Electrolyzer Durability at Low Catalyst Loading and with Dynamic Operation

Alia, Shaun M.; Stariha, Sarah; Borup, Rod L.

doi:10.1149/2.0231915jes

Title: Electrolyzer Durability at Low Catalyst Loading and with Dynamic Operation

Journal Article · Thu Oct 24 00:00:00 EDT 2019 · Journal of the Electrochemical Society

DOI:https://doi.org/10.1149/2.0231915jes· OSTI ID:1571705

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Research Organization:: National Renewable Energy Laboratory (NREL), Golden, CO (United States); Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Sustainable Transportation Office. Hydrogen Fuel Cell Technologies Office (HFTO); USDOE Office of Energy Efficiency and Renewable Energy (EERE). Fuel Cell Technologies Program (EE-3F)

Grant/Contract Number:: AC36-08GO28308; 89233218CNA000001

OSTI ID:: 1571705

Alternate ID(s):: OSTI ID: 1573203; OSTI ID: 1597349

Report Number(s):: NREL/JA-5900-75144; LA-UR-19-26971; /jes/166/15/F1164.atom

Journal Information:: Journal of the Electrochemical Society, Journal Name: Journal of the Electrochemical Society Vol. 166 Journal Issue: 15; ISSN 0013-4651

Publisher:: IOP Publishing - The Electrochemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 75 works

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References (41)

