skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Buckling and twisting of advanced materials into morphable 3D mesostructures

Journal Article · · Proceedings of the National Academy of Sciences of the United States of America
 [1];  [2];  [1];  [3];  [4];  [5];  [6];  [1];  [7];  [8]; ORCiD logo [2];  [9];  [2];  [10]; ORCiD logo [2];  [11];  [12];  [13];  [14];  [15]
  1. Center for Bio-Integrated Electronics, Northwestern University, Evanston, IL 60208,
  2. Department of Civil and Environmental Engineering, Northwestern University, Evanston, IL 60208,, Department of Mechanical Engineering, Northwestern University, Evanston, IL 60208,, Department of Materials Science and Engineering, Northwestern University, Evanston, IL 60208,
  3. Department of Civil and Environmental Engineering, Northwestern University, Evanston, IL 60208,, Department of Mechanical Engineering, Northwestern University, Evanston, IL 60208,, Department of Materials Science and Engineering, Northwestern University, Evanston, IL 60208,, School of Logistics Engineering, Wuhan University of Technology, 430063 Wuhan, China,
  4. NanoScience Technology Center, University of Central Florida, Orlando, FL 32826,, CREOL, The College of Optics and Photonics, University of Central Florida, Orlando, FL 32816,
  5. Center for Nanoscale Materials, Argonne National Laboratory, Lemont, IL 60439,
  6. Department of Civil and Environmental Engineering, Northwestern University, Evanston, IL 60208,, Department of Mechanical Engineering, Northwestern University, Evanston, IL 60208,, Department of Materials Science and Engineering, Northwestern University, Evanston, IL 60208,, Department of Engineering Mechanics, Dalian University of Technology, 116024 Dalian, China,
  7. State Key Laboratory for Mechanical Behavior of Materials, School of Materials Science and Engineering, Xi’an Jiaotong University, 710049 Xi’an, China,
  8. Center for Bio-Integrated Electronics, Northwestern University, Evanston, IL 60208,, Department of Mechanical and Aerospace Engineering, University of Missouri-Columbia, Columbia, MO 65211,
  9. Department of Mechanical Engineering, Northwestern University, Evanston, IL 60208,
  10. Center for Bio-Integrated Electronics, Northwestern University, Evanston, IL 60208,, Key Laboratory of Mechanism Theory and Equipment Design of Ministry of Education, Tianjin University, 300072 Tianjin, China,, School of Mechanical Engineering, Tianjin University, 300072 Tianjin, China,
  11. Center for Nanoscale Materials, Argonne National Laboratory, Lemont, IL 60439,, Department of Chemistry, Northwestern University, Evanston, IL 60208,
  12. NanoScience Technology Center, University of Central Florida, Orlando, FL 32826,, CREOL, The College of Optics and Photonics, University of Central Florida, Orlando, FL 32816,, Department of Physics, University of Central Florida, Orlando, FL 32816,
  13. Center for Bio-Integrated Electronics, Northwestern University, Evanston, IL 60208,, Department of Civil and Environmental Engineering, Northwestern University, Evanston, IL 60208,, Department of Mechanical Engineering, Northwestern University, Evanston, IL 60208,, Department of Materials Science and Engineering, Northwestern University, Evanston, IL 60208,
  14. Center for Flexible Electronics Technology, Tsinghua University, 100084 Beijing, China,, Applied Mechanics Laboratory, Department of Engineering Mechanics, Tsinghua University, 100084 Beijing, China,
  15. Center for Bio-Integrated Electronics, Northwestern University, Evanston, IL 60208,, Department of Mechanical Engineering, Northwestern University, Evanston, IL 60208,, Department of Materials Science and Engineering, Northwestern University, Evanston, IL 60208,, Department of Chemistry, Northwestern University, Evanston, IL 60208,, Department of Biomedical Engineering, Northwestern University, Evanston, IL 60208,

Recently developed methods in mechanically guided assembly provide deterministic access to wide-ranging classes of complex, 3D structures in high-performance functional materials, with characteristic length scales that can range from nanometers to centimeters. These processes exploit stress relaxation in prestretched elastomeric platforms to affect transformation of 2D precursors into 3D shapes by in- and out-of-plane translational displacements. This paper introduces a scheme for introducing local twisting deformations into this process, thereby providing access to 3D mesostructures that have strong, local levels of chirality and other previously inaccessible geometrical features. Here, elastomeric assembly platforms segmented into interconnected, rotatable units generate in-plane torques imposed through bonding sites at engineered locations across the 2D precursors during the process of stress relaxation. Nearly 2 dozen examples illustrate the ideas through a diverse variety of 3D structures, including those with designs inspired by the ancient arts of origami/kirigami and with layouts that can morph into different shapes. Here, a mechanically tunable, multilayered chiral 3D metamaterial configured for operation in the terahertz regime serves as an application example guided by finite-element analysis and electromagnetic modeling.

