M. R. Physical Review B, Vol. 78, Issue 3 https://doi.org/10.1103/PhysRevB.78.035109	journal	July 2008
High Field Gap Closure in the Kondo Insulator SmB6 Cooley, J. C.; Mielke, C. H.; Hults, W. L. Journal of Superconductivity, Vol. 12, Issue 1, p. 171-173 https://doi.org/10.1023/A:1007771030747	journal	February 1999
Probing a topological quantum critical point in semiconductor-superconductor heterostructures Tewari, Sumanta; Sau, J. D.; Scarola, V. W. Physical Review B, Vol. 85, Issue 15 https://doi.org/10.1103/PhysRevB.85.155302	journal	April 2012
Magnetization Process of the Kondo Insulator YbB ₁₂ in Ultrahigh Magnetic Fields Terashima, Taku T.; Ikeda, Akihiko; Matsuda, Yasuhiro H. Journal of the Physical Society of Japan, Vol. 86, Issue 5 https://doi.org/10.7566/JPSJ.86.054710	journal	May 2017
Observation of possible topological in-gap surface states in the Kondo insulator SmB6 by photoemission Jiang, J.; Li, S.; Zhang, T. Nature Communications, Vol. 4, Issue 1 https://doi.org/10.1038/ncomms4010	journal	December 2013
Theory of the Hall effect in heavy-fermion compounds Fert, A.; Levy, P. M. Physical Review B, Vol. 36, Issue 4 https://doi.org/10.1103/PhysRevB.36.1907	journal	August 1987
Fermi surface in the absence of a Fermi liquid in the Kondo insulator SmB6 Hartstein, M.; Toews, W. H.; Hsu, Y. -T. Nature Physics, Vol. 14, Issue 2 https://doi.org/10.1038/nphys4295	journal	October 2017

Similar Records

Intrinsic metallic behavior above 50 tesla in a Kondo insulator

Conference · Tue Dec 31 00:00:00 EST 1996 · OSTI ID:1619599

Boebinger, G S; Passner, A; Canfield, P C; +1 more

Pressure-induced concomitant topological and metal-insulator quantum phase transitions in Ce3Pd3Bi4

Journal Article · Thu Feb 03 00:00:00 EST 2022 · npj Quantum Materials · OSTI ID:1619599

Xu, Chenchao; Cao, Chao; Zhu, Jian-Xin

Spin-hole doping in the Kondo insulator Ce{sub 3}Bi{sub 4}Pt{sub 3} studied by neutron scattering

Conference · Wed Sep 01 00:00:00 EDT 1993 · OSTI ID:1619599

Severing, A; Perring, T; Thompson, J D; +2 more

Related Subjects

36 MATERIALS SCIENCE
High Magnetic Field Science
Kondo insulator
Fermi liquid
High magnetic field

Title: Magnetic field-tuned Fermi liquid in a Kondo insulator

Citation Formats

References (53)

Similar Records

Related Subjects