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Title: Origin of enhanced anisotropy in FePt-C granular films revealed by XMCD

Journal Article · · Applied Physics Letters
DOI:https://doi.org/10.1063/1.5092719· OSTI ID:1574323
ORCiD logo [1]; ORCiD logo [2];  [3];  [3];  [4]
  1. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
  3. Western Digital, San Jose, CA (United States)
  4. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of California, Santa Cruz, CA (United States)

We study the effect of carbon segregants on the spin and orbital moments of L10 FePt granular media using x-ray magnetic circular dichroism (XMCD) spectroscopy and report an effective decoupling of the structural film properties from the magnetic parameters of the grains. The carbon concentration reduces the grain size from (200 ± 160) nm2 down to (50 ± 20) nm2 for 40 mol. %C and improves sphericity and the order of grains, while preserving the crystalline order, spin and orbital moments, and perpendicular magnetocrystalline anisotropy. Here, we identify the primary cause of enhanced saturation and coercive fields as the reduced demagnetization fields of individual grains. The ability to shrink grains without impairing their magnetic properties is a critical requirement for the commercialization of Heat-Assisted Magnetic Recording.

Research Organization:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-05CH11231; AC02-05-CH11231
OSTI ID:
1574323
Alternate ID(s):
OSTI ID: 1508435
Journal Information:
Applied Physics Letters, Vol. 114, Issue 16; ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 2 works
Citation information provided by
Web of Science

References (15)

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FePt-C nanogranular films for perpendicular magnetic recording journal April 2009
A HAMR Media Technology Roadmap to an Areal Density of 4 Tb/in$^2$ journal January 2014
Effects of grain microstructure on magnetic properties in FePtAg-C media for heat assisted magnetic recording journal January 2013
Effects of cobalt substitution in L 1 0 -(Fe,Co)Pt thin films journal October 2017
Microstructure and magnetic properties of ultrathin FePt granular films journal December 2018
Magnetic moment of Fe in oxide-free FePt nanoparticles journal August 2007
Voltage controlled interfacial magnetism through platinum orbits journal June 2017
Development of ${\rm L}1_{0}$ FePt:C (001) Thin Films With High Coercivity and Small Grain Size for Ultra-High-Density Magnetic Recording Media journal February 2009
X-ray circular dichroism as a probe of orbital magnetization journal March 1992
Impact of carbon segregant on microstructure and magnetic properties of FePt-C nanogranular films on MgO (001) substrate journal March 2019
X-ray circular dichroism and local magnetic fields journal February 1993
Large enhancement of magnetic moment in L 1 0 ordered FePt thin films by Nd substitutional doping journal May 2015
Effect(s) of Cobalt Substitution in $L1_{0}$-(Fe,Co)Pt Thin Films text January 2017

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