Research Organization:
Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Organization:
National Science Foundation (NSF); National Natural Science Foundation of China (NSFC); USDOE Office of Science (SC)
Grant/Contract Number:
AC02-06CH11357
OSTI ID:
1527191
Alternate ID(s):
OSTI ID: 1559024
Journal Information:
Proceedings of the National Academy of Sciences of the United States of America, Journal Name: Proceedings of the National Academy of Sciences of the United States of America Vol. 116 Journal Issue: 27; ISSN 0027-8424
Publisher:
Proceedings of the National Academy of SciencesCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 73 works
Citation information provided by
Web of Science

References (46)

Negative refractive index due to chirality journal March 2009
Three-dimensional mesostructures as high-temperature growth templates, electronic cellular scaffolds, and self-propelled microrobots journal October 2017
Origami Biosystems: 3D Assembly Methods for Biomedical Applications journal September 2018
Programmable matter by folding journal June 2010
Optical Chirality in Nonlinear Optics: Application to High Harmonic Generation journal March 2018
Engineering the shape and structure of materials by fractal cut journal November 2014
Controlling the self-folding of a polymer sheet using a local heater: the effect of the polymer–heater interface journal January 2017
High-power lithium ion microbatteries from interdigitated three-dimensional bicontinuous nanoporous electrodes journal April 2013
A mechanically driven form of Kirigami as a route to 3D mesostructures in micro/nanomembranes journal September 2015
Printing, folding and assembly methods for forming 3D mesostructures in advanced materials journal March 2017
Voxelated liquid crystal elastomers journal February 2015
Freestanding 3D Mesostructures, Functional Devices, and Shape-Programmable Systems Based on Mechanically Induced Assembly with Shape Memory Polymers journal October 2018
Compliant and stretchable thermoelectric coils for energy harvesting in miniature flexible devices journal November 2018
Ultralight, ultrastiff mechanical metamaterials journal June 2014
Chiral sensing of amino acids and proteins chelating with Eu III complexes by Raman optical activity spectroscopy journal January 2016
Exploiting Nanoroughness on Holographically Patterned Three-Dimensional Photonic Crystals journal April 2012
Gold helix photonic metamaterials: A numerical parameter study journal January 2010
Multidimensional Architectures for Functional Optical Devices journal February 2010
Functional stimuli responsive hydrogel devices by self-folding journal August 2014
3D-Printed Artificial Microfish journal June 2015
Assembly of micro/nanomaterials into complex, three-dimensional architectures by compressive buckling journal January 2015
Printing soft matter in three dimensions journal December 2016
Chiral plasmonics journal May 2017
Elastocapillary fabrication of three-dimensional microstructures journal July 2010
Macroporous nanowire nanoelectronic scaffolds for synthetic tissues journal August 2012
3D Printing of Interdigitated Li-Ion Microbattery Architectures journal June 2013
Guided Folding of Nematic Liquid Crystal Elastomer Sheets into 3D via Patterned 1D Microchannels journal September 2016
A double perturbation method of postbuckling analysis in 2D curved beams for assembly of 3D ribbon-shaped structures journal February 2018
Design of Hierarchically Cut Hinges for Highly Stretchable and Reconfigurable Metamaterials with Enhanced Strength journal October 2015
Robust Hierarchically Structured Biphasic Ambipolar Oxide Photoelectrodes for Light-Driven Chemical Regulation and Switchable Logic Applications journal September 2016
Morphable 3D mesostructures and microelectronic devices by multistable buckling mechanics journal January 2018
Gold Helix Photonic Metamaterial as Broadband Circular Polarizer journal August 2009
Nano-kirigami with giant optical chirality journal July 2018
Laser-assisted direct ink writing of planar and 3D metal architectures journal May 2016
Designing Responsive Buckled Surfaces by Halftone Gel Lithography journal March 2012
Controlled Mechanical Buckling for Origami-Inspired Construction of 3D Microstructures in Advanced Materials journal February 2016
Generating Switchable and Reconfigurable Optical Vortices via Photopatterning of Liquid Crystals journal December 2013
Metamaterial with negative index due to chirality journal January 2009
Engineered Elastomer Substrates for Guided Assembly of Complex 3D Mesostructures by Spatially Nonuniform Compressive Buckling journal November 2016
Chiral metamaterials with negative refractive index based on four “U” split ring resonators journal August 2010
Mechanical assembly of complex, 3D mesostructures from releasable multilayers of advanced materials journal September 2016
Instrumented cardiac microphysiological devices via multimaterial three-dimensional printing journal October 2016
Self-folding thin-film materials: From nanopolyhedra to graphene origami journal September 2012
Three-dimensional piezoelectric polymer microsystems for vibrational energy harvesting, robotic interfaces and biomedical implants journal January 2019
Mechanical Self-Assembly of a Strain-Engineered Flexible Layer: Wrinkling, Rolling, and Twisting journal January 2016
Past achievements and future challenges in the development of three-dimensional photonic metamaterials journal July 2011

Figures / Tables (21)


Similar Records

Three-dimensional mesostructures as high-temperature growth templates, electronic cellular scaffolds, and self-propelled microrobots
Journal Article · Wed Oct 25 00:00:00 EDT 2017 · Proceedings of the National Academy of Sciences of the United States of America · OSTI ID:1527191

A mechanically driven form of Kirigami as a route to 3D mesostructures in micro/nanomembranes
Journal Article · Tue Sep 08 00:00:00 EDT 2015 · Proceedings of the National Academy of Sciences of the United States of America · OSTI ID:1527191

Mechanical assembly of complex, 3D mesostructures from releasable multilayers of advanced materials
Journal Article · Fri Sep 23 00:00:00 EDT 2016 · Science Advances · OSTI ID:1527191