Engineered Enzymes and Bioinspired Catalysts for Energy Conversion
Journal Article
·
· ACS Energy Letters
- Department of Chemistry, University of Rochester, Rochester, New York 14627, United States
Metalloenzymes play critical roles in the environment by catalyzing redox reactions in biogeochemical cycles. The elucidation of structure–function relationships in these biocatalysts has provided a foundation for the development of bioinspired catalysts for fuel production and small-molecule activation. In this Perspective, we highlight developments in engineered biomolecular and bioinspired catalysts for the reduction of H+, O2, and CO2 and for the oxidation of H2 and H2O. The roles of proton transfers and second-sphere interactions in particular are highlighted.
- Research Organization:
- Univ. of Rochester, NY (United States)
- Sponsoring Organization:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- Grant/Contract Number:
- FG02-09ER16121; SC0002106
- OSTI ID:
- 1558717
- Alternate ID(s):
- OSTI ID: 1561994
- Journal Information:
- ACS Energy Letters, Journal Name: ACS Energy Letters Vol. 4 Journal Issue: 9; ISSN 2380-8195
- Publisher:
- American Chemical SocietyCopyright Statement
- Country of Publication:
- United States
- Language:
- English
Cited by: 46 works
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