Synthesis and optical properties of ordered-vacancy perovskite cesium bismuth halide nanocrystals

Nelson, R. D.; Santra, K.; Wang, Y.; Hadi, A.; Petrich, J. W.; Panthani, M. G.

doi:10.1039/c7cc07223f

Title: Synthesis and optical properties of ordered-vacancy perovskite cesium bismuth halide nanocrystals

Journal Article · Tue Mar 13 00:00:00 EDT 2018 · ChemComm

DOI:https://doi.org/10.1039/c7cc07223f· OSTI ID:1556931

Nelson, R. D. ^[1];

^[1]; Wang, Y. ^[1]; Hadi, A. ^[1]; Petrich, J. W. ^[1];

^[1]

Iowa State Univ., Ames, IA (United States)

Perovskite-phase cesium bismuth halide (Cs₃Bi₂X₉; X= Cl, Br, I) nanocrystals were synthesized using a hot-injection approach. These nanocrystals adopted ordered-vacancy perovskite crystal structures and demonstrated composition-tunable optical properties. Growth occurred by initial formation of Bi⁰ seeds, and morphology was controlled by precursor and seed concentration. The Cs₃Bi₂I₉ nanocrystals demonstrated excellent stability under ambient conditions for several months. Contrary to previous reports, we find that photoluminescence originates from the precursor material as opposed to the perovskite nanocrystals.

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Research Organization:: Ames Laboratory (AMES), Ames, IA (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02-07CH11358; DGE1247194

OSTI ID:: 1556931

Alternate ID(s):: OSTI ID: 1434096

Report Number(s):: IS-J-9654; CHCOFS

Journal Information:: ChemComm, Vol. 54, Issue 29; ISSN 1359-7345

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 49 works

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