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Title: Adaptive Sample Preparation and Target Fabrication for High-Throughput Materials Science

Technical Report ·
DOI:https://doi.org/10.2172/1542805· OSTI ID:1542805
 [1]; ORCiD logo [1];  [2];  [3];  [4];  [5];  [1];  [6];  [7]
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  2. Texas A & M Univ., College Station, TX (United States)
  3. SLAC National Accelerator Lab., Menlo Park, CA (United States)
  4. General Atomics, San Diego, CA (United States)
  5. National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)
  6. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  7. Helmholtz-Zentrum Dresden-Rossendorf (Germany)

High-repetition-rate brilliant and coherent light sources are significantly increasing the rate at which scientific experiments can be performed. An investment in transformative technologies to make samples of condensed matter could enable a paradigm shift for that field or open new exciting frontiers in high-energy density science (HEDS). This will especially be true for dynamic materials in extremes research or HEDS, where the repetition rate for placing samples into extreme environments is increasing and the samples or targets are irreversibly destroyed in each experiment. Research teams that are able to implement solutions to all aspects of the experimental process and enable a paradigm of high-throughput science will have the greatest success and impact. There are two different directions for adaptive samples. One is research when the number of experiments can be greatly increased with increased volume, such as in high energy density science. The other is when flexibility and agility can aid Bayesian optimization computational methods and speed up the discovery process, as with materials science. Conducting a similar equation-of-state (EOS) experiment took three years on the OMEGA laser facility, compared to five days of shifts at the LCLS XFEL. New materials with improved properties have been found by guided optimization of experimental science. Adaptive sample preparation and target fabrication can create a tremendous return on scientific investment. High-throughput enabling precision science is also a desirable goal. To address these issues, we sought a diverse set of innovative participants who had ideas of how to achieve this paradigm shift. We invited 42 researchers from a variety of disciplines and fields to attend a workshop in College Station, Texas, May 14–16, 2019. Many of the participants had never been in the same room before, and most found it very exciting to hear about new and different research. The goal was twofold: to define the challenges, i.e., “what would we like to be able to do and why it is difficult to do so,” and to describe the progress, approaches and capabilities, as well as the vision, “what we could do if we had more support.”

Research Organization:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA), Office of Defense Programs (DP)
DOE Contract Number:
89233218CNA000001
OSTI ID:
1542805
Report Number(s):
LA-UR-19-26624
Resource Relation:
Conference: Adaptive Sample Preparation and Target Fabrication for High-Throughput Materials Science, College Station, TX (United States), 14-16 May 2019
Country of Publication:
United States
Language:
English

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