Probing double Rydberg wave packets in a helium atom with fast single-cycle pulses

Wang, Xiao; Robicheaux, F.

doi:10.1103/physreva.96.043409

Title: Probing double Rydberg wave packets in a helium atom with fast single-cycle pulses

Journal Article · Wed Oct 11 00:00:00 EDT 2017 · Physical Review A

DOI:https://doi.org/10.1103/physreva.96.043409· OSTI ID:1540658

Wang, Xiao ^[1]; Robicheaux, F. ^[2]

Purdue Univ., West Lafayette, IN (United States)
Purdue Univ., West Lafayette, IN (United States); Purdue Univ., West Lafayette, IN (United States). Purdue Quantum Center

Fully quantum and classical calculations on a helium atom with two excited, radially localized Rydberg wave packets are performed. The differences between classical and quantum methods are compared for a wide range of principal quantum numbers to study the validity of the classical method for low-lying states. Furthermore, the effects of fast terahertz single-cycle pulses on an atomic system with one or two Rydberg wave packets are also studied using classical equations of motion. These results suggest that single-cycle pulses can be used as time-resolved probes to detect motion of the wave packets and to investigate autoionization properties.

View Accepted Manuscript (DOE)

Cite

Export

Save

Research Organization:: Purdue Univ., West Lafayette, IN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0012193

OSTI ID:: 1540658

Alternate ID(s):: OSTI ID: 1399066

Journal Information:: Physical Review A, Vol. 96, Issue 4; ISSN 2469-9926

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 4 works

Citation information provided by
Web of Science

References (39)

