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Title: PEDOT:PSS for Flexible and Stretchable Electronics: Modifications, Strategies, and Applications

Abstract

Substantial effort has been devoted to both scientific and technological developments of wearable, flexible, semitransparent, and sensing electronics (e.g., organic/perovskite photovoltaics, organic thin-film transistors, and medical sensors) in the past decade. The key to realizing those functionalities is essentially the fabrication of conductive electrodes with desirable mechanical properties. Conductive polymers (CPs) of poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) have emerged to be the most promising flexible electrode materials over rigid metallic oxides and play a critical role in these unprecedented devices as transparent electrodes, hole transport layers, interconnectors, electroactive layers, or motion-sensing conductors. Here, the current status of research on PEDOT:PSS is summarized including various approaches to boosting the electrical conductivity and mechanical compliance and stability, directly linked to the underlying mechanism of the performance enhancements. Along with the basic principles, the most cutting edge-progresses in devices with PEDOT:PSS are highlighted. Meanwhile, the advantages and plausible problems of the CPs and as-fabricated devices are pointed out. Finally, new perspectives are given for CP modifications and device fabrications. This work stresses the importance of developing CP films and reveals their critical role in the evolution of these next-generation devices featuring wearable, deformable, printable, ultrathin, and see-through characteristics.

Authors:
ORCiD logo [1];  [2];  [2];  [3];  [4];  [1];  [5];  [1];  [3];  [6]
  1. Ningbo Institute of Materials Technology and EngineeringChinese Academy of Sciences Ningbo 315201 China
  2. Division of Materials Physics and ApplicationLos Alamos National Laboratory Los Alamos NM 87545 USA
  3. Department of Applied PhysicsThe Hong Kong Polytechnic University Hung Hom Kowloon Hong Kong 999077 China
  4. School of Physics and ElectronicsHunan University Changsha 410082 China
  5. Ningbo Institute of Materials Technology and EngineeringChinese Academy of Sciences Ningbo 315201 China, School of Physics and ElectronicsHunan University Changsha 410082 China
  6. Ningbo Institute of Materials Technology and EngineeringChinese Academy of Sciences Ningbo 315201 China, Center of Materials Science and Optoelectronics EngineeringUniversity of Chinese Academy of Sciences Beijing 100049 China
Publication Date:
Research Org.:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE; USDOE Office of Science (SC). Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1568922
Alternate Identifier(s):
OSTI ID: 1558072; OSTI ID: 1568926
Report Number(s):
LA-UR-19-24580
Journal ID: ISSN 2198-3844
Grant/Contract Number:  
89233218CNA000001
Resource Type:
Journal Article: Published Article
Journal Name:
Advanced Science
Additional Journal Information:
Journal Name: Advanced Science Journal Volume: 6 Journal Issue: 19; Journal ID: ISSN 2198-3844
Publisher:
Wiley Blackwell (John Wiley & Sons)
Country of Publication:
Germany
Language:
English
Subject:
36 MATERIALS SCIENCE; Material Science

Citation Formats

Fan, Xi, Nie, Wanyi, Tsai, Hsinhan, Wang, Naixiang, Huang, Huihui, Cheng, Yajun, Wen, Rongjiang, Ma, Liujia, Yan, Feng, and Xia, Yonggao. PEDOT:PSS for Flexible and Stretchable Electronics: Modifications, Strategies, and Applications. Germany: N. p., 2019. Web. doi:10.1002/advs.201900813.
Fan, Xi, Nie, Wanyi, Tsai, Hsinhan, Wang, Naixiang, Huang, Huihui, Cheng, Yajun, Wen, Rongjiang, Ma, Liujia, Yan, Feng, & Xia, Yonggao. PEDOT:PSS for Flexible and Stretchable Electronics: Modifications, Strategies, and Applications. Germany. https://doi.org/10.1002/advs.201900813
Fan, Xi, Nie, Wanyi, Tsai, Hsinhan, Wang, Naixiang, Huang, Huihui, Cheng, Yajun, Wen, Rongjiang, Ma, Liujia, Yan, Feng, and Xia, Yonggao. Tue . "PEDOT:PSS for Flexible and Stretchable Electronics: Modifications, Strategies, and Applications". Germany. https://doi.org/10.1002/advs.201900813.
@article{osti_1568922,
title = {PEDOT:PSS for Flexible and Stretchable Electronics: Modifications, Strategies, and Applications},
author = {Fan, Xi and Nie, Wanyi and Tsai, Hsinhan and Wang, Naixiang and Huang, Huihui and Cheng, Yajun and Wen, Rongjiang and Ma, Liujia and Yan, Feng and Xia, Yonggao},
abstractNote = {Substantial effort has been devoted to both scientific and technological developments of wearable, flexible, semitransparent, and sensing electronics (e.g., organic/perovskite photovoltaics, organic thin-film transistors, and medical sensors) in the past decade. The key to realizing those functionalities is essentially the fabrication of conductive electrodes with desirable mechanical properties. Conductive polymers (CPs) of poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) have emerged to be the most promising flexible electrode materials over rigid metallic oxides and play a critical role in these unprecedented devices as transparent electrodes, hole transport layers, interconnectors, electroactive layers, or motion-sensing conductors. Here, the current status of research on PEDOT:PSS is summarized including various approaches to boosting the electrical conductivity and mechanical compliance and stability, directly linked to the underlying mechanism of the performance enhancements. Along with the basic principles, the most cutting edge-progresses in devices with PEDOT:PSS are highlighted. Meanwhile, the advantages and plausible problems of the CPs and as-fabricated devices are pointed out. Finally, new perspectives are given for CP modifications and device fabrications. This work stresses the importance of developing CP films and reveals their critical role in the evolution of these next-generation devices featuring wearable, deformable, printable, ultrathin, and see-through characteristics.},
doi = {10.1002/advs.201900813},
url = {https://www.osti.gov/biblio/1568922}, journal = {Advanced Science},
issn = {2198-3844},
number = 19,
volume = 6,
place = {Germany},
year = {2019},
month = {7}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record at https://doi.org/10.1002/advs.201900813

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Cited by: 24 works
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