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Title: Bose glass and Mott glass of quasiparticles in a doped quantum magnet

Journal Article · · Nature (London)
DOI:https://doi.org/10.1038/nature11406· OSTI ID:1564845

The low-temperature states of bosonic fluids exhibit fundamental quantum effects at the macroscopic scale: the best-known examples are Bose–Einstein condensation and superfluidity, which have been tested experimentally in a variety of different systems. When bosons interact, disorder can destroy condensation, leading to a ‘Bose glass’. This phase has been very elusive in experiments owing to the absence of any broken symmetry and to the simultaneous absence of a finite energy gap in the spectrum. Here we report the observation of a Bose glass of field-induced magnetic quasiparticles in a doped quantum magnet (bromine-doped dichloro-tetrakis-thiourea-nickel, DTN). The physics of DTN in a magnetic field is equivalent to that of a lattice gas of bosons in the grand canonical ensemble; bromine doping introduces disorder into the hopping and interaction strength of the bosons, leading to their localization into a Bose glass down to zero field, where it becomes an incompressible Mott glass. The transition from the Bose glass (corresponding to a gapless spin liquid) to the Bose–Einstein condensate (corresponding to a magnetically ordered phase) is marked by a universal exponent that governs the scaling of the critical temperature with the applied field, in excellent agreement with theoretical predictions. Our study represents a quantitative experimental account of the universal features of disordered bosons in the grand canonical ensemble.

Research Organization:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Oak Ridge Leadership Computing Facility (OLCF); Univ. of Southern California, Los Angeles, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC)
DOE Contract Number:
FG02-05ER46240; FG03-01ER45908
OSTI ID:
1564845
Journal Information:
Nature (London), Vol. 489, Issue 7416; ISSN 0028-0836
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English

References (28)

Localization: theory and experiment journal December 1993
Anderson localization and interactions in one-dimensional metals journal January 1988
Boson localization and the superfluid-insulator transition journal July 1989
Onset of superfluidity in He 4 films adsorbed on disordered substrates journal May 1997
Localization of preformed Cooper pairs in disordered superconductors journal January 2011
Single- and two-particle energy gaps across the disorder-driven superconductor–insulator transition journal July 2011
Disordered quantum gases under control journal February 2010
Exciton-polariton Bose-Einstein condensation journal May 2010
Bose–Einstein condensation in magnetic insulators journal March 2008
Bose-Glass Phases in Disordered Quantum Magnets journal November 2005
Quantum Localization in Bilayer Heisenberg Antiferromagnets with Site Dilution journal November 2005
Field-induced quantum-disordered phases in S = 1 2 weakly coupled dimer systems with site dilution journal October 2006
Disordered States in IPA Cu ( Cl x Br 1 x ) 3 Induced by Bond Randomness journal August 2008
Evidence of a magnetic Bose glass in ( CH 3 ) 2 CHNH 3 Cu ( Cl { 0.95 } Br { 0.05 } ) 3 from neutron diffraction journal February 2010
Bose-Einstein Condensation of S = 1 Nickel Spin Degrees of Freedom in NiCl 2 4 SC ( NH 2 ) 2 journal February 2006
Direct Measurement of the Bose-Einstein Condensation Universality Class in NiCl 2 4 SC ( NH 2 ) 2 at Ultralow Temperatures journal October 2008
Possible New Phase of Commensurate Insulators with Disorder: The Mott Glass journal September 1999
Superfluid-Insulator Transition in Commensurate Disordered Bosonic Systems: Large-Scale Worm Algorithm Simulations journal January 2004
Phase Transition in a System of One-Dimensional Bosons with Strong Disorder journal October 2004
Mott Glass in Site-Diluted S = 1 Antiferromagnets with Single-Ion Anisotropy journal July 2007
Magnetic Excitations in the Spin-1 Anisotropic Heisenberg Antiferromagnetic Chain System NiCl 2 4 SC ( NH 2 ) 2 journal January 2007
Spin dynamics of Ni Cl 2 4 S C ( N H 2 ) 2 in the field-induced ordered phase journal March 2008
Magnetic Susceptibility Measurements at Ultra-low Temperatures journal November 2009
Superfluid-Insulator Transition in a Commensurate One-Dimensional Bosonic System with Off-Diagonal Disorder journal July 2005
Universal phase diagram of disordered bosons from a doped quantum magnet journal January 2010
Low-temperature thermodynamic properties near the field-induced quantum critical point in NiCl 2 -4SC(NH 2 ) 2 journal May 2012
Quantum Critical Point of the X Y Model and Condensation of Field-induced Quasiparticles in Dimer Compounds journal December 2004
Quantum critical scaling at a Bose-glass/superfluid transition: Theory and experiment for a model quantum magnet journal October 2012

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