The stability of MEA in SPE water electrolysis for hydrogen production Wei, Guoqiang; Wang, Yuxin; Huang, Chengde International Journal of Hydrogen Energy, Vol. 35, Issue 9 https://doi.org/10.1016/j.ijhydene.2010.01.153	journal	May 2010
Developing titanium micro/nano porous layers on planar thin/tunable LGDLs for high-efficiency hydrogen production Kang, Zhenye; Yang, Gaoqiang; Mo, Jingke International Journal of Hydrogen Energy, Vol. 43, Issue 31 https://doi.org/10.1016/j.ijhydene.2018.05.139	journal	August 2018
Influence of the preparation method on the morphological and electrochemical properties of Ti/IrO2-coated electrodes de Oliveira-Sousa, A.; da Silva, M. A. S.; Machado, S. A. S. Electrochimica Acta, Vol. 45, Issue 27 https://doi.org/10.1016/S0013-4686(00)00508-9	journal	September 2000
Polymer Electrolyte Water Electrolysis: Correlating Performance and Porous Transport Layer Structure: Part II. Electrochemical Performance Analysis Schuler, Tobias; Schmidt, Thomas J.; Büchi, Felix N. Journal of The Electrochemical Society, Vol. 166, Issue 10 https://doi.org/10.1149/2.1241908jes	journal	January 2019
Oxygen evolution activity and stability of iridium in acidic media. Part 1. – Metallic iridium Cherevko, Serhiy; Geiger, Simon; Kasian, Olga Journal of Electroanalytical Chemistry, Vol. 773 https://doi.org/10.1016/j.jelechem.2016.04.033	journal	July 2016
Degradation of Proton Exchange Membrane (PEM) Water Electrolysis Cells: Looking Beyond the Cell Voltage Increase Suermann, Michel; Bensmann, Boris; Hanke-Rauschenbach, Richard Journal of The Electrochemical Society, Vol. 166, Issue 10 https://doi.org/10.1149/2.1451910jes	journal	January 2019
Nano-size IrOx catalyst of high activity and stability in PEM water electrolyzer with ultra-low iridium loading Yu, Haoran; Danilovic, Nemanja; Wang, Yang Applied Catalysis B: Environmental, Vol. 239 https://doi.org/10.1016/j.apcatb.2018.07.064	journal	December 2018
Preparation and characterisation of platinum and platinum–iridium coated titanium electrodes Kamachi Mudali, U.; Raju, V. R.; Dayal, R. K. Journal of Nuclear Materials, Vol. 277, Issue 1 https://doi.org/10.1016/S0022-3115(99)00141-5	journal	January 2000
Pathways to ultra-low platinum group metal catalyst loading in proton exchange membrane electrolyzers Ayers, Katherine E.; Renner, Julie N.; Danilovic, Nemanja Catalysis Today, Vol. 262 https://doi.org/10.1016/j.cattod.2015.10.019	journal	March 2016
Investigation of Mass Transport Losses in Polymer Electrolyte Electrolysis Cells Suermann, M.; Schmidt, T. J.; Buchi, F. N. ECS Transactions, Vol. 69, Issue 17 https://doi.org/10.1149/06917.1141ecst	journal	September 2015
Electrocatalytic Oxygen Evolution Reaction (OER) on Ru, Ir, and Pt Catalysts: A Comparative Study of Nanoparticles and Bulk Materials Reier, Tobias; Oezaslan, Mehtap; Strasser, Peter ACS Catalysis, Vol. 2, Issue 8 https://doi.org/10.1021/cs3003098	journal	July 2012
Impact of Intermittent Operation on Lifetime and Performance of a PEM Water Electrolyzer Weiß, A.; Siebel, A.; Bernt, M. Journal of The Electrochemical Society, Vol. 166, Issue 8 https://doi.org/10.1149/2.0421908jes	journal	January 2019
Improved durability of iridium oxide coated titanium anode with interlayers for oxygen evolution at high current densities Kamegaya, Y.; Sasaki, K.; Oguri, M. Electrochimica Acta, Vol. 40, Issue 7 https://doi.org/10.1016/0013-4686(94)00339-3	journal	May 1995
Highly Active, Durable Dispersed Iridium Nanocatalysts for PEM Water Electrolyzers Zhao, Shuai; Stocks, Allison; Rasimick, Brian Journal of The Electrochemical Society, Vol. 165, Issue 2 https://doi.org/10.1149/2.0981802jes	journal	January 2018
Performance of gold-coated titanium bipolar plates in unitized regenerative fuel cell operation Jung, Ho-Young; Huang, Sheng-Yang; Ganesan, Prabhu Journal of Power Sources, Vol. 194, Issue 2 https://doi.org/10.1016/j.jpowsour.2009.06.030	journal	December 2009
Gas Crossover Mitigation in PEM Water Electrolysis: Hydrogen Cross-over Benchmark Study of 3M's Ir-NSTF Based Electrolysis Catalyst-Coated Membranes Bessarabov, D.; Kruger, A.; Luopa, S. M. ECS Transactions, Vol. 75, Issue 14 https://doi.org/10.1149/07514.1165ecst	journal	August 2016
Durable PEM Fuel Cell Electrode Materials: Requirements and Benchmarking Methodologies Makharia, Rohit; Kocha, Shyam; Yu, Paul 208th ECS Meeting, ECS Transactions https://doi.org/10.1149/1.2214540	conference	January 2006
Electrochemical Equilibria Pourbaix, Marcel; Staehle, Roger W.; Pourbaix, Marcel Lectures on Electrochemical Corrosion, p 83-183 https://doi.org/10.1007/978-1-4684-1806-4_4	book	January 1973
Communication—Contribution of Catalyst Layer Proton Transport Resistance to Voltage Loss in Polymer Electrolyte Water Electrolyzers Babic, Ugljesa; Schmidt, Thomas J.; Gubler, Lorenz Journal of The Electrochemical Society, Vol. 165, Issue 15 https://doi.org/10.1149/2.0031815jes	journal	January 2018
Cell Performance Determining Parameters in High Pressure Water Electrolysis Suermann, Michel; Schmidt, Thomas J.; Büchi, Felix N. Electrochimica Acta, Vol. 211 https://doi.org/10.1016/j.electacta.2016.06.120	journal	September 2016
The stability challenge on the pathway to high-current-density polymer electrolyte membrane water electrolyzers Rakousky, Christoph; Keeley, Gareth P.; Wippermann, Klaus Electrochimica Acta, Vol. 278 https://doi.org/10.1016/j.electacta.2018.04.154	journal	July 2018