Dynamics of Rydberg wave packets generated by half-cycle pulses Reinhold, C. O.; Burgdörfer, J.; Frey, M. T. Physical Review A, Vol. 54, Issue 1 https://doi.org/10.1103/PhysRevA.54.R33	journal	July 1996
Ramsey fringes in atomic Rydberg wave packets Noordam, L. D.; Duncan, D. I.; Gallagher, T. F. Physical Review A, Vol. 45, Issue 7 https://doi.org/10.1103/PhysRevA.45.4734	journal	April 1992
Autoionizing Rydberg states of NO in strong electric fields Warntjes, J. B. M.; Robicheaux, F.; Bakker, J. M. The Journal of Chemical Physics, Vol. 111, Issue 6 https://doi.org/10.1063/1.479533	journal	August 1999
Tracing and controlling electronic dynamics in atoms and molecules by attosecond pulses Peng, Liang-You; Jiang, Wei-Chao; Geng, Ji-Wei Physics Reports, Vol. 575 https://doi.org/10.1016/j.physrep.2015.02.002	journal	April 2015
Attosecond Two-Photon Interferometry for Doubly Excited States of Helium Feist, J.; Nagele, S.; Ticknor, C. Physical Review Letters, Vol. 107, Issue 9 https://doi.org/10.1103/PhysRevLett.107.093005	journal	August 2011
Comparisons of classical and quantum dynamics for initially localized states Davis, M. J.; Heller, E. J. The Journal of Chemical Physics, Vol. 80, Issue 10 https://doi.org/10.1063/1.446571	journal	May 1984
The classical limit of ionization in fast ion-atom collisions Reinhold, C. O.; Burgdorfer, J. Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 26, Issue 18 https://doi.org/10.1088/0953-4075/26/18/018	journal	September 1993
Modulation of Attosecond Beating in Resonant Two-Photon Ionization Jiménez-Galán, Álvaro; Argenti, Luca; Martín, Fernando Physical Review Letters, Vol. 113, Issue 26 https://doi.org/10.1103/PhysRevLett.113.263001	journal	December 2014
The theory of two-electron atoms: between ground state and complete fragmentation Tanner, Gregor; Richter, Klaus; Rost, Jan-Michael Reviews of Modern Physics, Vol. 72, Issue 2 https://doi.org/10.1103/RevModPhys.72.497	journal	April 2000
Rydberg wave packets in many-electron atoms excited by short laser pulses Henle, W. A.; Ritsch, H.; Zoller, P. Physical Review A, Vol. 36, Issue 2 https://doi.org/10.1103/PhysRevA.36.683	journal	July 1987
Angular Correlation between Photoelectrons and Auger Electrons from $K$ -Shell Ionization of Neon Landers, A. L.; Robicheaux, F.; Jahnke, T. Physical Review Letters, Vol. 102, Issue 22 https://doi.org/10.1103/PhysRevLett.102.223001	journal	June 2009
Time-Domain Investigation of Electron Recapture via Post-Collision Interaction in a Double Photoionization Continuum Pisharody, S. N.; Jones, R. R. Physical Review Letters, Vol. 91, Issue 20 https://doi.org/10.1103/PhysRevLett.91.203002	journal	November 2003
Quantum Theory of Angular Momentum Varshalovich, D. A.; Moskalev, A. N.; Khersonskii, V. K. https://doi.org/10.1142/0270	book	October 1988
Probing Two-Electron Dynamics of an Atom Pisharody, S. N. Science, Vol. 303, Issue 5659 https://doi.org/10.1126/science.1092220	journal	February 2004
Two-photon finite-pulse model for resonant transitions in attosecond experiments Jiménez-Galán, Álvaro; Martín, Fernando; Argenti, Luca Physical Review A, Vol. 93, Issue 2 https://doi.org/10.1103/PhysRevA.93.023429	journal	February 2016
Rydberg Wave Packets and the Classical Limit Parker, Jonathan; Stroud, C. R. Physica Scripta, Vol. T12 https://doi.org/10.1088/0031-8949/1986/T12/010	journal	January 1986
Quantum intramolecular dynamics: Criteria for stochastic and nonstochastic flow Heller, Eric J. The Journal of Chemical Physics, Vol. 72, Issue 2 https://doi.org/10.1063/1.439197	journal	January 1980
Rydberg-wave-packet evolution in a frozen gas of dipole-dipole-coupled atoms Zhou, Tao; Li, Sha; Jones, R. R. Physical Review A, Vol. 89, Issue 6 https://doi.org/10.1103/PhysRevA.89.063413	journal	June 2014
Charge-transfer and impact-ionization cross sections for fully and partially stripped positive ions colliding with atomic hydrogen Olson, R. E.; Salop, A. Physical Review A, Vol. 16, Issue 2 https://doi.org/10.1103/PhysRevA.16.531	journal	August 1977
Observation of Radially Localized Atomic Electron Wave Packets ten Wolde, A.; Noordam, L. D.; Lagendijk, A. Physical Review Letters, Vol. 61, Issue 18 https://doi.org/10.1103/PhysRevLett.61.2099	journal	October 1988
Single-shot detection of wavepacket evolution Campbell, M.; Bensky, T.; Jones, Robert Optics Express, Vol. 1, Issue 7 https://doi.org/10.1364/OE.1.000197	journal	January 1997
Generation and detection of Rydberg wave packets by short laser pulses Alber, G.; Ritsch, H.; Zoller, P. Physical Review A, Vol. 34, Issue 2 https://doi.org/10.1103/PhysRevA.34.1058	journal	August 1986
