PEDOT:PSS for Flexible and Stretchable Electronics: Modifications, Strategies, and Applications

Fan, Xi; Nie, Wanyi; Tsai, Hsinhan; Wang, Naixiang; Huang, Huihui; Cheng, Yajun; Wen, Rongjiang; Ma, Liujia; Yan, Feng; Xia, Yonggao

doi:10.1002/advs.201900813

Title: PEDOT:PSS for Flexible and Stretchable Electronics: Modifications, Strategies, and Applications

Journal Article · Tue Jul 30 00:00:00 EDT 2019 · Advanced Science

DOI:https://doi.org/10.1002/advs.201900813· OSTI ID:1568922

^[1]; Nie, Wanyi ^[2]; Tsai, Hsinhan ^[2]; Wang, Naixiang ^[3]; Huang, Huihui ^[4]; Cheng, Yajun ^[1]; Wen, Rongjiang ^[5]; Ma, Liujia ^[1]; Yan, Feng ^[3]; Xia, Yonggao ^[6]

Ningbo Institute of Materials Technology and Engineering Chinese Academy of Sciences Ningbo 315201 China
Division of Materials Physics and Application Los Alamos National Laboratory Los Alamos NM 87545 USA
Department of Applied Physics The Hong Kong Polytechnic University Hung Hom Kowloon Hong Kong 999077 China
School of Physics and Electronics Hunan University Changsha 410082 China
Ningbo Institute of Materials Technology and Engineering Chinese Academy of Sciences Ningbo 315201 China, School of Physics and Electronics Hunan University Changsha 410082 China
Ningbo Institute of Materials Technology and Engineering Chinese Academy of Sciences Ningbo 315201 China, Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences Beijing 100049 China

Abstract Substantial effort has been devoted to both scientific and technological developments of wearable, flexible, semitransparent, and sensing electronics (e.g., organic/perovskite photovoltaics, organic thin‐film transistors, and medical sensors) in the past decade. The key to realizing those functionalities is essentially the fabrication of conductive electrodes with desirable mechanical properties. Conductive polymers (CPs) of poly(3,4‐ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) have emerged to be the most promising flexible electrode materials over rigid metallic oxides and play a critical role in these unprecedented devices as transparent electrodes, hole transport layers, interconnectors, electroactive layers, or motion‐sensing conductors. Here, the current status of research on PEDOT:PSS is summarized including various approaches to boosting the electrical conductivity and mechanical compliance and stability, directly linked to the underlying mechanism of the performance enhancements. Along with the basic principles, the most cutting edge‐progresses in devices with PEDOT:PSS are highlighted. Meanwhile, the advantages and plausible problems of the CPs and as‐fabricated devices are pointed out. Finally, new perspectives are given for CP modifications and device fabrications. This work stresses the importance of developing CP films and reveals their critical role in the evolution of these next‐generation devices featuring wearable, deformable, printable, ultrathin, and see‐through characteristics.

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE; USDOE Office of Science (SC). Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: 89233218CNA000001

OSTI ID:: 1568922

Alternate ID(s):: OSTI ID: 1558072; OSTI ID: 1568926

Report Number(s):: LA-UR-19-24580; 1900813

Journal Information:: Advanced Science, Journal Name: Advanced Science Vol. 6 Journal Issue: 19; ISSN 2198-3844

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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Cited by: 421 works

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