Effects of microstructure of IrO2-based anodes on electrocatalytic properties Otogawa, Ryuichi; Morimitsu, Masatsugu; Matsunaga, Morio Electrochimica Acta, Vol. 44, Issue 8-9 https://doi.org/10.1016/S0013-4686(98)00274-6	journal	December 1998
Failure of PEM water electrolysis cells: Case study involving anode dissolution and membrane thinning Grigoriev, S. A.; Dzhus, K. A.; Bessarabov, D. G. International Journal of Hydrogen Energy, Vol. 39, Issue 35 https://doi.org/10.1016/j.ijhydene.2014.05.043	journal	December 2014
Performance enhancement of PEM electrolyzers through iridium-coated titanium porous transport layers Liu, Chang; Carmo, Marcelo; Bender, Guido Electrochemistry Communications, Vol. 97 https://doi.org/10.1016/j.elecom.2018.10.021	journal	December 2018
Initial Performance and Durability of Ultra-Low Loaded NSTF Electrodes for PEM Electrolyzers Debe, M. K.; Hendricks, S. M.; Vernstrom, G. D. Journal of The Electrochemical Society, Vol. 159, Issue 6 https://doi.org/10.1149/2.065206jes	journal	January 2012
The Common Intermediates of Oxygen Evolution and Dissolution Reactions during Water Electrolysis on Iridium Kasian, Olga; Grote, Jan-Philipp; Geiger, Simon Angewandte Chemie International Edition, Vol. 57, Issue 9 https://doi.org/10.1002/anie.201709652	journal	February 2018
Initial approaches in benchmarking and round robin testing for proton exchange membrane water electrolyzers Bender, G.; Carmo, M.; Smolinka, T. International Journal of Hydrogen Energy, Vol. 44, Issue 18 https://doi.org/10.1016/j.ijhydene.2019.02.074	journal	April 2019
Iridium Oxygen Evolution Activity and Durability Baselines in Rotating Disk Electrode Half-Cells Alia, Shaun M.; Anderson, Grace C. Journal of The Electrochemical Society, Vol. 166, Issue 4 https://doi.org/10.1149/2.0731904jes	journal	January 2019
An analysis of degradation phenomena in polymer electrolyte membrane water electrolysis Rakousky, Christoph; Reimer, Uwe; Wippermann, Klaus Journal of Power Sources, Vol. 326 https://doi.org/10.1016/j.jpowsour.2016.06.082	journal	September 2016
Novel thin/tunable gas diffusion electrodes with ultra-low catalyst loading for hydrogen evolution reactions in proton exchange membrane electrolyzer cells Kang, Zhenye; Yang, Gaoqiang; Mo, Jingke Nano Energy, Vol. 47 https://doi.org/10.1016/j.nanoen.2018.03.015	journal	May 2018
Research Advances towards Low Cost, High Efficiency PEM Electrolysis Ayers, Katherine E.; Anderson, Everett B.; Capuano, Christopher 218th ECS Meeting, ECS Transactions https://doi.org/10.1149/1.3484496	conference	January 2010
Decoupling structure-sensitive deactivation mechanisms of Ir/IrOx electrocatalysts toward oxygen evolution reaction Tan, Xuehai; Shen, Jing; Semagina, Natalia Journal of Catalysis, Vol. 371 https://doi.org/10.1016/j.jcat.2019.01.018	journal	March 2019
Activity and Durability of Iridium Nanoparticles in the Oxygen Evolution Reaction Alia, Shaun M.; Rasimick, Brian; Ngo, Chilan Journal of The Electrochemical Society, Vol. 163, Issue 11 https://doi.org/10.1149/2.0151611jes	journal	January 2016
Perspectives on Low-Temperature Electrolysis and Potential for Renewable Hydrogen at Scale Ayers, Katherine; Danilovic, Nemanja; Ouimet, Ryan Annual Review of Chemical and Biomolecular Engineering, Vol. 10, Issue 1 https://doi.org/10.1146/annurev-chembioeng-060718-030241	journal	June 2019
Activity–Stability Trends for the Oxygen Evolution Reaction on Monometallic Oxides in Acidic Environments Danilovic, Nemanja; Subbaraman, Ramachandran; Chang, Kee-Chul The Journal of Physical Chemistry Letters, Vol. 5, Issue 14 https://doi.org/10.1021/jz501061n	journal	July 2014
Hydrogen at Scale (H ₂ @Scale): Key to a Clean, Economic, and Sustainable Energy System Pivovar, Bryan; Rustagi, Neha; Satyapal, Sunita The Electrochemical Society Interface, Vol. 27, Issue 1 https://doi.org/10.1149/2.F04181if	journal	January 2018
(Invited) H2@Scale: The Effect of Loading, Test Parameters, and Oxides on Electrolyzer-Catalyst Durability Alia, Shaun M.; Stariha, Sarah; Borup, Rod L. ECS Meeting Abstracts, Vol. MA2018-02, Issue 46 https://doi.org/10.1149/MA2018-02/46/1604	journal	July 2018
NSTF Advances for PEM Electrolysis - the Effect of Alloying on Activity of NSTF Electrolyzer Catalysts and Performance of NSTF Based PEM Electrolyzers Lewinski, K. A.; van der Vliet, D.; Luopa, S. M. ECS Transactions, Vol. 69, Issue 17 https://doi.org/10.1149/06917.0893ecst	journal	September 2015
Study of the Exchange Current Density for the Hydrogen Oxidation and Evolution Reactions Neyerlin, K. C.; Gu, Wenbin; Jorne, Jacob Journal of The Electrochemical Society, Vol. 154, Issue 7 https://doi.org/10.1149/1.2733987	journal	January 2007
Polymer electrolyte membrane water electrolysis: Restraining degradation in the presence of fluctuating power Rakousky, Christoph; Reimer, Uwe; Wippermann, Klaus Journal of Power Sources, Vol. 342 https://doi.org/10.1016/j.jpowsour.2016.11.118	journal	February 2017
Recent Advances in Catalyst Accelerated Stress Tests for Polymer Electrolyte Membrane Fuel Cells Stariha, Sarah; Macauley, Natalia; Sneed, Brian T. Journal of The Electrochemical Society, Vol. 165, Issue 7 https://doi.org/10.1149/2.0881807jes	journal	January 2018

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