Time-Dependent Electron Interactions in Double Rydberg Wave Packets Zhang, X.; Jones, R. R.; Robicheaux, F. Physical Review Letters, Vol. 110, Issue 2 https://doi.org/10.1103/PhysRevLett.110.023002	journal	January 2013
The time-dependent close-coupling method for atomic and molecular collision processes Pindzola, M. S.; Robicheaux, F.; Loch, S. D. Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 40, Issue 7 https://doi.org/10.1088/0953-4075/40/7/R01	journal	March 2007
Realization of Localized Bohr-Like Wave Packets Mestayer, J. J.; Wyker, B.; Lancaster, J. C. Physical Review Letters, Vol. 100, Issue 24 https://doi.org/10.1103/PhysRevLett.100.243004	journal	June 2008
Mixed quantum wave packet/classical trajectory treatment of the photodissociation process ArHCl→Ar+H+Cl García‐Vela, A.; Gerber, R. B.; Imre, D. G. The Journal of Chemical Physics, Vol. 97, Issue 10 https://doi.org/10.1063/1.463550	journal	November 1992
Field-ionization threshold and its induced ionization-window phenomenon for Rydberg atoms in a short single-cycle pulse Yang, B. C.; Robicheaux, F. Physical Review A, Vol. 90, Issue 6 https://doi.org/10.1103/PhysRevA.90.063413	journal	December 2014
Temporal dynamics of a two-electron wave packet Lyons, B. J.; Schumacher, D. W.; Duncan, D. I. Physical Review A, Vol. 57, Issue 5 https://doi.org/10.1103/PhysRevA.57.3712	journal	May 1998
Time propagation of extreme two-electron wavefunctions Robicheaux, F. Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 45, Issue 13 https://doi.org/10.1088/0953-4075/45/13/135007	journal	June 2012
Field ionization of Rydberg atoms in a single-cycle pulse Yang, B. C.; Robicheaux, F. Physical Review A, Vol. 91, Issue 4 https://doi.org/10.1103/PhysRevA.91.043407	journal	April 2015
Photoionization of helium by attosecond pulses: Extraction of spectra from correlated wave functions Argenti, Luca; Pazourek, Renate; Feist, Johannes Physical Review A, Vol. 87, Issue 5 https://doi.org/10.1103/PhysRevA.87.053405	journal	May 2013
Calculation of Matrix Elements for One‐Dimensional Quantum‐Mechanical Problems and the Application to Anharmonic Oscillators Harris, David O.; Engerholm, Gail G.; Gwinn, William D. The Journal of Chemical Physics, Vol. 43, Issue 5 https://doi.org/10.1063/1.1696963	journal	September 1965
Ionization of Rydberg Wave Packets by Subpicosecond, Half-Cycle Electromagnetic Pulses Raman, C.; Conover, C. W. S.; Sukenik, C. I. Physical Review Letters, Vol. 76, Issue 14 https://doi.org/10.1103/PhysRevLett.76.2436	journal	April 1996
Pulse-induced focusing of Rydberg wave packets Arbó, D. G.; Reinhold, C. O.; Burgdörfer, J. Physical Review A, Vol. 67, Issue 6 https://doi.org/10.1103/PhysRevA.67.063401	journal	June 2003
Propagation of double Rydberg wave packets Robicheaux, F.; Forrey, R. C. Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 38, Issue 2 https://doi.org/10.1088/0953-4075/38/2/027	journal	January 2005
Comparison of the propagation of semiclassical frozen Gaussian wave functions with quantum propagation for a highly excited anharmonic oscillator Kluk, Edward; Herman, Michael F.; Davis, Heidi L. The Journal of Chemical Physics, Vol. 84, Issue 1 https://doi.org/10.1063/1.450142	journal	January 1986
The semiclassical two-electron atom and the old quantum theory Leopold, J. G.; Percival, I. C. Journal of Physics B: Atomic and Molecular Physics, Vol. 13, Issue 6 https://doi.org/10.1088/0022-3700/13/6/012	journal	March 1980
Creating and Probing Electronic Wave Packets Using Half-Cycle Pulses Jones, R. R. Physical Review Letters, Vol. 76, Issue 21 https://doi.org/10.1103/PhysRevLett.76.3927	journal	May 1996
Comparison of different quantum mechanical methods for inner atomic shell photo-ionization followed by Auger decay Wang, Qianxia; Sheinerman, S.; Robicheaux, F. Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 47, Issue 21 https://doi.org/10.1088/0953-4075/47/21/215003	journal	October 2014

Similar Records

Ionization from Rydberg atoms and wave packets by scaled terahertz single-cycle pulses

Journal Article · Wed Mar 20 00:00:00 EDT 2019 · Physical Review A · OSTI ID:1540658

Wang, Xiao; Robicheaux, F.

Dynamics of Rydberg wave packets generated by half-cycle pulses

Journal Article · Mon Jul 01 00:00:00 EDT 1996 · Physical Review A · OSTI ID:1540658

Reinhold, C O; Burgdoerfer, J; Frey, M T; +1 more

Probing coordinates of Rydberg wave packets

Journal Article · Wed Aug 01 00:00:00 EDT 2001 · Physical Review A · OSTI ID:1540658

Tannian, B E; Stokely, C L; Dunning, F B; +2 more

Related Subjects

74 ATOMIC AND MOLECULAR PHYSICS
strong electromagnetic field effects
Rydberg atoms & molecules

Title: Probing double Rydberg wave packets in a helium atom with fast single-cycle pulses

Citation Formats

References (39)

Similar Records

Related Subjects